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Using magnetic neutron scattering we characterize an unusual low temperature phase in orthorhombic SrCuO2. The material contains zigzag spin ladders formed by pairs of S=1/2 chains (J=180 meV) coupled through a weak frustrated interaction…

Materials Science · Physics 2009-10-31 I. A. Zaliznyak , C. Broholm , M. Kibune , M. Nohara , H. Takagi

We have performed inelastic neutron scattering on a single crystal sample of Sr14Cu24O41 to study the spin dynamics of the Cu2O3 spin ladder layers, and CuO2 chains. Data collected with incident energies of 50 meV, 200 meV, 350 meV and 500…

Frustration in quantum spin systems promote a variety of novel quantum phases. An important example is the frustrated spin-$1$ model on the square lattice with the nearest-neighbor bilinear ($J_1$) and biquadratic ($K_1$) interactions. We…

Strongly Correlated Electrons · Physics 2019-11-06 Wen-Jun Hu , Shou-Shu Gong , Hsin-Hua Lai , Haoyu Hu , Qimiao Si , Andriy H. Nevidomskyy

Detailed neutron scattering measurements on the bond frustrated magnet ZnCr2S4 reveal a rich H-T phase diagram. The field dependence of the two subsequent antiferromagnetic transitions follows closely that of recently reported structural…

Strongly Correlated Electrons · Physics 2014-06-03 D. Hsieh , Y. W. Li , S. Watauchi , Chang Liu , Q. Huang , R. J. Cava , J. W. Lynn , M. Z. Hasan

We explore the Mott transition in orthorhombic diamond lattices relevant to (ET)Ag$_4$(CN)$_5$ molecular compounds. The non-interacting phases include nodal line, Dirac and/or Weyl semimetals depending on the strength of spin-orbit coupling…

Strongly Correlated Electrons · Physics 2025-04-25 Javier Castro Luaces , Manuel Fernández López , Jorge Bravo-Abad , Jaime Merino

We report a quasi-one-dimensional S = 1 spin chain compound BaNiTe2O7. This magnetic system has been investigated by magnetic susceptibility, specific heat, and neutron powder diffraction. These results indicate that BaNiTe2O7 develops a…

The neutral charge state plays an important role in quantum information and sensing applications based on nitrogen-vacancy centers. However, the orbital and spin dynamics remain unexplored. Here, we use resonant excitation of single centers…

Quantum Physics · Physics 2020-11-11 S. Baier , C. E. Bradley , T. Middelburg , V. V. Dobrovitski , T. H. Taminiau , R. Hanson

We analyzed the magnetic susceptibilities of several Cr spinels using two recent models for the geometrically frustrated pyrochlore lattice, the Quantum Tetrahedral Mean Field model and a Generalized Constant Coupling model. Both models can…

Strongly Correlated Electrons · Physics 2010-03-01 Ch. Kant , J. Deisenhofer , V. Tsurkan , A. Loidl

We report high-resolution single-crystal inelastic neutron scattering measurements on the spin-1/2 antiferromagnet Ba(TiO)Cu$_4$(PO$_4$)$_4$. This material is formed from layers of four-site \cupola" structures, oriented alternately upwards…

We present a theory of spin and orbital physics in the A-site spinel compound FeSc2S4, which experimentally exhibits a broad "spin-orbital liquid" regime. A spin-orbital Hamiltonian is derived from a combination of microscopic consideration…

Strongly Correlated Electrons · Physics 2009-05-17 Gang Chen , Leon Balents , Andreas P. Schnyder

Small single crystals of Rb$_3$Ni$_2$(NO$_3$)$_7$ were obtained by crystallization from anhydrous nitric acid solution of rubidium nitrate and nickel nitrate hexahydrate. The basic elements of the crystal structure of this new compound are…

A spinel related oxide, Na4Ir3O8, was found to have a three dimensional network of corner shared Ir4+ (t2g^5) triangles. This gives rise to an antiferromagnetically coupled S = 1/2 spin system formed on a geometrically frustrated…

Strongly Correlated Electrons · Physics 2009-11-13 Yoshihiko Okamoto , Minoru Nohara , Hiroko Aruga-Katori , Hidenori Takagi

We present measurements of spin relaxation times (T_1, T_1,rho, T_2) on very shallow (<5 nm) nitrogen-vacancy (NV) centers in high-purity diamond single crystals. We find a reduction of spin relaxation times up to 30x compared to bulk…

Mesoscale and Nanoscale Physics · Physics 2014-05-15 T. Rosskopf , A. Dussaux , K. Ohashi , M. Loretz , R. Schirhagl , H. Watanabe , S. Shikata , K. M. Itoh , C. L. Degen

We report on 7Li NMR studies of a spin S = 3/2 triangular lattice antiferromagnet LiCrO2 (Neel temperature TN = 62 K) in the paramagnetic state by using the free-induction decay of 7Li nuclear magnetization. We observed critical divergence…

Strongly Correlated Electrons · Physics 2014-08-01 Y. Itoh

We present the results of neutron diffraction studies on polycrystals of a metallic kagome lattice, Tb3Ru4Al12, reported recently to undergo reentrant magnetism, with the onset of long range antiferromagnetic order below (TN=) 22 K and…

Strongly Correlated Electrons · Physics 2019-02-20 Sudhindra Rayaprol , Andreas Hoser , Kartik K Iyer , Sanjay K Upadhyay , E. V. Sampathkumaran

Correlated materials with competing spin-orbit and crystal-field interactions can host composite spin-orbital magnons that are highly susceptible to structural and electronic perturbations, enabling the control of magnetic dynamics beyond…

We report neutron scattering measurements of the spinel oxide LiGaCr$_{4}$O$_{8}$, in which magnetic ions Cr$^{3+}$ form a breathing pyrochlore lattice. Our experiments reveal the coexistence of a nearly dispersionless resonance mode and…

Strongly Correlated Electrons · Physics 2021-12-23 Zheng He , Yiqing Gu , Hongliang Wo , Yu Feng , Die Hu , Yiqing Hao , Yimeng Gu , Helen C. Walker , Devashibhai T. Adroja , Jun Zhao

Inelastic neutron scattering has been used to measure the low-energy spin excitations in the ordered charge-stripe phase of La(2)NiO(4+d) with d=0.133. Spin-wave-like excitations disperse away from the incommensurate magnetic superlattice…

Superconductivity · Physics 2009-10-28 J. M. Tranquada , P. Wochner , D. J. Buttrey

Geometric frustration inhibits magnetic systems from ordering, opening a window to unconventional phases of matter. The paradigmatic frustrated lattice in three dimensions to host a spin liquid is the pyrochlore, although there remain few…

Recent inelastic neutron scattering studies by Pan et al., Nature Communications 8, 123 (2017), find evidence for spin excitations at energies above the quasi-particle gap in an iron-selenide high-Tc superconductor. The momenta of the spin…

Superconductivity · Physics 2020-08-03 J. P. Rodriguez