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As a way to further improve the electronic properties of group V layered semiconductors, we propose to form in-layer 2D heterostructures of black phosphorus and grey arsenic. We use \textit{ab initio} density functional theory to optimize…

Mesoscale and Nanoscale Physics · Physics 2015-10-28 Zhen Zhu , Jie Guan , David Tomanek

Quasi free standing monolayer graphene (QFMLG) grown on SiC by selective Si evaporation from the Si-rich SiC(0001) face and H intercalation displays irregularities in STM and AFM analysis, appearing as localized features, which we…

Mesoscale and Nanoscale Physics · Physics 2018-04-27 Tommaso Cavallucci , Yuya Murata , Makoto Takamura , Hiroki Hibino , Stefan Heun , Valentina Tozzini

Screening in reduced dimensions has strong consequences on the electronic properties in van der Waals semiconductors, impacting the quasiparticle band gap and exciton binding energy. Screening in these materials is typically treated…

The interlayer breathing and shear modes in few-layer black phosphorus are investigated for their symmetry and lattice dynamical properties. The symmetry groups for the even-layer and odd-layer few-layer black phosphorus are utilized to…

Materials Science · Physics 2014-12-25 Jin-Wu Jiang , Bing-Shen Wang , Harold S. Park

We explore the oxidation of a single layer of black phosphorous using ab initio density functional theory calculation. We search for the equilibrium structures of phosphorene oxides, PO$_x$ with various oxygen concentrations $x$…

Materials Science · Physics 2020-07-22 Seoung-Hun Kang , Jejune Park , Sungjong Woo , Young-Kyun Kwon

Understanding how foreign chemical species bond to atomic vacancies in graphene layers can advance our ability to tailor the electronic and magnetic properties of defective graphenic materials. Here we use ultra-high vacuum scanning…

Materials Science · Physics 2014-04-07 Maxim Ziatdinov , Shintaro Fujii , Koichi Kusakabe , Manabu Kiguchi , Takehiko Mori , Toshiaki Enoki

Few-layer black phosphorus was recently rediscovered as a narrow-bandgap atomically thin semiconductor and has already attracted unprecedented attention due to its interesting properties. One feature of this material that sets it apart from…

Mesoscale and Nanoscale Physics · Physics 2017-04-04 Artem Mishchenko , Yang Cao , Geliang Yu , Colin R. Woods , Roman V. Gorbachev , Kostya S. Novoselov , Andre K. Geim , Leonid S. Levitov

This paper presents a DFT study for phosphine adsorption on a Si(001)-2$\times$1 surface covered by a chlorine monolayer, including adsorption on local defects, i.e. mono- and bivacancies in the adsorbate layer (Cl, Cl$_2$), and combined…

Materials Science · Physics 2019-01-04 Tatiana V. Pavlova , Georgy M. Zhidomirov , Konstantin N. Eltsov

Black phosphorene is not stable at ambient conditions, so atomic defects and oxidation effects are unavoidable in black phosphorus samples in the experiment. The effects of these defects on the performance of the black phosphorus…

Materials Science · Physics 2017-04-05 Cui-Xia Wang , Chao Zhang , Jin-Wu Jiang , Timon Rabczuk

Raman scattering and photoluminescence spectroscopy are used to investigate the optical properties of single layer black phosphorus obtained by mechanical exfoliation of bulk crystals under an argon atmosphere. The Raman spectroscopy,…

Mesoscale and Nanoscale Physics · Physics 2016-03-23 A. Surrente , A. A. Mitioglu , K. Galkowski , W. Tabis , D. K. Maude , P. Plochocka

We investigate theoretically the effects of modulated periodic perpendicular magnetic fields on the electronic states and optical absorption spectrum in a monolayer black phosphorus (phosphorene). We demonstrate that different phosphorene…

Mesoscale and Nanoscale Physics · Physics 2018-04-04 X. J. Li , J. H. Yu , Z. H. Wu , W. Yang

Using detailed first-principles calculations, we investigate the hopping rate of vacancies in phosphorene, an emerging elemental 2D material besides graphene. Our work predicts that a direct observation of these mono-vacancies (MVs),…

Materials Science · Physics 2017-04-25 Yongqing Cai , Qingqing Ke , Gang Zhang , Boris I. Yakobson , Yong-Wei Zhang

We study the stability and electronic properties of intrinsic point defects, vacancy and self-interstitial, in mono- and bi-layer phosphorene. We calculate the formation energies, quasiparticle defect states and charge transition levels…

Materials Science · Physics 2020-07-01 Sudipta Kundu , Mit H. Naik , Manish Jain

By performing \emph{ab initio} calculations for one- to four-layer black phosphorus within the $GW$ approximation, we obtain a significant difference in the band gap ($\sim$1.5 eV), which is in line with recent experimental data. The…

Materials Science · Physics 2014-06-25 Alexander N. Rudenko , Mikhail I. Katsnelson

A single atomic layer of black phosphorus, phosphorene, was experimentally realized in 2014. It has a puckered honeycomb lattice structure and a semiconducting electronic structure. In the first part of this paper, we use a simple LCAO…

Mesoscale and Nanoscale Physics · Physics 2015-10-22 Shuhei Fukuoka , Toshihiro Taen , Toshihito Osada

We theoretically explore the effect of metal and disulphur vacancies on electronic and optical properties of MoS$_2$ and WS$_2$ monolayers based on a Slater-Koster tight-binding model and including the spin-orbit coupling. We show that the…

Mesoscale and Nanoscale Physics · Physics 2018-05-25 Saboura Salehi , Alireza Saffarzadeh

Two-dimensional crystals are emerging materials for nanoelectronics. Development of the field requires candidate systems with both a high carrier mobility and, in contrast to graphene, a sufficiently large electronic bandgap. Here we…

Materials Science · Physics 2014-07-08 Jingsi Qiao , Xianghua Kong , Zhi-Xin Hu , Feng Yang , Wei Ji

Semi-metallic graphene and semiconducting monolayer transition metal dichalcogenides (TMDCs) are the two-dimensional (2D) materials most intensively studied in recent years. Recently, black phosphorus emerged as a promising new 2D material…

Mesoscale and Nanoscale Physics · Physics 2014-11-07 Xiaomu Wang , Aaron M. Jones , Kyle L. Seyler , Vy Tran , Yichen Jia , Huan Zhao , Han Wang , Li Yang , Xiaodong Xu , Fengnian Xia

We experimentally determine the lattice dynamics of black phosphorus layered crystals through a combination of x-ray diffuse scattering and inelastic x-ray scattering, and we rationalize our experimental findings using $\textit{ab initio}$…

Using density functional tight-binding theory, we investigated the elastic properties and deformation and failure behaviors of pristine and defective carbon-phosphide (CP) monolayers subjected to uniform uniaxial tensile strain along…

Materials Science · Physics 2018-09-26 V. Sorkin , Y. W. Zhang