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We performed nuclear magnetic resonance (NMR) and muon spin relaxation ({\mu}SR) experiments to identify the magnetic ground state of the frustrated quantum A-site spinel, CuAl2O4. Our results verify that the ground state does not exhibit a…

Dynamical magnetic correlations in the geometrically frustrated Nd$\_3$Ga$\_5$SiO$\_{14}$ compound were probed by inelastic neutron scattering on a single crystal. A scattering signal with a ring shape distribution in reciprocal space and…

Strongly Correlated Electrons · Physics 2007-05-23 Julien Robert , Virginie Simonet , Benjamin Canals , Rafik Ballou , Pierre Bordet , Pascal Lejay , Anne Stunault

In antiferromagnets, the interplay of spin frustration and spin-lattice coupling has been extensively studied as the source of complex spin patterns and exotic magnetism. Here, we demonstrate that, although neglected in the past, the…

A unique type of frustrated lattice is found in two A-site ordered spinel oxides, LiGaCr4O8 and LiInCr4O8. Because of the large size mismatch between Li+ and Ga3+/In3+ ions at the A site, the pyrochlore lattice, made up of Cr3+ ions…

Materials Science · Physics 2015-06-12 Yoshihiko Okamoto , Gøran J. Nilsen , J. Paul Attfield , Zenji Hiroi

Inelastic neutron scattering studies in single crystals of TbInO3 and TbIn0.95Mn0.05O3 with nearly-triangular antiferromagnetic lattice are reported. At low energies, a broad and apparently gapless continuum of magnetic excitations, located…

Strongly Correlated Electrons · Physics 2019-07-10 M. G. Kim , B. Winn , S. Chi , A. T. Savici , J. A. Rodriguez-Rivera , W. C. Chen , X. Xu , Y. Li , J. W. Kim , S. -W. Cheong , V. Kiryukhin

The mixed spinel, MgFe2O4 has been synthesized by ball-milling assisted sintering method. X-ray diffraction study confirms formation of cubic MgFe2O4 and the lattice parameter values calculated are a = b = c = 8.369(3) {\AA}. Vibrating…

Materials Science · Physics 2018-10-01 B. Santhosh Kumar , N. Praveen Shankar , N. Aparna devi , C. Venkateswaran

Frustration refers to competition between different interactions that cannot be simultaneously satisfied, a familiar feature in many magnetic solids. Strong frustration results in highly degenerate ground states, and a large suppression of…

Strongly Correlated Electrons · Physics 2007-07-03 Doron Bergman , Jason Alicea , Emanuel Gull , Simon Trebst , Leon Balents

The A-site ordered chromate spinels LiGa1-xInxCr4O8 host a network of size-alternating spin-3/2 Cr3+ tetrahedra known as a 'breathing' pyrochlore lattice. For the x=0.05 composition, the complex magneto-structural ordering observed in the…

Strong spin-lattice coupling and prominent frustration effects observed in the 50$\%$ Fe-doped frustrated hexagonal ($h$)LuMnO$_3$ are reported. A N\'{e}el transition at $T_{\mathrm N} \approx$ 112~K and a possible spin re-orientation…

Strongly Correlated Electrons · Physics 2015-12-24 Harikrishnan S. Nair , Zhendong Fu , C. M. N. Kumar , V. Y. Pomjakushin , Yinguo Xiao , Tapan Chatterji , André M. Strydom

We discuss the ground state of a pyrochlore lattice of threefold-orbitally-degenerate $S=1/2$ magnetic ions. We derive an effective spin-orbital Hamiltonian and show that the orbital degrees of freedom can modulate the spin exchange,…

Strongly Correlated Electrons · Physics 2007-05-23 S. Di Matteo , G. Jackeli , C. Lacroix , N. B. Perkins

A new type of magnetically frustrated lattice is found in the layered fluoride NaBa2Mn3F11. A kagome-type array of regular triangles composed of Mn2+ ions (spin 5/2) deforms so as to generate the next-nearest-neighbor interaction J2 between…

Materials Science · Physics 2014-03-11 Hajime Ishikawa , Tsuyoshi Okubo , Yoshihiko Okamoto , Zenji Hiroi

We present our theoretical and numerical results on thermodynamic properties and the microscopic mechanism of two successive transitions in vanadium spinel oxides $A$V$_2$O$_4$ ($A$=Zn, Mg, or Cd) obtained by Monte Carlo calculations of an…

Strongly Correlated Electrons · Physics 2007-05-23 Yukitoshi Motome , Hirokazu Tsunetsugu

We report muon spin relaxation ($\mu$SR) and magnetic susceptibility measurements on Cu(Cl,Br)La(Nb,Ta)$_{2}$O$_{7}$, which demonstrate: (a) the absence of static magnetism in (CuCl)LaNb$_{2}$O$_{7}$ down to 15 mK confirming a spin-gapped…

Tb2Ti2O7 is a pyrochlore antiferromagnet that has dynamical spins and only short-range correlations even at 50 mK; the lowest temperature explored so far, which is much smaller than the scale set by the Curie-Weiss temperature T_{CW}~14 K.…

Statistical Mechanics · Physics 2009-12-16 Hamid R. Molavian , Paul A. McClarty , Michel J. P. Gingras

Correlation functions (CFs) of the classical Heisenberg antiferromagnet on the pyrochlore lattice are studied by solving exactly the infinite-component spin-vector model. % As in many Fully Frustrated Lattices, the constraint due to the…

Strongly Correlated Electrons · Physics 2009-11-07 Benjamin Canals , Dmitry Garanin

The spin wave excitations of the ideal S=5/2 Kagome lattice antiferromagnet KFe3(OH)6(SO4)2 have been measured using high-resolution inelastic neutron scattering. We directly observe a flat mode which corresponds to a lifted "zero energy…

Strongly Correlated Electrons · Physics 2008-10-31 K. Matan , D. Grohol , D. G. Nocera , T. Yildirim , A. B. Harris , S. H. Lee , S. E. Nagler , Y. S. Lee

The Faraday rotation technique is used to map out the finite-temperature phase diagram of the prototypical frustrated magnet ZnCr2O4, in magnetic fields of up to 190 T generated by the single-turn coil method. We find evidence for a number…

Strongly Correlated Electrons · Physics 2015-03-19 Atsuhiko Miyata , Hiroaki Ueda , Yutaka Ueda , Yukitoshi Motome , Nic Shannon , Karlo Penc , Shojiro Takeyama

Lattice and magnetic dynamics of NiWO$_4$ single crystals were studied with the use of polarized Raman spectroscopy in a wide temperature range of 10-300 K including the antiferromagnetic ordering temperature $T_N$=62 K. Static magnetic…

Materials Science · Physics 2017-07-26 M. A. Prosnikov , V. Yu. Davydov , A. N. Smirnov , M. P. Volkov , R. V. Pisarev , P. Becker , L. Bohatý

The chromium spinels MgCr2O4 and ZnCr2O4 are prime examples of the highly frustrated pyrochlore lattice antiferromagnet. Experiment has carefully established that both materials, upon cooling, distort to lower symmetry and order…

Strongly Correlated Electrons · Physics 2025-02-28 Ludovic D. C. Jaubert , Yasir Iqbal , Harald O. Jeschke

We report on the quasi-two-dimensional magnetism of the natural mineral diaboleite Pb2Cu(OH)4Cl2 with a tetragonal crystal structure, which is closely related to that of the frustrated spin-1/2 magnet PbVO3. Magnetic susceptibility of…

Materials Science · Physics 2013-02-15 Alexander A. Tsirlin , Oleg Janson , Stefan Lebernegg , Helge Rosner