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We report a random singlet ground state in the $S=\frac{1}{2}$ Heisenberg pyrochlore antiferromagnet NaCdCu$_2$F$_7$. Cationic Na$^+$/Cd$^{2+}$ disorder on the pyrochlore $A$ site generates a broad distribution of…

Single phase polycrystalline sample of perovskite Sr2TiMnO6 (STMO) has been successfully synthesized via solid state reaction route. Its detailed structural and physical properties have been studied using x-ray diffraction, transmission…

Materials Science · Physics 2016-09-06 Shivani Sharma , R. Rawat , N. P. Lalla

Recent experiments on the spin-ice material Dy2Ti2O7 suggest that the Pauling "ice entropy", characteristic of its classical Coulombic spin-liquid state, may be lost at low temperatures [D. Pomaranski et al., Nature Phys. 9, 353 (2013)].…

Strongly Correlated Electrons · Physics 2015-09-16 Paul McClarty , Olga Sikora , Roderich Moessner , Karlo Penc , Frank Pollmann , Nic Shannon

We report the a.c. susceptibility study of Dy_xTb_{2-x}Ti_2O_7 with x in [0, 2]. In addition to the single-ion effect at Ts (single-ion effect peak temperature) corresponding to the Dy3+ spins as that in spin ice Dy_2Ti_2O_7 and a possible…

Materials Science · Physics 2015-03-13 Hui Xing , Mi He , Chunmu Feng , Hanjie Guo , Hao Zeng , Zhu-An Xu

The dipolar-octupolar (DO) pyrochlores, R$_2$M$_2$O$_7$ (R = Ce, Sm, Nd), are key players in the search for realizable novel quantum spin liquid (QSL) states as a large parameter space within the DO pyrochlore phase diagram is theorized to…

Neutron powder diffraction and inelastic measurements were performed examining the 5d pyrochlore Y$_2$Ir$_2$O$_7$. Temperature dependent measurements were performed between 3.4 K and 290 K, spanning the magnetic transition at 155 K. No sign…

Strongly Correlated Electrons · Physics 2014-05-30 M. C. Shapiro , S. C. Riggs , M. B. Stone , C. R. de la Cruz , S. Chi , A. A. Podlesnyak , I. R. Fisher

Recent work has highlighted remarkable effects of classical thermal fluctuations in the dipolar spin ice compounds, such as "artificial magnetostatics", manifesting as Coulombic power-law spin correlations and particles behaving as…

Strongly Correlated Electrons · Physics 2011-10-11 Kate A. Ross , Lucile Savary , Bruce D. Gaulin , Leon Balents

The pyrochlore materials have long been predicted to harbor a quantum spin liquid, an intrinsic long-range-entangled state supporting fractionalized excitations. Existing pyrochlore experiments, on the other hand, have discovered several…

Strongly Correlated Electrons · Physics 2019-08-19 Chunxiao Liu , Gábor B. Halász , Leon Balents

Using resonant magnetic x-ray scattering we address the unresolved nature of the magnetic groundstate and the low-energy effective Hamiltonian of Sm$_2$Ir$_2$O$_7$, a prototypical pyrochlore iridate with a finite temperature metal-insulator…

Strongly Correlated Electrons · Physics 2016-07-19 C. Donnerer , M. C. Rahn , M. Moretti Sala , J. G. Vale , D. Pincini , J. Strempfer , M. Krisch , D. Prabhakaran , A. T. Boothroyd , D. F. McMorrow

The pyrochlore compounds Ho2Ti2O7 and Dy2Ti2O7 show an exotic form of magnetism called the spin ice state, resulting from the interplay between geometrical frustration and ferromagnetic coupling. A fascinating feature of this state is the…

Materials Science · Physics 2013-09-11 D. P. Leusink , F. Coneri , M. Hoek , S. Turner , H. Idrissi , G. Van Tendeloo , H. Hilgenkamp

Frustration in magnetic interactions can give rise to disordered ground states with subtle and beautiful properties. The spin ices Ho2Ti2O7 and Dy2Ti2O7 exemplify this phenomenon, displaying a classical spin liquid state, with…

Strongly Correlated Electrons · Physics 2017-12-11 Mathieu Taillefumier , Owen Benton , Han Yan , L. D. C. Jaubert , Nic Shannon

We report our comprehensive study of physical properties of a ternary intermetallic compound PrIrSi3 investigated by dc magnetic susceptibility chi(T), isothermal magnetization M(H), thermo-remnant magnetization M(t), ac magnetic…

Strongly Correlated Electrons · Physics 2014-07-22 V. K. Anand , D. T. Adroja , A. Bhattacharyya , A. D. Hillier , J. W. Taylor , A. M. Strydom

The Co2V2O7 is recently reported to exhibit amazing magnetic field-induced magnetization plateaus and ferroelectricity, but its magnetic ground state remains ambiguous due to its structural complexity. Magnetometry measurements, and…

Strongly Correlated Electrons · Physics 2019-10-23 W. H. Ji , Y. C. Sun , C. M. N. Kumar , C. Li , S. Nandi , W. T. Jin , Y. Su , X. Sun , Y. Lee , B. Harmon , L. Ke , Z. W. Ouyang , Y. Xiao , Th. Brueckel

Disorder is ubiquitous in any quantum many-body system and is usually considered to be an obstacle to the elucidation of the underlying physics of complex systems, but its presence can often introduce exotic phases of matter that cannot…

Strongly Correlated Electrons · Physics 2024-07-31 S. M. Hossain , S. S. Rahaman , H. Gujrati , Dilip Bhoi , A. Matsuo , K. Kindo , M. Kumar , M. Majumder

We present results from muon spin relaxation/rotation, magnetization, neutron scattering and transport measurements on polycrystalline samples of the pyrochlore iridates Y2Ir2O7 (Y-227) and Yb2Ir2O7 (Yb-227). Well-defined spontaneous…

Strongly Correlated Electrons · Physics 2012-08-08 S. M. Disseler , Chetan Dhital , A. Amato , S. R. Giblin , Clarina de la Cruz , Stephen D. Wilson , M. J. Graf

We report detailed measurements of the low temperature magnetic phase diagram of Er$_2$Ti$_2$O$_7$. Heat capacity and time-of-flight neutron scattering studies of single crystals, subject to magnetic fields applied along the…

Strongly Correlated Electrons · Physics 2012-07-16 J. P. C. Ruff , J. P. Clancy , A. Bourque , M. A. White , M. Ramazanoglu , J. S. Gardner , Y. Qiu , J. R. D. Copley , H. A. Dabkowska , B. D. Gaulin

We report low-temperature powder X-ray and neutron diffraction studies on breathing pyrochlore magnets Cu$M$Cr$_{4}$S$_{8}$ ($M$ = Al, Ga), which undergo a magnetic transition at $T_{\rm N} \approx$ 21 and 31 K for {$M$ = Al and Ga,…

Materials Science · Physics 2024-05-09 Masaki Gen , Taro Nakajima , Hiraku Saito , Yusuke Tokunaga , Taka-hisa Arima

Quantum magnetic properties in a geometrically frustrated lattice of spin-1/2 magnet, such as quantum spin liquid or solid and the associated spin fractionalization, are considered key in developing a new phase of matter. The feasibility of…

Strongly Correlated Electrons · Physics 2018-03-21 J. Gunasekera , A. Dahal , Y. Chen , J. Rodriguez , L. Harriger , S. Thomas , T. Heitmann , V. Dugaev , A. Ernst , D. K. Singh

The magnetic behavior of single-crystal Ho$_2$PdSi$_3$, crystallizing in an AlB$_2$-derived hexagonal structure, is investigated by magnetic susceptibility ($\chi$) and electrical resistivity ($\rho$) measurements along two directions.…

Strongly Correlated Electrons · Physics 2009-11-07 E. V. Sampathkumaran , H. Bitterlich , K. K. Iyer , W. Löser , G. Behr

The complex metal oxides Mn2ASbO6 (A=In, Sc) with a corundum-related structure A3BO6 have been prepared as polycrystalline powders by a solid state reaction route. The crystal structure and magnetic properties have been investigated using a…

Materials Science · Physics 2011-11-21 S. A. Ivanov , P. Nordblad , R. Mathieu , R. Tellgren , E. Politova , G. André
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