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Atom scattering is becoming recognized as a sensitive probe of the electron-phonon interaction parameter $\lambda$ at metal and metal-overlayer surfaces. Here, the theory is developed linking $\lambda$ to the thermal attenuation of atom…

Superconductivity · Physics 2020-05-20 G. Benedek , J. R. Manson , S. Miret-Artés

CrSBr, a van der Waals material, stands out as an air-stable magnetic semiconductor with appealing intrinsic properties such as crystalline anisotropy, quasi-1D electronic characteristics, layer-dependent antiferromagnetism, and non-linear…

We present polarization resolved Raman scattering study of surface vibration modes in the topological insulator Bi$_2$Se$_3$ single crystal and thick films. Besides the four Raman active bulk phonons, we observed four additional modes with…

Layered van der Waals (vdW) materials have emerged as a promising platform for nanophotonics due to large refractive indexes and giant optical anisotropy. Unlike conventional dielectrics and semiconductors, the absence of covalent bonds…

Van der Waals materials and their heterostructures offer a versatile platform for studying a variety of quantum transport phenomena due to their unique crystalline properties and the exceptional ability in tuning their electronic spectrum.…

Mesoscale and Nanoscale Physics · Physics 2019-08-05 P. Kumaravadivel , M. T. Greenaway , D. Perello , A. Berdyugin , J. Birkbeck , J. Wengraf , S. Liu , J. H. Edgar , A. K. Geim , L. Eaves , R. Krishna Kumar

We have found that the polarization dependence of Raman scattering in organic crystals at finite temperatures can only be described by a fourth-rank formalism. This generalization of the second-rank Raman tensor $\mathcal{R}$ stems from the…

Combining atomically-thin van der Waals materials into heterostructures provides a powerful path towards the creation of designer electronic devices. The interaction strength between neighboring layers, most easily controlled through their…

Mesoscale and Nanoscale Physics · Physics 2017-01-27 Matthew Yankowitz , K. Watanabe , T. Taniguchi , Pablo San-Jose , Brian J. LeRoy

Fe3GeTe2 has emerged as one of the most fascinating van der Waals crystals due to its two-dimensional (2D) itinerant ferromagnetism, topological nodal lines and Kondo lattice behavior. However, lattice dynamics, chirality of phonons and…

Heterogeneous integration strategies are increasingly being employed to achieve more compact and capable electronics systems for multiple applications including space, electric vehicles, and wearable and medical devices. To enable new…

Raman scattering in the spin-crossover system [Fe(pmd)(H2O){Au(CN)2}2]*H2O reveals a complex three-phase spin-state transition in contrast to earlier observations in magnetization measurements. We observe different spin state phases as…

Strongly Correlated Electrons · Physics 2010-03-09 V. Gnezdilov , P. Lemmens , P. Scheib , M. Ghosh , Yu. G. Pashkevich , H. Paulsen , V. Schuenemann , J. A. Wolny , G. Agusti , J. A. Real

Photonics has been revolutionized by breakthroughs in optical metasurfaces and layered two-dimensional materials. Yet, integrating these two fields in a singular system has remained challenging. Here, we introduce the concept of van der…

A completely quantum description of Raman process is used to investigate the nonclassical properties of the modes in the stimulated, spontaneous and partially spontaneous Raman process. Both coherent scattering (where all the initial modes…

Quantum Physics · Physics 2022-06-10 Anirban Pathak , Jaromir Krepelka , Jan Perina

We have performed polarized Raman scattering measurements on the newly discovered superconductor Ba$_{2}$Ti$_{2}$Fe$_{2}$As$_{4}$O$_{2}$ ($T_c = 21$ K). We observe seven out of eight Raman active modes, with frequencies in good accordance…

Superconductivity · Physics 2014-05-07 S. -F. Wu , P. Richard , W. -L. Zhang , C. -S. Lian , Y. -L. Sun , G. -H. Cao , J. -T. Wang , H. Ding

The plasmon and phonon polaritons of two-dimensional (2d) and van-der-Waals materials have recently gained substantial interest. Unfortunately, they are notoriously hard to observe in linear response because of their strong confinement, low…

Mesoscale and Nanoscale Physics · Physics 2020-08-13 Christian Wolff , N. Asger Mortensen

We present a detailed temperature dependent Raman light scattering study of optical phonons in Ba{1-x}K{x}Fe{2}As{2} (x ~ 0.28, superconducting Tc ~ 29 K), Sr{1-x}K{x}Fe{2}As{2} (x ~ 0.15, Tc ~ 29 K) and non-superconducting BaFe{2}As{2}…

Superconductivity · Physics 2009-08-18 M. Rahlenbeck , G. L. Sun , D. L. Sun , C. T. Lin , B. Keimer , C. Ulrich

Superconductivity evolves as functions of pressure or doping from charge-ordered phases in a variety of strongly correlated systems, suggesting that there may be universal characteristics associated with the competition between…

Strongly Correlated Electrons · Physics 2016-03-03 S. L. Gleason , Y. Gim , T. Byrum , A. Kogar , P. Abbamonte , E. Fradkin , G. J. MacDougall , D. J. Van Harlingen , Xiangde Zhu , C. Petrovic , S. L. Cooper

We theoretically investigate multiphonons resonance Raman scattering between the Landau levels in graphene on the polar substrate using the Huang-Rhys's model. We not only present the single and multiple surface optical (SO) phonons…

Mesoscale and Nanoscale Physics · Physics 2017-12-01 Zi-Wu Wang , Zhi-Qing Li

We investigated emission and propagation of polaritons in a two dimensional van der Waals material hexagonal boron nitride (hBN). Our specific emphasis in this work is on hyperbolic phonon polariton emission that we investigated by means of…

We consider a model of Raman scattering for a two--dimensional $S=1/2$ Heisenberg Anti-Ferromagnet which includes a {\it dynamical} spin--phonon interaction. We observe a broadening of the line shape due to increased coupling with excited…

Condensed Matter · Physics 2009-10-28 Matthew J. Reilly , A. G. Rojo

We show that electronic Raman scattering affords a window into the essential properties of the pairing potential $V_{\mathbf{k},\mathbf{k^{\prime}}}$ of iron-based superconductors. In Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ we observe band…