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THz-frequency optical pulses can resonantly drive selected vibrational modes in solids and deform their crystal structure. In complex oxides, this method has been used to melt electronic orders, drive insulator to metal transitions or…

We report on a photo-induced transient state of YBa2Cu2O6+x in which transport perpendicular to the Cu-O planes becomes highly coherent. This effect is achieved by excitation with mid-infrared optical pulses, tuned to the resonant frequency…

Superconductivity · Physics 2014-06-04 S. Kaiser , C. R. Hunt , D. Nicoletti , W. Hu , I. Gierz , H. Y. Liu , M. Le Tacon , T. Loew , D. Haug , B. Keimer , A. Cavalleri

We use femtosecond resonant soft x-ray diffraction to measure the optically stimulated ultrafast changes of charge density wave correlations in underdoped YBa2Cu3O6.6. We find that when coherent interlayer transport is enhanced by optical…

Nonlinear optical excitation of infrared active lattice vibrations has been shown to melt magnetic or orbital orders and to transform insulators into metals. In cuprates, this technique has been used to remove charge stripes and promote…

Superconductivity · Physics 2014-09-03 W. Hu , S. Kaiser , D. Nicoletti , C. R. Hunt , I. Gierz , M. C. Hoffmann , M. Le Tacon , T. Loew , B. Keimer , A. Cavalleri

Optical excitation of large-amplitude apical oxygen phonon oscillations has been shown to renormalize the electronic properties of YBa$_2$Cu$_3$O$_{6+x}$, inducing a superconducting-like optical response above equilibrium $T_C$. All of the…

Superconductivity · Physics 2026-01-05 M. Rosenberg , D. Nicoletti , M. Buzzi , A. Iudica , C. Putzke , Y. Liu , B. Keimer , A. Cavalleri

Optical excitation of apical oxygen vibrations in YBa$_{2}$Cu$_{3}$O$_{6+\delta}$ has been shown to enhance its c-axis superconducting-phase rigidity, as evidenced by a transient blue shift of the equilibrium inter-bilayer Josephson plasma…

Superconductivity · Physics 2016-12-21 C. R. Hunt , D. Nicoletti , S. Kaiser , D. Pröpper , T. Loew , J. Porras , B. Keimer , A. Cavalleri

Intense laser pulses have recently emerged as a tool to tune between different orders in complex quantum materials. Among different light-induced phenomena, transient superconductivity far above the equilibrium transition temperature in…

Superconductivity · Physics 2020-03-11 S. J. Zhang , Z. X. Wang , H. Xiang , X. Yao , Q. M. Liu , L. Y. Shi , T. Lin , T. Dong , D. Wu , N. L. Wang

Optical excitation in the cuprates has been shown to induce transient superconducting correlations above the thermodynamic transition temperature, $T_C$, as evidenced by the terahertz frequency optical properties in the non-equilibrium…

Superconductivity · Physics 2020-03-25 B. Liu , M. Först , M. Fechner , D. Nicoletti , J. Porras , T. Loew , B. Keimer , A. Cavalleri

We investigated transient optical responses in an optimally-doped high-Tc superconductor La2-xSrxCuO4 (x=0.15) by using 800-nm optical pump and terahertz probe spectroscopy. With increasing the photoexcitation intensities, the Josephson…

Superconductivity · Physics 2018-03-15 Kaito Tomari , Ryusuke Matsunaga , Hiroaki Niwa , Dongjoon Song , Hiroshi Eisaki , Ryo Shimano

We report measurements of the photoinduced change in reflectivity of an untwinned single crystal of YBa2Cu3O6.5 in the ortho II structure. The decay rate of the transient change in reflectivity is found to decrease rapidly with decreasing…

Superconductivity · Physics 2009-11-07 G. P. Segre , N. Gedik , J. Orenstein , D. A. Bonn , Ruixing Liang , W. N. Hardy

The possibility of enhancing desirable functional properties of complex materials by optical driving is motivating a series of studies of their nonlinear terahertz response. In high-Tc cuprates, large amplitude excitation of certain…

Superconductivity · Physics 2024-07-12 A. von Hoegen , M. Fechner , M. Först , N. Taherian , E. Rowe , A. Ribak , J. Porras , B. Keimer , M. Michael , E. Demler , A. Cavalleri

The Ortho-II phase of YBa$_2$Cu$_3$O$_6.5$ is characterized by a periodic alternation of empty Cu and filled Cu-O b-axis doubling the unit cell in the a direction. The extra oxygen in the full chains gives rise to an attractive potential…

Superconductivity · Physics 2009-11-10 E. Bascones , T. M. Rice , A. O. Shorikov , V. I. Anisimov

Low energy electronic structure of optimally doped YBa2Cu3O7-d is investigated using laser-excited angle-resolved photoemission spectroscopy. The surface state and the CuO chain band that usually overlap the CuO2 plane derived bands are not…

Ultrafast light pulses can modify the electronic properties of quantum materials by perturbing the underlying, intertwined degrees of freedom. In particular, iron-based superconductors exhibit a strong coupling among electronic nematic…

We recently demonstrated that the superconductor-to-insulator transition induced by ionic liquid gating of the high temperature superconductor YBa2Cu3O7 (YBCO) is accompanied by a deoxygenation of the sample [Perez-Munoz et al., PNAS 114,…

Materials Science · Physics 2019-01-30 Roberta Poloni , Lorenzo A. Mariano , David Prendergast , Javier Garcia-Barriocanal

Recent pump-probe experiments reported an enhancement of superconducting transport along the $c$-axis of underdoped YBa$_2$Cu$_3$O$_{6+\delta}$ (YBCO), induced by a mid-infrared optical pump pulse tuned to a specific lattice vibration. To…

Superconductivity · Physics 2017-10-17 Jun-ichi Okamoto , Wanzheng Hu , Andrea Cavalleri , Ludwig Mathey

We have measured the extended x-ray absorption-fine-structure (EXAFS) at the Y-K edge of YBa_2Cu_3O_x for x=6.801, 6.947, 6.968, 6.984 at T=20-300 K. Across the underdoped-overdoped transition the Y-Cu2 pairs exhibit harmonic vibrations…

Superconductivity · Physics 2008-02-03 J. Röhler , P. W. Loeffen , S. Müllender , K. Conder , E. Kaldis

We use time- and angle-resolved photoemission to measure quasiparticle relaxation dynamics across a laser-induced superconducting phase transition in Bi2Sr2CaCu2O8+delta. Whereas low-fluence measurements reveal picosecond dynamics, sharp…

Far and mid infrared optical pulses have been shown to induce non-equilibrium unconventional orders in complex materials, including photo-induced ferroelectricity in quantum paraelectrics, magnetic polarization in antiferromagnets and…

Here we report extensive ultrafast time-resolved reflectivity experiments on overdoped Bi$_{2}$Sr$_{2}$Ca$_{1-x}$Y$_x$Cu$_{2}$O$_{8+\delta}$ single crystals (T$_C$=78 K) aimed to clarify the nature of the superconducting-to-normal-state…

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