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We investigate the crystal electric field (CEF) excitations of Yb$^{3+}$ ions in powder samples of the triangular-lattice rare-earth-based antiferromagnet YbZn$_2$GaO$_5$ using inelastic neutron scattering (INS). Three CEF excitations from…

Strongly Correlated Electrons · Physics 2025-07-18 Leshan Zhao , Tong Chen , Matthew B. Stone , Qiang Zhang , Colin L. Sarkis , S. M. Koohpayeh , Collin Broholm

Very recently we revealed a large family of triangular lattice quantum spin liquid candidates named rare-earth chalcogenides, which features a high-symmetry structure without structural/charge disorders and spin impurities, and may serve as…

We use inelastic neutron scattering to study the crystalline electric field (CEF) excitations of Ce$^{3+}$ in CeFeAsO$_{1-x}$F$_{x}$($x=0,0.16$). For nonsuperconducting CeFeAsO, the Ce CEF levels have three magnetic doublets in the…

We report a comprehensive experimental investigation of the structural, thermodynamic, static, and dynamic properties of a triangular lattice antiferromagnet Rb$_3$Yb(VO$_4$)$_2$. Through the analysis of magnetic susceptibility,…

Materials Science · Physics 2025-06-10 Sebin J. Sebastian , R. Kolay , Abhidev. B , Q. -P. Ding , Y. Furukawa , R. Nath

We present the low-temperature magnetic properties of two Yb$^{3+}$-based triangular lattice compounds NaSrYb(BO$_3$)$_2$ and K$_3$YbSi$_2$O$_7$ via thermodynamic measurements followed by crystal electric field (CEF) calculations.…

Materials Science · Physics 2025-01-27 S. Guchhait , R. Kolay , A. Magar , R. Nath

Recently reported van der Waals layered honeycomb rare-earth chalcohalides REChX (RE = rare earth, Ch = chalcogen, and X = halogen) are considered to be promising Kitaev spin liquid (KSL) candidates. The high-quality single crystals of…

Strongly Correlated Electrons · Physics 2024-10-28 Yanzhen Cai , Wei Ren , Xijing Dai , Jing Kang , Weizhen Zhuo , Mingtai Xie , Anmin Zhang , Jianting Ji , Feng Jin , Zheng Zhang , Qingming Zhang

The interplay of magnetic correlations, crystal electric field interactions, and spin-orbit coupling in low-dimensional frustrated magnets fosters novel ground states with unusual excitations. Here, we report the magnetic properties and…

Materials Science · Physics 2024-09-02 S. Guchhait , A. Painganoor , S. S. Islam , J. Sichelschmidt , M. D. Le , N. B. Christensen , R. Nath

In this paper, we performed thermodynamic and electron spin resonance (ESR) measurements to study low-energy magnetic excitations, which were significantly affected by crystalline electric field (CEF) excitations due to relatively small…

Strongly Correlated Electrons · Physics 2021-08-24 Weiwei Liu , Zheng Zhang , Dayu Yan , Jianshu Li , Zhitao Zhang , Jianting Ji , Feng Jin , Youguo Shi , Qingming Zhang

Inelastic neutron scattering measurement is performed on a breathing pyrochlore antiferromagnet Ba3Yb2Zn5O11. The observed dispersionless excitations are explained by a crystalline electric field (CEF) Hamiltonian of Kramers ion Yb3+ of…

Materials Science · Physics 2016-03-03 T. Haku , M. Soda , M. Sera , K. Kimura , S. Itoh , T. Yokoo , T. Masuda

The symmetry of local moments plays a defining role in the nature of exotic grounds states stabilized in frustrated magnetic materials. We present inelastic neutron scattering (INS) measurements of the crystal electric field (CEF)…

Disordered Systems and Neural Networks · Physics 2019-11-20 D. Reig-i-Plessis , A. Cote , S. van Geldern , R. D. Mayrhofer , A. A. Aczel , G. J. MacDougall

We investigate the magnetic and crystal electric field (CEF) states of the Kondo lattice system CeCuGa3 by muon spin relaxation (muSR), neutron diffraction, and inelastic neutron scattering (INS) measurements. A noncentrosymmetric…

Time-of-flight neutron spectroscopy has been used to determine the crystalline electric field (CEF) Hamiltonian, eigenvalues and eigenvectors appropriate to the $J$ = 7/2 Yb$^{3+}$ ion in the candidate quantum spin ice pyrochlore magnet…

Strongly Correlated Electrons · Physics 2016-03-09 J. Gaudet , D. D. Maharaj , G. Sala , E. Kermarrec , K. A. Ross , H. A. Dabkowska , A. I. Kolesnikov , G. E. Granroth , B. D. Gaulin

We have measured crystalline electric field (CEF) excitations of Nd3+ ions in the two-channel Kondo lattice candidates NdT2Zn20 (T = Co, Rh, and Ir) by means of inelastic neutron scattering (INS). In the INS measurements at 5 K,…

Strongly Correlated Electrons · Physics 2023-02-15 Rikako Yamamoto , Manh Duc Le , Devashibhai T. Adroja , Yasuyuki Shimura , Toshiro Takabatake , Takahiro Onimaru

We have measured the crystalline electric field (CEF) excitations of the CeMIn5 (M = Co, Rh, Ir) series of heavy fermion superconductors by means of inelastic neutron scattering. Fits to a CEF model reproduce the inelastic neutron…

Frustration, spin correlations and interplay between competing degrees of freedom are some of the key ingredients that underlie exotic states with fractional excitations in quantum materials. Rare-earth based two dimensional magnetic…

Strongly Correlated Electrons · Physics 2022-09-13 J. Khatua , M. Pregelj , A. Elghandour , Z. Jaglicic , R. Klingeler , A. Zorko , P. Khuntia

ErMgGaO$_4$ is a quantum antiferromagnet wherein the pseudospin-1/2 degrees of freedom of Er$^{3+}$ decorate two-dimensional triangular planes separated by disordered non-magnetic bilayers of Mg$^{2+}$ and Ga$^{3+}$. Unlike its sister…

The crystalline electric field (CEF) is investigated in Pr$_3$Pt$_{23}$Si$_{11}$ and Nd$_3$Pt$_{23}$Si$_{11}$ by neutron spectroscopy (NS). At low temperature, the number of observed CEF excitations is consistent with the orthorhombic…

Strongly Correlated Electrons · Physics 2016-12-13 R. M. Galéra , C. Opagiste , M. Amara , J. C. Toussaint , M. B. Lepetit , S. Rols

Magnetic order in most materials occurs when magnetic ions with finite moments in a crystalline lattice arrange in a particular pattern below the ordering temperature determined by exchange interactions between the ions. However, when the…

DC-magnetization data measured down to 40 mK speak against conventional freezing and reinstate YbMgGaO$_4$ as a triangular spin-liquid candidate. Magnetic susceptibility measured parallel and perpendicular to the $c$-axis reaches constant…

A layered triangular lattice with spin-1/2 ions is an ideal platform to explore highly entangled exotic states like quantum spin liquid (QSL). Here, we report a systematic in-field neutron scattering study on a perfect two-dimensional…

Strongly Correlated Electrons · Physics 2024-07-18 Tao Xie , Jie Xing , S. E. Nikitin , S. Nishimoto , M. Brando , P. Khanenko , J. Sichelschmidt , L. D. Sanjeewa , Athena S. Sefat , A. Podlesnyak
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