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We combine ultrafast electron diffraction and time-resolved terahertz spectroscopy measurements to unravel the connection between structure and electronic transport properties during the photoinduced insulator-metal transitions in vanadium…

Femtosecond pulses have been used to reveal hidden broken symmetry states and induce transitions to metastable states. However, these states are mostly transient and disappear after laser removal. Photoinduced phase transitions towards…

Materials Science · Physics 2023-10-13 Stefano Mocatti , Giovanni Marini , Matteo Calandra

We study the effect of laser driving on a minimal model for a hexagonal two-dimensional material with broken inversion symmetry. Through the application of circularly polarised light and coupling to a thermal free electron bath, the system…

Strongly Correlated Electrons · Physics 2019-09-04 Oliver Hart , Garry Goldstein , Claudio Chamon , Claudio Castelnovo

Optically induced ultrafast electronic excitations with sufficiently long lifetimes may cause strong effects on phase transitions like structural and nonmetal to metal ones. Examples are transitions diamond to graphite, graphite to…

Materials Science · Physics 2010-09-21 K. H. Bennemann

X-ray diffraction experiments under pressure in a diamond anvil cell have been performed to gauge any response of the crystalline lattice of URu2Si2 to the "hidden order" or antiferromagnetic transitions, the latter of which is accessible…

Strongly Correlated Electrons · Physics 2010-09-29 J. R. Jeffries , N. P. Butch , J. J. Hamlin , S. V. Sinogeikin , W. J. Evans , M. B. Maple

In-situ diffuse neutron scattering experiments revealed that when electric current is passed through single crystals of rutile TiO2 under conditions conducive to flash sintering, it induces the formation of parallel planes of oxygen…

Materials Science · Physics 2024-10-22 Tyler C. Sterling , Feng Ye , Seohyeon Jo , Anish Parulekar , Yu Zhang , Gang Cao , Rishi Raj , Dmitry Reznik

Approaching energy coupling in laser-irradiated metals, we point out the role of electron-electron collision as an efficient control factor for ultrafast optical absorption. The high degree of laser-induced electron-ion nonequilibrium…

Recently, direct bandgap double perovskites are becoming more popular among photovoltaic research community owing to their potential to address issues of lead (Pb) toxicity and structural instability inherent in lead halide (simple)…

Materials Science · Physics 2021-01-13 I. B. Ogunniranye , T. Atsue , O. E. Oyewande

Charge-transfer excitations are of paramount importance for understanding the electronic structure of copper-oxide based high-temperature superconductors. In this study, we investigate the response of a Bi$_2$Sr$_2$CaCu$_2$O$_{\mathrm{8}+…

The optical properties of a large, detwinned single crystal of BaFe$_2$As$_2$ have been examined over a wide frequency range above and below the structural and magnetic transition at $T_{\rm N}\simeq 138$ K. Above $T_{\rm N}$ the real part…

Strongly Correlated Electrons · Physics 2020-11-12 Christopher C. Homes , Thomas Wolf , Christoph Meingast

The in-plane infrared and visible (3 meV-3 eV) reflectivity of Bi2Sr2CaCu2O8+d (Bi-2212) thin films is measured between 300 K and 10 K for different doping levels with unprecedented accuracy. The optical conductivity is derived through an…

Utrafast control of material physical properties represents a rapid developing field in condensed matter physics. Yet, accessing to the long-lived photoinduced electronic states is still in its early stage, especially with respect to an…

Strongly Correlated Electrons · Physics 2021-04-20 Q. M. Liu , D. Wu , Z. A. Li , L. Y. Shi , Z. X. Wang , S. J. Zhang , T. Lin , T. C. Hu , H. F. Tian , J. Q. Li , T. Dong , N. L. Wang

Motivated by recent pump-probe experiments indicating enhanced coherent $c$-axis transport in underdoped YBCO, we study Josephson junctions periodically driven by optical pulses. We propose a mechanism for this observation by demonstrating…

Superconductivity · Physics 2017-05-11 Jun-ichi Okamoto , Andrea Cavalleri , Ludwig Mathey

Manipulating spin in antiferromagnetic (AFM) materials has great potential in AFM opto-spintronics. Laser pulses can induce a transient ferromagnetic (FM) state in AFM metallic systems, but have never been proven in two-dimensional (2D) AFM…

Materials Science · Physics 2022-03-11 Shuo Li , Junjie He , Thomas Frauenheim

The existence of large nonlinear optical coefficients is one of the preconditions for using nonlinear optical materials in nonlinear optical devices. For a crystal, such large coefficients can be achieved by matching photon energies with…

Materials Science · Physics 2018-12-27 J. L. Cheng , J. E. Sipe , S. W. Wu , Chunlei Guo

Correlation in temperature behavior of the optical, neutron, and muon experimental data is established for YBa2Cu3O6+x in both the pseudogap state at Tc<T<T* and the superconducting state at T<Tc. We have showed that our absorption spectra…

Superconductivity · Physics 2009-11-10 Vladimir N. Samovarov , Volodymyr L. Vakula

Observed optical reflectivity in the infrared spectral region is compared with theoretical predictions in a strongly coupled electron-phonon system. Starting from a Froehlich Hamiltonian, the spectral functions and their temperature…

Superconductivity · Physics 2007-05-23 H. J. Kaufmann , E. G. Maksimov , E. K. H. Salje

X-ray absorption spectroscopy (XAS) and high resolution X-ray diffraction are combined to study the interplay between electronic and lattice structures in controlling the superconductivity in cuprates with a model charge-compensated…

Superconductivity · Physics 2009-08-18 S. Sanna , S. Agrestini , K. Zheng , R. De Renzi , N. L. Saini

We report a detailed Raman scattering study of the lattice dynamics in detwinned single crystals of the underdoped high temperature superconductor YBa2Cu3O6+x (x=0.75, 0.6, 0.55 and 0.45). Whereas at room temperature the phonon spectra of…

We show that disruption of charge-density-wave (stripe) order by charge transfer excitation, enhances the superconducting phase rigidity in La_{1.885}Ba_{0.115}CuO_4 (LBCO). Time-Resolved Resonant Soft X-Ray Diffraction demonstrates that…

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