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A rare combination of strong spin-orbit coupling and electron-electron correlations makes the iridate Mott insulator Sr$_2$IrO$_4$ a promising host for novel electronic phases of matter. The resemblance of its crystallographic, magnetic and…

Strongly Correlated Electrons · Physics 2016-01-11 L. Zhao , D. H. Torchinsky , H. Chu , V. Ivanov , R. Lifshitz , R. Flint , T. Qi , G. Cao , D. Hsieh

An anapole state that breaks inversion and time reversal symmetries with preserving translation symmetry of underlying lattice has aroused great interest as a new quantum state, but only a few candidate materials have been reported.…

Strongly Correlated Electrons · Physics 2021-02-10 H. Murayama , K. Ishida , R. Kurihara , T. Ono , Y. Sato , Y. Kasahara , H. Watanabe , Y. Yanase , G. Cao , Y. Mizukami , T. Shibauchi , Y. Matsuda , S. Kasahara

Sr2IrO4 is one of the prime candidates for realizing exotic quantum spin orders owing to the subtle combination of spin-orbit coupling and electron correlation. Sensitive local magnetization measurement can serve as a powerful tool to study…

Materials Science · Physics 2025-03-26 Hyeokjun Heo , Jeongha An , Junyoung Kwon , Kwangrae Kim , Youngoh Son , B. J. Kim , Joonho Jang

Protected by the interplay of on-site Coulomb interactions and spin-orbit coupling, Sr$_2$IrO$_4$ at high pressure is a rare example of a Mott insulator with a paramagnetic ground state. Here, using optical Raman scattering, we measure both…

Strongly Correlated Electrons · Physics 2021-11-29 Xiang Li , S. E. Cooper , A. Krishnadas , A. de la Torre , R. S. Perry , F. Baumberger , D. M. Silevitch , D. Hsieh , T. F. Rosenbaum , Yejun Feng

There is considerable evidence that the superconducting state of Sr$_2$RuO$_4$ breaks time reversal symmetry. In the experiments showing time reversal symmetry breaking its onset temperature, $T_\text{TRSB}$, is generally found to match the…

Sr$_{2}$IrO$_{4}$ with strong spin-orbit coupling (SOC) and Hubbard repulsion (U) hosts Mott insulating states. The similar crystal structure, magnetic and electronic properties, particularly the $d$-wave gap observed in Sr$_{2}$IrO$_{4}$…

Strongly Correlated Electrons · Physics 2023-12-04 Haozhe Wang , Madalynn Marshall , Zhen Wang , Kemp W. Plumb , Martha Greenblatt , Yimei Zhu , David Walker , Weiwei Xie

We discuss the notions of spin-orbital polarization and ordering in paramagnetic materials, and address their consequences in transition metal oxides. Extending the combined density functional and dynamical mean field theory scheme to the…

Strongly Correlated Electrons · Physics 2014-12-16 Cyril Martins , Markus Aichhorn , Loig Vaugier , Silke Biermann

We formulate and study an effective Hamiltonian for low-energy Kramers doublets of $d^1$-ions on a square lattice. We find that the system exhibits a magnetically hidden order in which the expectation values of the local spin and orbital…

Strongly Correlated Electrons · Physics 2009-08-09 George Jackeli , Giniyat Khaliullin

Recent optical second-harmonic generation experiments observed unexpected broken spatial symmetries in the undoped spin-orbit Mott insulator Sr$_2$IrO$_4$, leading to intensive debates on the nature of its ground state. We propose that it…

Strongly Correlated Electrons · Physics 2021-11-05 Yun-Peng Huang , Jin-Wei Dong , Ziqiang Wang , Sen Zhou

We report muon spin relaxation measurements on the superconductor Sr2RuO4 that reveal the spontaneous appearance of an internal magnetic field below the transition temperature: the appearance of such a field indicates that the…

We report a La2CuO4-like interlayer antiferromagnetic order in Sr2IrO4 films with large orthorhombic distortion (> 1.5%). The biaxial lattice strain in epitaxial heterostructures of Sr2IrO4/Ca3Ru2O7 lowers the crystal symmetry of Sr2IrO4…

Strongly Correlated Electrons · Physics 2022-03-23 S. Shrestha , M. Krautloher , M. Zhu , J. Kim , J. Hwang , J. Kim , J. -W. Kim , B. Keimer , A. Seo

In electronic solids with strong spin-orbit interactions (SOIs), the spin and orbital degrees of freedom of an electron are quantum mechanically entangled, which may result in an exotic multipolar order instead of a conventional dipolar…

Strongly Correlated Electrons · Physics 2020-07-01 Daigorou Hirai , Hajime Sagayama , Shang Gao , Hiroyuki Ohsumi , Gang Chen , Taka-hisa Arima , Zenji Hiroi

Numerous experiments have reported discrete symmetry breaking in the high temperature pseudogap phase of the hole-doped cuprates, including breaking of one or more of lattice rotation, inversion, or time-reversal symmetries. In the absence…

Strongly Correlated Electrons · Physics 2017-05-31 Shubhayu Chatterjee , Subir Sachdev

We used femtosecond optical spectroscopy to study ultrafast spin and orbital ordering dynamics in the antiferromagnetic Mott insulator $\alpha$-Sr$_2$CrO$_4$. This chromate system possesses multiple spin and orbital ordered phases, and…

Using resonant x-ray diffraction, we observe an easy c-axis collinear antiferromagnetic structure for the bilayer Sr$_3$Ir$_2$O$_7$, a significant contrast to the single layer Sr$_2$IrO$_4$ with in-plane canted moments. Based on a…

Strongly Correlated Electrons · Physics 2012-12-11 J. W. Kim , Y. Choi , Jungho Kim , J. F. Mitchell , G. Jackeli , M. Daghofer , J. van den Brink , G. Khaliullin , B. J. Kim

We propose a candidate for the hidden order in URu2Si2: a rank-5 E type spin density wave between Uranium 5f crystal field doublets breaking time reversal and lattice tetragonal symmetry in a manner consistent with recent torque…

Strongly Correlated Electrons · Physics 2012-07-09 Jeffrey G. Rau , Hae-Young Kee

Sr2IrO4 exhibits a novel insulating state assisted by spin-orbit interactions. A series of polycrystalline samples of Sr2-xIrO4 have been synthesized. It is found that deep Sr-vacancies of Sr2-xIrO4 greatly reduce the rotation of IrO6…

Strongly Correlated Electrons · Physics 2016-11-01 Xuanyong Sun , S. L. Liu , Haiyun Wang , Bin Li , Jie Cheng , Z. H. Wang

Materials with strongly correlated electrons exhibit physical properties that are often difficult to predict as they result from the interactions of large numbers of electrons combined with several quantum degrees of freedom. The layered…

Sr2IrO4 is a magnetic insulator driven by spin-orbit interaction (SOI) whereas the isoelectronic and isostructural Sr2RhO4 is a paramagnetic metal. The contrasting ground states have been shown to result from the critical role of the strong…

Strongly Correlated Electrons · Physics 2012-09-07 T. F. Qi , O. B. Korneta , L. Li , K. Butrouna , V. S. Cao , Xiangang Wan , P. Schlottmann , R. K. Kaul , G. Cao

At room temperature, the normal oxide spinels NiCr_2O_4 and CuCr_2O_4 are tetragonally distorted and crystallize in the I4_1/amd space group due to cooperative Jahn-Teller ordering driven by the orbital degeneracy of tetrahedral Ni$^{2+}$…

Materials Science · Physics 2012-09-11 Matthew R. Suchomel , Daniel P. Shoemaker , Lynn Ribaud , Moureen C. Kemei , Ram Seshadri
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