Related papers: Gain and loss in open quantum systems
Photosystems II and I (PSII and PSI) are the reaction centre complexes that drive the light reactions of photosynthesis. PSII performs light-driven water oxidation (quantum efficiencies and catalysis rates of up to 80% and 1000…
Unitary transformations are routinely modeled and implemented in the field of quantum optics. In contrast, nonunitary transformations that can involve loss and gain require a different approach. In this theory work, we present a universal…
We show that quantum optical systems preserving the total number of excitations admit a simple classification of possible resonant transitions (including effective), which can be classified by analizying the free Hamiltonian and the…
We analyze a theoretical model for energy and electron transfer in an artificial photosynthetic system. The photosystem consists of a molecular triad (i.e., with a donor, a photosensitive unit, and an acceptor) coupled to four accessory…
The description of an open quantum system's decay almost always requires several approximations as to remain tractable. Here, we first revisit the meaning, domain and seeming contradictions of a few of the most widely used of such…
We study light propagation in a photonic system that shows stepwise evolution in a discretized environment. It resembles a discrete-time version of photonic waveguide arrays or quantum walks. By introducing controlled photon losses to our…
Using a density matrix approach, we study the simplest systems that display both gain and feedback: clusters of 2 to 5 atoms, one of which is pumped. The other atoms supply feedback through multiple scattering of light. We show that, if the…
The coherent energy transfer between a quantum charger and a quantum battery is analyzed. In particular, we study how to improve the direct energy transfer by adding a photonic cavity as a mediator. We show that the additional degree of…
Photoinduced biological processes occur via one photon absorption in natural light, which is weak, CW and incoherent, but are often studied in the laboratory using pulsed coherent light. Here we compare the response of a molecule to these…
The spontaneous decay of an excited atom by photon emission is one of the most common and elementary physical process present in nature and in laboratories. The decay is random in time with constant probability density, as it can be…
Photoemission experiments involve the motion of an electron near a conducting surface. This necessarily generates heat by ohmic losses from eddy currents. This inelastic scattering of the electrons will result in a downward shift in…
Photosystem II (PSII) reaction center is a unique protein-chromophore complex that is capable of efficiently separating electronic charges across the membrane after photoexcitation. In the PSII reaction center, the primary energy- and…
We explore energy transfer in a generic three-level system, which is coupled to three non-equilibrium baths. Built on the concept of quantum heat engine, our three-level model describes non-equilibrium quantum processes including…
Photosynthesis, the process by which energy from sunlight drives cellular metabolism, relies on a unique organization of light-harvesting and reaction center complexes. Recently, the organization of light-harvesting LH2 complexes and…
During the first steps of photosynthesis, the energy of impinging solar photons is transformed into electronic excitation energy of the light-harvesting biomolecular complexes. The subsequent energy transfer to the reaction center is…
We model energy transfer between two coupled four-level chromophores with arbitrarily spaced energy levels. Our analysis takes into account the crucial---yet often ignored---process of initial excitation by light that is incident on the…
Multi-photon processes are the essence of nonlinear optics. Optical harmonics generation and multi-photon absorption, ionization, polymerization or spectroscopy are widely used in practical applications. Generally, the rate of an n-photon…
Excitonic transport in photosynthesis exhibits a wide range of time scales. Absorption and initial relaxation takes place over tens of femtoseconds. Excitonic lifetimes are on the order of a nanosecond. Hopping rates, energy differences…
Elementary physics of photovoltaic energy conversion in a two-level atomic PV is considered. We explain the conditions for which the Carnot efficiency is reached and how it can be exceeded! The loss mechanisms - thermalization, angle…
A model of charge separation in quantum photosynthesis as a model of quantum feedback control in a system of interacting excitons and vibrons is introduced. Quantum feedback in this approach describes the Landau--Zener transition with…