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Ammonia inversion lines are often used as probes of the physical conditions in the dense ISM. The excitation temperature between the first two para metastable (rotational) levels is an excellent probe of the gas kinetic temperature.…

Astrophysics of Galaxies · Physics 2015-05-13 Sebastien Maret , Alexandre Faure , Emanuele Scifoni , Laurent Wiesenfeld

A scarcity of known chemical kinetic parameters leads to the use of many reaction rate estimates, which are not always sufficiently accurate, in the construction of detailed kinetic models. To reduce the reliance on these estimates and…

Intermolecular hydrogen transfer free radical reactions are common in the combustion process and in a number of organic chemistry reactions. Therefore, evaluating the pressure and temperature-dependent rate constants of them is of great…

Chemical Physics · Physics 2024-04-01 Yi Sun

Machine learning techniques have been quite popular recently in the high-energy physics community and have led to numerous developments in this field. In heavy-ion collisions, one of the crucial observables, the impact parameter, plays an…

High Energy Physics - Phenomenology · Physics 2021-10-11 Aditya Nath Mishra , Neelkamal Mallick , Sushanta Tripathy , Suman Deb , Raghunath Sahoo

Jet event rates in deep inelastic ep scattering at HERA are investigated applying the modified JADE jet algorithm. The analysis uses data taken with the H1 detector in 1994 and 1995. The data are corrected for detector and hadronization…

High Energy Physics - Experiment · Physics 2008-11-26 C. Adloff

We propose an efficient method to compute reaction rate constants of thermally activated processes occurring in many-body systems at finite temperature. The method consists in two steps: first, paths are sampled using a transition path…

Statistical Mechanics · Physics 2011-12-22 Massimiliano Picciani

Dependence of transition frequencies on the fine structure constant $\alpha=e^2/\hbar c$ is calculated for several many-electron systems which are used or planned to be used in the laboratory search for the time variation of the fine…

Atomic Physics · Physics 2009-11-13 V. A. Dzuba , V. V. Flambaum

Reaction rates of chemical reactions under nonequilibrium conditions can be determined through the construction of the normally hyperbolic invariant manifold (NHIM) [and moving dividing surface (DS)] associated with the transition state…

We present theoretical thermally-averaged rate constants for vibrational and rotational (de-)excitation of the H3+ ion by electron impact. The constants are calculated using the multi-channel quantum-defect approach. The calculation…

Atomic Physics · Physics 2015-05-18 Viatcheslav Kokoouline , Alexandre Faure , Jonathan Tennyson , Chris H. Greene

The title reaction is studied using a quasi-classical trajectory method for collision energies between 0.1 meV and 10 eV, considering the vibrational excitation of H$_2^+$ reactant. A new potential energy surface is developed based on a…

Chemical Physics · Physics 2023-03-06 P. del Mazo-Sevillano , D. Félix-González , A. Aguado , C. Sanz-Sanz , D. -H. Kwon , O. Roncero

Fe II emission lines are observed from nearly all classes of astronomical objects over a wide spectral range from the infrared to the ultraviolet. To meaningfully interpret these lines, reliable atomic data are necessary. In work presented…

Atomic Physics · Physics 2019-03-12 Yier Wan , C. Favreau , S. D. Loch , B. M. McLaughlin , Yueying Qi , P. C. Stancil

Linear mixed models with large imbalanced crossed random effects structures pose severe computational problems for maximum likelihood estimation and for Bayesian analysis. The costs can grow as fast as $N^{3/2}$ when there are N…

Methodology · Statistics 2017-05-30 K. Gao , A. B. Owen

We present a theory and accompanying importance sampling method for computing rate constants in spatially inhomogenious systems. Using the relationship between rate constants and path space partition functions, we illustrate that the…

Statistical Mechanics · Physics 2019-06-05 Addison J. Schile , David T. Limmer

A new database of collisional rate coefficients for transitions between the rotational states of H$_2$O collided with H$_2$ background gas is developed. The goal is to expand over the other existing databases in terms of the rotational…

Quantum Physics · Physics 2024-12-18 Carolin Joy , Dulat Bostan , Bikramaditya Mandal , Dmitri Babikov

Rate coefficients for collisional processes such as rotational and vibrational excitation are essential inputs in many astrophysical models. When rate coefficients are unknown, they are often estimated using known values from other systems.…

Astrophysics of Galaxies · Physics 2015-06-22 Kyle M. Walker , B. H. Yang , P. C. Stancil , N. Balakrishnan , R. C. Forrey

To understand the recently observed mysterious non-adiabatic energy transfer for hyperthermal H atom scattering from a semiconductor surface, Ge(111)c(2*8), we present a mixed quantum-classical non-adiabatic molecular dynamics model based…

Complex transition density can be constructed by a nuclear structure model with a complex basis and/or complex coefficient. In general, the complex transition density is converted to the real one with phase factor. In this study, we apply…

Nuclear Theory · Physics 2022-05-26 T. Furumoto

We identify two metastable excited states in Sm$ ^{10+} $ highly charged ion as candidates for high accuracy optical clocks. Several atomic properties relevant to optical clock development are calculated using relativistic many-body…

High Energy Physics - Phenomenology · Physics 2024-09-04 Saleh O. Allehabi , V. A. Dzuba , V. V. Flambaum

Canonical instanton theory is known to overestimate the rate constant close to a system-dependent crossover temperature and is inapplicable above that temperature. We compare the accuracy of the reaction rate constants calculated using…

Chemical Physics · Physics 2020-09-15 Sean McConnell , Johannes Kästner

Recently, machine learning (ML) techniques have led to a range of numerous developments in the field of nuclear and high-energy physics. In heavy-ion collisions, the impact parameter of a collision is one of the crucial observables which…

High Energy Physics - Phenomenology · Physics 2021-06-02 Neelkamal Mallick , Sushanta Tripathy , Aditya Nath Mishra , Suman Deb , Raghunath Sahoo