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Photocatalytic water splitting represents a pivotal pathway for converting solar energy into chemical energy, with the core challenge lying in the design and optimization of photocatalysts [1] . TiO2, as a quintessential photocatalytic…

Materials Science · Physics 2025-02-20 Zhihao Shen

In this work an overall electronic structure including the position and formation energies of various intrinsic defects are computed for anatase using Density Functional Theory aided by Hubbard correction (DFT+U). The intrinsic point…

Insulator-to-metal (MI) phase transition in vanadium dioxide (VO2) thin films with controlled lattice distortion was investigated by thermopower measurements. VO2 epitaxial films with different crystallographic orientations, grown on (0001)…

Strongly Correlated Electrons · Physics 2015-07-15 Takayoshi Katase , Kenji Endo , Hiromichi Ohta

Highly ordered TiO2 nanotube arrays (TNAs) codoped with V and N were synthesized by electrochemical anodization in association with hydrothermal treatment. The samples were characterized by field emission scanning electron microscopy, X-ray…

Materials Science · Physics 2014-05-28 Min Zhang , Dandan Lu , Zhihua Zhang , Jianjun Yang

The ternary nitride CaZn2N2, composed only of earth-abundant elements, is a novel semiconductor with a band gap of 1.8 eV. First-principles calculations predict that continuous Mg substitution at the Zn site will change the optical band gap…

Materials Science · Physics 2019-09-17 Masatake Tsuji , Hidenori Hiramatsu , Hideo Hosono

Motivated by our previous work on bulk NbOX2 , where we have reported its high 1dielectric polarisation and finite piezoelectric response, this work extends to its 2D homo bilayer system to explore its potential for photocatalytic water…

An extensive theoretical study is performed for wide bandgap crystalline oxides and nitrides, namely, SiO_{2}, GeO_{2}, Al_{2}O_{3}, Si_{3}N_{4}, and Ge_{3}N_{4}. Their important polymorphs are considered which are for SiO_{2}:…

Materials Science · Physics 2009-11-11 C. Sevik , C. Bulutay

Here, we propose titanium nitride (TiN) as an alternative plasmonic material for an on-chip silicon plasmonic Schottky photodetector that is based on an internal photoemission process and operating at telecom wavelengths. The examined…

Applied Physics · Physics 2020-02-12 Jacek Gosciniak , Fatih B. Atar , Brian Corbett , Mahmoud Rasras

In this work, we report on the electrochemical behavior of nitrided spaced TiO$_2$ nanotubes conformally coated with a nanocrystalline Nb$_2$O$_5$ layer and find for these hierarchical structures an excellent supercapacitor performance.…

Applied Physics · Physics 2020-05-05 Selda Ozkan , Nhat Truong Nguyen , Imgon Hwang , Anca Mazare , Patrik Schmuki

We have determined the electronic and atomic structure of N doped TiO2 using a combination of hard x-ray photoelectron spectroscopy (HAXPES) and first- principles density functional theory calculations. Our results reveal that N doping of…

Materials Science · Physics 2015-05-14 Abdul K. Rumaiz , J. C. Woicik , E. Cockayne , H. Y. Lin , G. Hassnain Jaffari , S. Ismat Shah

Using a density-functional theory plus dynamical mean-field theory methodology, we compute the many-body electronic structure and optical conductivity of NdNiO$_{2}$ under the influence of large scattering rates on the Nd($5d$) bands and…

Strongly Correlated Electrons · Physics 2023-06-14 Harrison LaBollita , Alexander Hampel , Jonathan Karp , Antia S. Botana , Andrew J. Millis

Anatase TiO$_2$ is among the most studied materials for light-energy conversion applications, but the nature of its fundamental charge excitations is still unknown. Yet it is crucial to establish whether light absorption creates…

Photo-rechargeable (solar) battery can be considered as an energy harvesting cum storage system, where it can charge the conventional metal-ion battery using light instead of electricity, without having other parasitic reactions. Here we…

We use density functional theory (DFT) calculations to investigate structural models consisting of anatase TiO2(101) slabs covered by reduced overlayers formed by (101) crystallographic shear planes (CSPs). Ab initio thermodynamics supports…

Materials Science · Physics 2018-01-17 Xunhua Zhao , Sencer Selcuk , Annabella Selloni

Ti2O3 exhibits a unique metal-insulator transition (MIT) at approximately 450 K over a wide temperature range of ~ 150 K. This broad MIT accompanied by lattice deformation differs from the sharp MITs observed in most other transition-metal…

Dye Sensitized Solar Cells (DSSCs) have recently regained attention for indoor light harvesting and powering wireless devices. Advantages such as cost-effectiveness, flexibility, wide angular response, and lightweight design have driven the…

Two dimensional (2D) semiconducting light absorbers, have recently considered as promising components to improve the efficiency in the photocatalytic hydrogen production via water splitting. In this work, by employing density functional…

Materials Science · Physics 2021-09-07 Fazel Shojaei , Bohayra Mortazavi , Xiaoying Zhuang , Maryam Azizi

It has been recently revealed that strontium titanate (SrTiO$_3$) displays persistent photoconductivity with unique characteristics: it occurs at room temperature and lasts over a very long period of time. Illumination of SrTiO$_3$ crystals…

Materials Science · Physics 2020-09-23 Zhiqiang Zhang , Anderson Janotti

Low resistivity (~3-24 mOhm.cm) with tunable n- and p-type phase pure Cu2O thin films have been grown by pulsed laser deposition at 25-200 0C by varying the background oxygen partial pressure (O2pp). Capacitance data obtained by…

Materials Science · Physics 2020-06-01 Syed Farid Uddin Farhad , David Cherns , James Smith , Neil Fox , David Fermín

We perform first-principles calculations to investigate the band structure, density of states, optical absorption, and the imaginary part of dielectric function of Cu, Ag, and Au-doped anatase TiO2 in 72 atoms systems. The electronic…

Materials Science · Physics 2015-08-10 Meili Guo , Jiulin Du