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Recently, there have been contrary claims of Kitaev spin-liquid behaviour and ordered behavior in the honeycomb compound Ag$_3$LiIr$_2$O$_6$ based on various experimental signatures. Our investigations on this system reveal a…

The layered triangular lattice owing to $1:2$ order of $B$ and $B'$ sites in the triple perovskite $A_3 B B'_2$O$_9$ family provides an enticing domain for exploring the complex phenomena of quantum spin liquids (QSLs). We report a…

Strongly Correlated Electrons · Physics 2024-08-07 K. Bhattacharya , S. Mohanty , A. D. Hillier , M. T. F. Telling , R. Nath , M. Majumder

The triangular-lattice system $\alpha$-RuI$_3$ is isostructural to the widely-studied $\alpha$-RuCl$_3$ compound which was identified as a potential Kitaev system but exhibits, instead of spin liquid behaviour, a magnetically ordered…

Strongly Correlated Electrons · Physics 2024-06-07 Hank C. H. Wu , Benjamin M. Huddart , Francis L. Pratt , Danrui Ni , Robert J. Cava , Stephen J. Blundell

We carried out AC magnetic susceptibility measurements and muon spin relaxation spectroscopy on the cubic double perovskite Ba2YMoO6, down to 50 mK. Below ~1 K the muon relaxation is typical of a magnetic insulator with a spin-liquid type…

Strongly Correlated Electrons · Physics 2013-06-03 M. A. de Vries , J. O. Piatek , M. Misek , J. S. Lord , H. M. Ronnow , J. -W. G. Bos

Quantum spin liquid represents an intriguing state where electron spins are highly entangled yet spin fluctuation persists even at 0 K. Recently, the hexaaluminates \textit{R}MgAl$_{11}$O$_{19}$ (\textit{R} = rare earth) have been proposed…

Strongly Correlated Electrons · Physics 2025-04-01 Yantao Cao , Akihiro Koda , M. D. Le , V. Pomjakushin , Benqiong Liu , Zhendong Fu , Zhiwei Li , Jinkui Zhao , Zhaoming Tian , Hanjie Guo

A recently discovered material, 6H-B-Ba3NiSb2O9 was found to display unusual low-temperature phenomenology, interpreted as a quantum spin liquid with spin S = 1 on a triangular lattice. We study a spin S = 1 quantum exchange model on an AB…

Strongly Correlated Electrons · Physics 2012-08-27 Gang Chen , Michael Hermele , Leo Radzihovsky

We report the structural transformation of hexagonal Ba3YIr2O9 to a cubic double perovskite form (stable in ambient conditions) under an applied pressure of 8GPa at 1273K. While the ambient pressure (AP) synthesized sample undergoes…

Strongly Correlated Electrons · Physics 2013-10-28 Tusharkanti Dey , A. V. Mahajan , R. Kumar , B. Koteswararao , F. C. Chou , A. A. Omrani , H. M. Ronnow

Quantum spin liquids (QSLs) represent a novel state where spins are highly entangled but do not order even at zero temperature due to strong quantum fluctuations. Such a state is mostly studied in Heisenberg models defined on geometrically…

The signature for a non-Fermi liquid behavior near a quantum phase transition has been observed in thermal and transport properties of many metallic systems at low temperatures. In the present work we consider specific examples of itinerant…

Strongly Correlated Electrons · Physics 2009-10-30 Suresh G. Mishra , P. A. Sreeram

DC-magnetization data measured down to 40 mK speak against conventional freezing and reinstate YbMgGaO$_4$ as a triangular spin-liquid candidate. Magnetic susceptibility measured parallel and perpendicular to the $c$-axis reaches constant…

We investigate via exact diagonalization of finite clusters the electronic structure and magnetism of M$_2$O$_9$ dimers in the mixed-valence hexagonal perovskites A$_3$B'M$_2$O$_9$ for various different fillings of 4$d$ and 5$d$…

Strongly Correlated Electrons · Physics 2021-01-04 Ying Li , Alexander A. Tsirlin , Tusharkanti Dey , Philipp Gegenwart , Roser Valenti , Stephen M. Winter

We have performed thermodynamic and neutron scattering measurements on the S=1/2 kagome lattice antiferromagnet Zn Cu_3 (OH)_6 Cl_2. The susceptibility indicates a Curie-Weiss temperature of ~ -300 K; however, no magnetic order is observed…

Strongly Correlated Electrons · Physics 2007-05-23 J. S. Helton , K. Matan , M. P. Shores , E. A. Nytko , B. M. Bartlett , Y. Yoshida , Y. Takano , A. Suslov , Y. Qiu , J. -H. Chung , D. G. Nocera , Y. S. Lee

We report the structural and magnetic properties of the 4}\textit{\textcolor{black}{d }}\textcolor{black}{(M = Rh) based and 5}\textit{\textcolor{black}{d }}\textcolor{black}{(M = Ir) based systems Ba$_{3}$M$_{x}$Ti$_{3-x}$O$_{9}$…

Strongly Correlated Electrons · Physics 2017-08-03 R. Kumar , D. Sheptyakov , P. Khuntia , K. Rolfs , P. G. Freeman , H. M. Rønnow , Tusharkanti Dey , M. Baenitz , A. V. Mahajan

We have studied the low temperature a.c. magnetic susceptibility of the diluted spin ice compound Dy(2-x)MxTi2O7, where the magnetic Dy ions on the frustrated pyrochlore lattice have been replaced with non-magnetic ions, M = Y or Lu. We…

Materials Science · Physics 2007-05-23 J. Snyder , B. G. Ueland , Ari Mizel , J. S. Slusky , H. Karunadasa , R. J. Cava , P. Schiffer

We study the low-temperature physics of the $SU(2)$-symmetric spin-$1/2$ Heisenberg antiferromagnet on a pyrochlore lattice and find fingerprint evidence for the thermal spin-ice state in this frustrated quantum magnet. Our conclusions are…

Strongly Correlated Electrons · Physics 2016-05-04 Yuan Huang , Kun Chen , Youjin Deng , Nikolay Prokof'ev , Boris Svistunov

We present a muon spin relaxation study on the Ising pyrochlore Nd$_2$Zr$_2$O$_7$ which develops an "all-in-all-out" magnetic order below 0.4~K. At 20~mK far below the ordering transition temperature, the zero-field muon spin relaxation…

Materials Science · Physics 2016-09-07 J. Xu , C. Balz , C. Baines , H. Luetkens , B. Lake

The three-dimensional $S = {\frac{1}{2}}$ system Y$_{3}$Cu$_{2}$Sb$_{3}$O$_{14}$ consists of two inequivalent Cu$^{2+}$ sites, each forming an edge shared triangular lattice. Our magnetic susceptibility $\chi(T)$, specific heat $C_p(T)$,…

The rare-earth-based geometrically frustrated triangular magnets have attracted considerable attention due to the intricate interplay between strong spin-orbit coupling and the crystal electric field (CEF), which often leads to effective…

Inelastic neutron scattering technique is employed to investigate the paramagnetic spin dynamics in a single crystalline sample of the magnetocaloric compound MnFe$_4$Si$_3$. In the investigated temperature range, 1.033$\times T_{C}$ to…

Materials Science · Physics 2025-02-21 N. Biniskos , K. Schmalzl , J. Persson , S. Raymond

Quantum spin liquids~(QSLs) represent a unique quantum disordered state of matter that hosts long-range quantum entanglement and fractional excitations. However, structural disorder resulting from site mixing between different types of ions…