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A new iridium containing layered cuprate material, IrSr_2Sm_{1.15}Ce_{0.85}Cu_{2.175}O_{10, has been synthesized by conventional ambient-pressure solid-state techniques. The material's structure has been fully characterized by Rietveld…

Materials Science · Physics 2012-09-22 R. H. Colman , A. C. Mclaughlin

We theoretically investigate the low-temperature phase of the recently synthesized Lu$_2$Mo$_2$O$_5$N$_2$ material, an extraordinarily rare realization of a $S=1/2$ three-dimensional pyrochlore Heisenberg antiferromagnet in which Mo$^{5+}$…

We have investigated the dilute magnetic impurity effect on the magnetic properties of a quantum spin liquid candidate Ba3ZnRu2O9 and a spin gapped compound Ba3CaRu2O9. The magnetic ground state of each compound stands against 2%…

Strongly Correlated Electrons · Physics 2018-08-09 Takafumi D. Yamamoto , Hiroki Taniguchi , Ichiro Terasaki

Quantum spin liquids are long-range entangled states of matter with emergent gauge fields and fractionalized excitations. While candidate materials, such as the Kitaev honeycomb ruthenate $\alpha$-RuCl$_3$, show magnetic order at low…

Strongly Correlated Electrons · Physics 2019-07-16 I. Rousochatzakis , S. Kourtis , J. Knolle , R. Moessner , N. B. Perkins

Spin correlations of the frustrated pyrochlore oxide Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ have been investigated by using inelastic neutron scattering on single crystalline samples ($x=-0.007, 0.000,$ and $0.003$), which have the putative…

Strongly Correlated Electrons · Physics 2019-01-08 Hiroaki Kadowaki , Mika Wakita , Björn Fåk , Jacques Ollivier , Seiko Ohira-Kawamura , Kenji Nakajima , Jeffrey W. Lynn

^{139}La NMR measurements of La_{2/3}Ca_{1/3}MnO_3 performed in the paramagnetic state and high magnetic fields are reported. Analysis of the high temperature spectrum measured establishes that the spectrum it is a standard powder pattern…

Strongly Correlated Electrons · Physics 2009-10-31 K. E. Sakaie , C. P. Slichter , P. Lin , M. Jaime , M. B. Salamon

Magnetic properties of a one-dimensional frustrated quantum spin system Rb2Cu2Mo3O12 is investigated by the muon spin relaxation (muSR) technique. Although this system shows an incommensurate spin correlation in neutron scattering, it has…

Strongly Correlated Electrons · Physics 2018-04-04 Seiko Ohira-Kawamura , Keisuke Tomiyasu , Akihiro Koda , Dita P. Sari , Retno Asih , Sungwon Yoon , Isao Watanabe , Kenji Nakajima

We combine ultra-high-resolution inelastic neutron scattering and quantum Monte Carlo simulations to study thermodynamics and spin excitations in the spin-supersolid phase of the triangular lattice XXZ antiferromagnet K$_2$Co(SeO$_3$)$_2$…

$\gamma$-${\rm Ba}_{3}{\rm CoNb}_{2}{\rm O}_{9}$ realizes a disordered simple-cubic spin-$1/2$ lattice in which Co$^{2+}$ ions randomly occupy one third of the sites, placing the system close to the site-percolation threshold for magnetic…

We report magnetization, heat capacity, 7Li - nuclear magnetic resonance (NMR), and muSR (muon spin roration) measurements on the honeycomb 4d5 spin liquid candidate Li2RhO3. The magnetization in small magnetic fields provides evidence of…

Strongly Correlated Electrons · Physics 2017-09-27 P. Khuntia , S. Manni , F. R. Foronda , T. Lancaster , S. J. Blundell , P. Gegenwart , M. Baenitz

Quantum spin liquids (QSLs) are an exotic state of matter that is subject to extensive research. However, the relationship between the ubiquitous disorder and the QSL behaviors is still unclear. Here, by performing comparative experimental…

Frustration-induced strong quantum fluctuations accompanied by spin-orbit coupling and crystal electric field can give rise to rich and diverse magnetic phenomena associated with unconventional low-energy excitations in rare-earth based…

Strongly Correlated Electrons · Physics 2024-02-13 J. Khatua , S. Bhattacharya , A. M. Strydom , A. Zorko , J. S. Lord , A. Ozarowski , E. Kermarrec , P. Khuntia

We report the observation of a frequency shift and splitting of the electron spin resonance (ESR) mode of the low-dimensional S=1/2 frustrated antiferromagnet Cs2CuCl4 in the spin-correlated state below the Curie-Weiss temperature 4 K but…

Strongly Correlated Electrons · Physics 2015-03-18 K. Yu. Povarov , A. I. Smirnov , O. A. Starykh , S. V. Petrov , A. Ya. Shapiro

We have studied spin relaxation in the spin ice compound Dy2Ti2O7 through measurements of the a.c. magnetic susceptibility. While the characteristic spin relaxation time is thermally activated at high temperatures, it becomes almost…

Materials Science · Physics 2009-11-10 J. Snyder , B. G. Ueland , J. S. Slusky , H. Karunadasa , R. J. Cava , Ari Mizel , P. Schiffer

Tb2Ti2O7 is a pyrochlore antiferromagnet that has dynamical spins and only short-range correlations even at 50 mK; the lowest temperature explored so far, which is much smaller than the scale set by the Curie-Weiss temperature T_{CW}~14 K.…

Statistical Mechanics · Physics 2009-12-16 Hamid R. Molavian , Paul A. McClarty , Michel J. P. Gingras

We investigate the electronic structure of BaIrO3, an interesting compound exhibiting charge density wave transition in its insulating phase and ferromagnetic transition at the same temperature, using full potential linearized augmented…

Strongly Correlated Electrons · Physics 2009-11-11 Kalobaran Maiti

We study the spin dynamics in the quasi-2D spin-$1/2$ dimer compound Ba$_2$CuSi$_2$O$_6$Cl$_2$, which exhibits a magnetic field-induced Bose-Einstein condensate (BEC) of triplons. Using nuclear magnetic resonance (NMR) spin-lattice…

The frustrated pyrochlore iridate Pr$_2$Ir$_2$O$_7$ was proposed as a metallic quantum spin liquid located at a zero-field quantum critical point. Here we present the ultralow-temperature thermal conductivity measurements on the…

Strongly Correlated Electrons · Physics 2022-08-23 J. M. Ni , Y. Y. Huang , E. J. Cheng , Y. J. Yu , B. L. Pan , Q. Li , L. M. Xu , Z. M. Tian , S. Y. Li

The nature of the magnetic ground state of highly frustrated systems remained puzzling to this day. Here, we have performed multifrequency electron spin resonance (ESR) measurements on a putative quantum spin liquid compound…

We have performed field-swept 59Co NMR measurements on the 'exotic' spin-chain material, Ca3Co2O6, crystallizing in K4CdCl6-type rhombohedral structure, believed to exhibit two magnetic transition temperatures (around 24 and 12 K). This is…

Strongly Correlated Electrons · Physics 2009-11-10 E. V. Sampathkumaran , N. Fujiwara , S. Rayaprol , P. K. Madhu , Y. Uwatoko