English

Cotunnite-structured titanium dioxide: the hardest known oxide

Materials Science 2009-07-10 v1 Other Condensed Matter

Abstract

Despite great technological importance and many investigations, a material with measured hardness comparable to that of diamond or cubic boron nitride has yet to be identified. Combined theoretical and experimental investigations led to the discovery of a new polymorph of titanium dioxide with titanium nine-coordinated to oxygen in the cotunnite (PbCl2) structure. Hardness measurements on the cotunnite-structured TiO2 synthesized at pressures above 60 GPa and temperatures above 1000 K reveal that this material is the hardest oxide yet discovered. Furthermore, it is one of the least compressible (with a measured bulk modulus of 431 GPa) and hardest (with a microhardness of 38 GPa) polycrystalline materials studied thus far.

Cite

@article{arxiv.0907.1464,
  title  = {Cotunnite-structured titanium dioxide: the hardest known oxide},
  author = {L. S. Dubrovinsky and N. A. Dubrovinskaia and V. Swamy and J. Muscat and N. M. Harrison and R. Ahuja and B. Holm},
  journal= {arXiv preprint arXiv:0907.1464},
  year   = {2009}
}

Comments

This is full version of the paper published as Brief Communications in Nature, 410, 653-654

R2 v1 2026-06-21T13:22:56.832Z