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High-quality microresonators can greatly enhance light-matter interactions and are excellent platforms for studying nonlinear optics. Wavelength conversion through nonlinear processes is the key to many applications of integrated optics.…
We present a multimodal non-linear optical (NLO) laser-scanning microscope, based on a compact fiber-format excitation laser and integrating coherent anti-Stokes Raman scattering (CARS), stimulated Raman scattering (SRS) and…
We present an experimental set-up developed to perform optical spectroscopy experiments (Raman scattering and photoluminescence measurements) with a micrometer spatial resolution, in an extreme environment of low temperature, high magnetic…
Due to its particular geometry, stimulated Raman side-scattering (SRSS) drives scattered light emission at non-conventional directions, leading to scarce and complex experimental observations. Direct-irradiation campaigns at the SG-II UP…
A novel method for single-step, lithography-free, and large-scale laser writing of nanoparticle-based plasmonic structures has been developed. Changing energy of femtosecond laser pulses and thickness of irradiated gold film it is possible…
Optical spectroscopy and imaging of microscopic samples have opened up a wide range of applications throughout the physical, chemical, and biological sciences. High chemical specificity may be achieved by directly interrogating the…
The requirement of high space-time resolution and brightness is a great challenge for imaging atomic motion and making molecular movies. Important breakthroughs in ultrabright tabletop laser, x-ray and electron sources have enabled the…
Optical fields polarized along three dimensions are frequent in optical microscopy and nanophotonics, and yet retrieving their polarization distribution is challenging. We present the experimental implementation of three-dimensional (3D)…
Spectroscopic stimulated Raman scattering (SRS) imaging has become a useful tool finding a broad range of applications. Yet, wider adoption is hindered by the bulky and environmentally-sensitive solid-state optical parametric oscillator…
Coherent Raman scattering provides highly sensitive vibrational analysis through nonlinear light-matter interactions. However, its application to metal interfaces has remained challenging because the intrinsically large non-resonant…
Short-wavelength free-electron lasers with their ultrashort pulses at high intensities have originated new approaches for tracking molecular dynamics from the vista of specific sites. X-ray pump X-ray probe schemes even allow to address…
Collective coherent scattering of laser light by an ensemble of polarizable point particles creates long range interactions, whose properties can be tailored by choice of injected laser powers, frequencies and polarizations. We use a…
Three-dimensional phase contrast imaging of multiply-scattering samples in X-ray and electron microscopy is extremely challenging, due to small numerical apertures, the unavailability of wavefront shaping optics, and the highly nonlinear…
We use vortex photon fields with orbital and spin angular momentum to probe chiral fluctuations within liquid crystals. In the regime of iridescence with a well-defined pitch length of chirality, we find low energy Raman scattering that can…
Low-temperature electronic properties of rare-earth intermetallics are substantially influenced by the symmetry and magnitude of the crystal electric field. The direct spectroscopic analysis of crystal field splitting can be challenging,…
Dark-field X-ray microscopy (DFXM) is a nondestructive full-field imaging technique providing three dimensional mapping of microstructure and local strain fields in deeply embedded crystalline elements. This is achieved by placing an…
Interaction of a high intensity short laser pulse with near-critical plasmas allows to achieve extremely high coupling efficiency and transfer laser energy to energetic ions. One dimensional Particle-In-Cell (PIC) simulations are considered…
Stimulated low-frequency Raman scattering can give essential information about the elastic properties of different nanoparticles systems, in particular, biological nanostructures. In the present study, low-frequency vibrational modes in…
Raman scattering is a chemically selective probing mechanism with diverse applications in industry and clinical settings. Yet, most samples are optically opaque limiting the applicability of Raman probing at depth. Here, we demonstrate…
The lattice dynamics of preferentially aligned nanocrystals formed upon drying of aqueous Ba(NO$_3$)$_2$ solutions in a mesoporous silica glass traversed by tubular pores of approximately 12 nm are explored by Raman scattering. To interpret…