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The Tb$_2$Ti$_2$O$_7$ pyrochlore magnetic material is attracting much attention for its {\em spin liquid} state, failing to develop long range order down to 50 mK despite a Curie-Weiss temperature $\theta_{\rm CW} \sim -14$ K. In this paper…

Statistical Mechanics · Physics 2007-05-23 Hamid R. Molavian , Michel J. P. Gingras , Benjamin Canals

The pyrovanadate alpha-Cu2V2O7 belongs to the orthorhombic (Fdd2) class of crystals with noncentrosymmetric crystal structure. Recently, the compound has been identified to be a magnetic multiferroic with a substantial electric polarization…

Strongly Correlated Electrons · Physics 2016-11-23 A. Banerjee , J. Sannigrahi , S. Bhowal , I. Dasgupta , S. Majumdar , H. C. Walker , A. Bhattacharyya , D. T. Adroja

A quantum spin liquid is a novel state of matter characterized by quantum entanglement and the absence of any broken symmetry. In condensed matter, the frustrated rare-earth pyrochlore magnets Ho$_2$Ti$_2$O$_7$ and Dy$_2$Ti$_2$O$_7$,…

Strongly Correlated Electrons · Physics 2017-04-05 E. Kermarrec , J. Gaudet , K. Fritsch , R. Khasanov , Z. Guguchia , C. Ritter , K. A. Ross , H. A. Dabkowska , B. D. Gaulin

We report the low-temperature magnetothermal properties and spin dynamics of a mixed pyrochlore, Dy2GaSbO7 through the coordination of measurements of dc magnetization, ac susceptibility, and heat capacity, and CF computation. In Dy2GaSbO7,…

Materials Science · Physics 2021-04-19 Saikat Nandi , Yatramohan Jana , Jahangir Alam , Pallab Bag , S. S. Islam , Ramesh Nath

Pyrochlores offer an ideal playground to investigate the magnetic ground state of frustrated magnetic systems. In this class of materials, competition between various magnetic interactions remains frustrated and prevents an ordered magnetic…

Strongly Correlated Electrons · Physics 2022-10-06 Karan Singh , Dheeraj Ranaut , G. Sharma , K. Mukherjee

We report the anisotropic magnetic properties of Ho2Ge2O7 determined from dc and ac magnetization, specific heat and powder neutron diffraction experiments. The magnetic lanthanide sublattice, seen in our refinement of the tetragonal…

Other Condensed Matter · Physics 2009-11-13 E. Morosan , J. A. Fleitman , Q. Huang , J. W. Lynn , Y. Chen , X. Ke , M. L. Dahlberg , P. Schiffer , C. R. Craley , R. J. Cava

We use numerical linked cluster (NLC) expansions to compute the specific heat, C(T), and entropy, S(T), of a quantum spin ice model of Yb2Ti2O7 using anisotropic exchange interactions recently determined from inelastic neutron scattering…

Strongly Correlated Electrons · Physics 2012-10-11 R. Applegate , N. R. Hayre , R. R. P. Singh , T. Lin , A. G. R. Day , M. J. P. Gingras

We report magnetization and ac susceptibility of single crystals of the spin ice compound Dy2Ti2O7. Saturated moments at 1.8 K along the charasteristic axes [100] and [110] agree with the expected values for an effective ferromagnetic…

Strongly Correlated Electrons · Physics 2016-08-31 H. Fukazawa , R. G. Melko , R. Higashinaka , Y. Maeno , M. J. P. Gingras

Muon spin rotation and relaxation experiments in the pyrochlore iridate Eu2Ir2O7 yield a well-defined muon spin precession frequency below the metal-insulator/antiferromagnetic transition temperature TM = 120 K, indicative of long-range…

Strongly Correlated Electrons · Physics 2015-03-19 Songrui Zhao. J. M. Mackie , D. E. MacLaughlin , O. O. Bernal , J. J. Ishikawa , Y. Ohta , S. Nakatsuji

Nd2Hf2O7, belonging to the family of geometrically frustrated cubic rare earth pyrochlore oxides, was recently identified to order antiferromagnetically below T_N = 0.55 K with an all-in/all-out arrangement of Nd3+ moments, however with a…

Strongly Correlated Electrons · Physics 2017-12-15 V. K. Anand , D. L. Abernathy , D. T. Adroja , A. D. Hillier , P. K. Biswas , B. Lake

The pyrochlore magnet $\rm Yb_2Ti_2O_7$ has been proposed as a quantum spin ice candidate, a spin liquid state expected to display emergent quantum electrodynamics with gauge photons among its elementary excitations. However, $\rm…

Strongly Correlated Electrons · Physics 2018-06-20 Gabriele Sala , Dalini D. Maharaj , Matthew B. Stone , Hanna A. Dabkowska , Bruce D. Gaulin

The frustrated pyrochlore iridate Pr$_2$Ir$_2$O$_7$ was proposed as a metallic quantum spin liquid located at a zero-field quantum critical point. Here we present the ultralow-temperature thermal conductivity measurements on the…

Strongly Correlated Electrons · Physics 2022-08-23 J. M. Ni , Y. Y. Huang , E. J. Cheng , Y. J. Yu , B. L. Pan , Q. Li , L. M. Xu , Z. M. Tian , S. Y. Li

The XY pyrochlore Yb$_2$Ti$_2$O$_7$, with pseudo spin 1/2 at the Yb$^{3+}$ site, has been celebrated as potential host for the quantum spin ice state. The substitution of non-magnetic Ti with Pt gives Yb$_2$Pt$_2$O$_7$, a system with…

Strongly Correlated Electrons · Physics 2018-10-03 S. K. Takahashi , A. Arsenault , C. Mauws , A. M. Hallas , C. Sarkis , K. A. Ross , C. R. Wiebe , M. Tachibana , G. M. Luke , T. Imai

Magnetization and susceptibility studies on single crystals of the pyrochlore Ho$_{2}$Ti$_{2}$O$_{7}$ are reported for the first time. Magnetization isotherms are shown to be qualitatively similar to that predicted by the nearest neighbor…

Disordered Systems and Neural Networks · Physics 2009-11-07 A. L. Cornelius , J. S. Gardner

Muon spin relaxation measurements on some quantum spin ice candidate materials, the insulating pyrochlores Pr2B2O7 (B = Sn, Zr, Hf), have been performed for temperatures in the range 0.05-280 K. The results are indicative of a static…

Strongly Correlated Electrons · Physics 2015-06-22 F. R. Foronda , F. Lang , J. S. Möller , T. Lancaster , A. T. Boothroyd , F. L. Pratt , S. R. Giblin , D. Prabhakaran , S. J. Blundell

Quantum spin liquids with long-range entanglement are of great interest for applications in quantum technology. The quantum spin ice Pr$_2$Zr$_2$O$_7$ is a promising example, where it is believed that structural disorder plays a key role in…

From a microscopic model for the pyrochlore antiferromagnet Tb2Sn2O7, including the crystal field Hamiltonian and interactions between the angular momenta, we compute an effective pseudospin-1/2 Hamiltonian Heff$ that incorporates…

Statistical Mechanics · Physics 2010-11-30 Paul A. McClarty , Pawel Stasiak , Michel J. P. Gingras

Recent experiments suggest that the Ising pyrochlore magnets ${\rm Ho_{2}Ti_{2}O_{7}}$ and ${\rm Dy_{2}Ti_{2}O_{7}}$ display qualitative properties of the ferromagnetic nearest neighbor spin ice model proposed by Harris {\it et al.}, Phys.…

Disordered Systems and Neural Networks · Physics 2009-10-31 Michel J. P. Gingras , Byron C. den Hertog

The interplay of spin-orbit interactions and electronic correlations dominates the physical properties of pyrochlore iridates, R2Ir2O7 (R = Y, rare earth element), which are typically magnetic insulators. We report an…

Strongly Correlated Electrons · Physics 2015-06-03 T. F. Qi , O. B. Korneta , Xiangang Wan , L. E. DeLong , P. Schlottmann , G. Cao

Weak bond disorder disrupts the expected spin-liquid ground-state of the ideal $S$ = 1/2 Heisenberg pyrochlore antiferromagnet. Here we introduce a single crystal study of the structural and magnetic properties of the bond-disordered…

Strongly Correlated Electrons · Physics 2023-07-12 Andrej Kancko , Gerald Giester , Ross H. Colman