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The use of energy conservation arguments is ubiquitous in understanding the process of high harmonic generation, yet a complete quantum optical description of exact photon number exchange remained elusive. Here, we solve this gap in…

Quantum Physics · Physics 2026-03-24 Philipp Stammer

The high quantum efficiency of photosynthetic complexes has inspired researchers to explore new routes to utilize this process for photovoltaic devices. Quantum coherence has been demonstrated to play a crucial role within this process.…

Chemical Physics · Physics 2015-06-23 Yiteng Zhang , Sangchul Oh , Fahhad H. Alharbi , Greg Engel , Sabre Kais

Dynamics of open quantum systems depends on different types of initial correlations. On the one hand, when system and environment are both inherently multipartite, initial correlations between the parties of the composite environment make…

Quantum Physics · Physics 2020-05-06 Sina Hamedani Raja , K P Athulya , Anil Shaji , Jyrki Piilo

The striking efficiency of energy transfer in natural photosynthetic systems and the recent evidence of long-lived quantum coherence in biological light harvesting complexes has triggered much excitement, due to the evocative possibility…

Mesoscale and Nanoscale Physics · Physics 2015-10-13 Yonatan Dubi

The quantum dynamics of entanglement is widely revealed in photosynthetic light-harvesting complexes. Different from the previous work, we explore the properties of exciton transport and photosynthesis assisted by the quantum entanglement…

Applied Physics · Physics 2024-03-12 Lu-Xin Xu , Shun-Cai Zhao , Ling-Fang Li

We consider a coherent state of light propagating through an ensemble of two-level atoms where all the atoms are initially in their ground state. In ordinary absorption, the transition of atoms to their excited state along with the…

Quantum Physics · Physics 2019-07-31 I. C. Nodurft , R. A. Brewster , T. B. Pittman , J. D. Franson

We theoretically investigate exciton relaxation dynamics in molecular aggregates based on model photosynthetic complexes under various conditions of incoherent excitation. We show that noise-induced quantum coherence is generated between…

Biological Physics · Physics 2014-08-14 Dmitri V. Voronine , Konstantin E. Dorfman , Bin Cao , Amitabh Joshi

A simple model is constructed to describe dissociation of charge transfer excitons in bulk heterojunction solar cells, and its dependence on the physical parameters of the system. In bulk heterojunction organic photovoltaics (OPVs), exciton…

Strongly Correlated Electrons · Physics 2017-08-23 Guangqi Li , Abraham Nitzan , Mark A. Ratner

Biological molecular machines are enzymes that simultaneously catalyze two processes, one donating free energy and second accepting it. Recent studies show that most native protein enzymes have a rich stochastic dynamics that often…

Biological Physics · Physics 2018-12-21 Michal Kurzynski , Przemyslaw Chelminiak

Frequency up-conversion of few low-energy photons into a single high-energy photon, greatly contributes to imaging, light sources, detection and other fields of research. However, it offers negligible efficiency when up-converting many…

Optics · Physics 2013-06-11 Assaf Manor , Nimrod Kruger , Carmel Rotschild

We investigate the nonequilibrium thermodynamics of pure decoherence. In a pure decoherence process, the system Hamiltonian is a constant of motion and there is no direct energy exchange between the system and its surroundings.…

Quantum Physics · Physics 2023-04-20 Maria Popovic , Mark T. Mitchison , John Goold

Recently it has been discovered---contrary to expectations of physicists as well as biologists---that the energy transport during photosynthesis, from the chlorophyll pigment that captures the photon to the reaction centre where glucose is…

Quantum Physics · Physics 2015-05-27 Apoorva D. Patel

All natural things process and transform information. They receive environmental information as input, and transform it into appropriate output responses. Much of science is dedicated to building models of such systems -- algorithmic…

Quantum Physics · Physics 2017-02-14 Jayne Thompson , Andrew J. P. Garner , Vlatko Vedral , Mile Gu

Strong interaction between the light field and an atom is often achieved with cavities. Recent experiments have used a different configuration: a propagating light field is strongly focused using a system of lenses, the atom being supposed…

Quantum Physics · Physics 2011-08-11 Colin Teo , Valerio Scarani

It is commonly believed that decoherence is the main obstacle to quantum information processing. In contrast to this, we show how decoherence in the form of dissipation can improve the performance of certain quantum gates. As an example we…

Quantum Physics · Physics 2007-05-23 Almut Beige , Hugo Cable , Carsten Marr , Peter L. Knight

In this letter, we describe the modified decay rate and photonic Lamb (frequency) shift of quantum emitters in terms of the resonant states of a neighboring photonic resonator. This description illustrates a fundamental distinction in the…

Optics · Physics 2018-04-25 Emmanuel Lassalle , Nicolas Bonod , Thomas Durt , Brian Stout

Bose condensed light can form new phases [1] in a dye filled cavity due to the presence of the orientational disorder created by dye molecules which are essentially frozen on the time scale of the photonic thermalization (few ps). At longer…

Quantum Gases · Physics 2020-05-06 Victor Fleurov , Anatoly B. Kuklov

We develop a method to simulate the excitonic dynamics of realistic photosynthetic light harvesting systems including non-Markovian coupling to phonon degrees of freedom, under excitation by N-photon Fock state pulses. This method combines…

Biological Physics · Physics 2023-06-27 Liwen Ko , Robert L. Cook , K. Birgitta Whaley

We introduce a mathematically rigorous analysis of a generalized spin-boson system for the treatment of a donor-acceptor (reactant-product) quantum system coupled to a thermal quantum noise. The donor/acceptor probability dynamics describes…

Mathematical Physics · Physics 2012-09-05 Marco Merkli , Gennady Berman , Richard Sayre

Recently, we have theoretically proposed and experimentally demonstrated an exact and efficient quantum simulation of photosynthetic light harvesting in nuclear magnetic resonance (NMR), cf. B. X. Wang, \textit{et al.} npj Quantum…