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Water desalination by capacitive deionization (CDI) is performed via electrochemical cells consisting of two porous carbon electrodes. Upon transferring charge from one electrode to the other, ions are removed from the feedwater by…

Materials Science · Physics 2015-06-15 P. M. Biesheuvel , M. E. Suss , H. V. M. Hamelers

Capacitive deionization (CDI) is a fast-emerging technology most commonly applied to brackish water desalination. In CDI, salt ions are removed from the feedwater and stored in electric double layers (EDLs) within micropores of electrically…

Chemical Physics · Physics 2017-10-11 Matthew E. Suss

Many industrial and agricultural applications require the treatment of water streams containing high concentrations of ionic species for closing material cycles. High concentration factors are often desired, but hard to achieve with…

Several harmful or valuable ionic species present in sea, brackish and wastewaters are amphoteric, and thus their properties depend on the local water pH. Effective removal of these species can be challenging by conventional membrane…

Capacitive Deionization (CDI) is a non-energy intensive water treatment technology. To harness the enormous potential of CDI requires improving performance, while offering industrially feasible solutions. Following this idea, the…

We present porous electrode theory for capacitive deionization (CDI) with electrodes containing nanoparticles that consist of a redox-active intercalation material. A geometry of a desalination cell is considered which consists of two…

Chemical Physics · Physics 2019-12-24 K. Singh , H. J. M. Bouwmeester , L. C. P. M de Smet , M. Z. Bazant , P. M. Biesheuvel

Capacitive deionization (CDI) is a technology in which water is desalinated by ion electrosorption into the electric double layers (EDLs) of charging porous electrodes. In recent years significant advances have been made in modeling the…

Chemical Physics · Physics 2017-02-01 Amit N. Shocron , Matthew E. Suss

Faradaic deionization (FDI) is a promising technology for energy-efficient water desalination using porous electrodes containing redox-active materials. Herein, we demonstrate for the first time the capability of a symmetric FDI flow cell…

Chemical Physics · Physics 2023-06-09 Vu Q. Do , Erik R. Reale , Irwin C. Loud , Paul G. Rozzi , Haosen Tan , David A. Willis , Kyle C. Smith

Over the past decade, capacitive deionization (CDI) has realized a surge in attention in the field of water desalination and can now be considered as an important technology class, along with reverse osmosis and electrodialysis. While many…

A two-scale model is presented to simulate the dynamic ion transport and adsorption processes in porous electrodes used for capacitive deionization (CDI). At the pore scale, the Stokes equation governing water flow in porous CDI electrodes…

Fluid Dynamics · Physics 2022-01-14 Min Liu , John Waugh , Siddharth Komini Babu , Jacob S. Spendelow , Qinjun Kang

Flowing electrode capacitive deionization systems (FE-CDI) have recently garnered attention because of their ability to prevent cross contamination and operate in uninterrupted cycles ad infinitum. Typically, FE-CDI electrodes suffer from…

In the growing field of capacitive deionization (CDI), a number of performance metrics have emerged to describe the desalination process. Unfortunately, the separation conditions under which these metrics are measured are often not…

The rapid and efficient exchange of ions between porous electrodes and aqueous solutions is important in many applications, such as electrical energy storage by super-capacitors, water desalination and purification by capacitive…

Chemical Physics · Physics 2015-05-14 P. M. Biesheuvel , M. Z. Bazant

Freshwater scarcity demands desalination technologies that are efficient, scalable, and sustainable. Capacitive deionisation (CDI) is promising but remains limited by inefficient ion adsorption and poor charge utilisation. Here, we show…

Soft Condensed Matter · Physics 2026-04-20 Mamta Yadav , Clifford E. Woodward , Jan Forsman

Capacitive deionization (CDI) performance metrics can vary widely with operating methods. We here develop a theory around and experimentally demonstrate a new operation for CDI that uses sinusoidal forcing voltage (or sinusoidal current).…

Chemical Physics · Physics 2018-06-11 Ashwin Ramachandran , Steven A. Hawks , Michael Stadermann , Juan G. Santiago

Electrodes composed of activated carbon (AC) particles can desalinate water by ion electrosorption. To describe ion electrosorption mathematically, accurate models are required for the structure of the electrical double layers (EDLs) that…

Chemical Physics · Physics 2015-09-22 P. M. Biesheuvel

Electrochemical desalination devices that use redox-active cation intercalation electrodes show promise for desalination of salt-rich water resources with high water recovery and low energy consumption. While previous modeling and…

Applied Physics · Physics 2018-04-02 Sizhe Liu , Kyle C. Smith

The development of energy and infrastructure efficient water purification systems are among the most critical engineering challenges facing our society. Water purification is often a multi-step process involving filtration, desalination,…

Water scarcity is a dilemma facing much of the global population. Cation intercalation desalination (CID) cells, which use intercalation host compounds (IHCs) in combination with ion-exchange membranes (IEMs), could aid in addressing this…

Chemical Physics · Physics 2016-12-28 Kyle C. Smith

Capacitive mixing (CAPMIX) and capacitive deionization (CDI) are promising candidates for harvesting clean, renewable energy and for the energy efficient production of potable water, respectively. Both CAPMIX and CDI involve water-immersed…

Soft Condensed Matter · Physics 2016-08-08 Andreas Härtel , Mathijs Janssen , Sela Samin , René van Roij
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