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Spatial interaction effects between charge carriers in ionic systems play a sizable role beyond a classical Maxwellian description. We develop a nonlocal, two-fluid, hydrodynamic theory of charges and study ionic plasmon effects, i. e.…

Optics · Physics 2020-06-30 Christin David

We report a theoretical study of ion size effect on various properties in a soft nanochannel with pH-dependent charge density. We develop a free energy based mean-field theory taking into account ion size as well as pH-dependence of charged…

Soft Condensed Matter · Physics 2022-02-11 Jun-Sik Sin , Un-Hyok Kim

High-index spherical nanoparticles with low material losses support sharp high-Q electric and magnetic resonances and exhibit a number of interesting optical phenomena. Developments in fabrication techniques have enabled the further study…

Optics · Physics 2020-12-30 D. A. Pidgayko , Z. F. Sadrieva , K. S. Ladutenko , A. A. Bogdanov

Understanding the electrical double layer (EDL), i.e, the distribution of electrolyte at an electrified interface, in concentrated electrolytes is important for various technologies, such as supercapacitors, batteries and electrocatalysis.…

Soft Condensed Matter · Physics 2026-05-01 Zachary A. H. Goodwin

We theoretically investigate electrostatic properties between two charged surfaces with a grafted polyelectrolyte layer in an aqueous electrolyte solution by using the Poisson-Boltzmann approach accounting for ion partitioning. In order to…

Soft Condensed Matter · Physics 2022-02-07 Jun-Sik Sin

Ionic liquids offer unique bulk and interfacial characteristics as battery electrolytes. Our continuum approach naturally describes the electrolyte on a macroscale. An integral formulation for the molecular repulsion,which can be…

Chemical Physics · Physics 2022-11-30 Max Schammer , Arnulf Latz , Birger Horstmann

Classical theory of the electric double layer is based on the fundamental assumption of a dilute solution of point ions. There are a number of situations such as high applied voltages, high concentration of electrolytes, systems with…

Fluid Dynamics · Physics 2015-06-11 Brian D. Storey , Martin Z. Bazant

We utilize the self-consistent field theory to explore the mechanical and electrical properties of charged surfaces immersed in polyelectrolyte solutions that could be potentially useful for electrochemical applications. Our research…

Soft Condensed Matter · Physics 2023-08-25 Yu. A. Budkov , N. N. Kalikin

With nanoelectronics reaching the limit of atom-sized devices, it has become critical to examine how irregularities in the local environment can affect device functionality. Here, we characterize the influence of charged atomic species on…

We study the deformations of pH-responsive spherical microcapsules -- micrometer-scale liquid drops surrounded by thin, solid shells -- under the influence of electrostatic forces. When exposed to a large concentration of NaOH, the…

Soft Condensed Matter · Physics 2014-02-03 Sujit S. Datta , Alireza Abbaspourrad , David A. Weitz

The optical properties of rod-like two-layer nanoparticles are studied using the notions of equivalent prolate spheroid. The calculations are presented for frequency dependencies for polarizability and the absorption and scattering…

Optics · Physics 2024-07-02 Ya. V. Karandas

Nanoparticles (NPs) make for intriguing heterogeneous catalysts due to their large active surface area and excellent and often size-dependent catalytic properties that emerge from a multitude of chemically different surface reaction sites.…

The interfacial nature of the electric double layer (EDL) assumes that electrode surface morphology significantly impacts the EDL properties. Since molecular-scale roughness modifies the structure of EDL, it is expected to disturb the…

Chemical Physics · Physics 2024-02-09 Irina Nesterova , Aleksey Khlyupin , Nikolay Evstigneev , Oleg Ryabkov , Kirill M. Gerke

The ordering of a multilayer consisting of DSPC bilayers on a silica sol substrate is studied within the model-independent approach to the reconstruction of profiles of the electron density from X-ray reflectometry data. It is found that…

Within the Poisson-Boltzmann (PB) approach electrolytes in contact with planar, spherical, and cylindrical electrodes are analyzed systematically. The dependences of their capacitance $C$ on the surface charge density $\sigma$ and the ionic…

Soft Condensed Matter · Physics 2017-04-24 Andreas Reindl , Markus Bier , S. Dietrich

Simulations for the density and potential profiles of the ions in the planar electrical double layer of a model electrolyte or an ionic liquid are reported. The ions of a real electrolyte or an ionic liquid are usually not spheres; in ionic…

Soft Condensed Matter · Physics 2016-03-08 W. Silvestre-Alcantara , L. B. Bhuiyan , S. Lamperski , M. Kaja , D. Henderson

Here, we correlate the nanoscale morphology and chemical composition of solid electrolyte interphases (SEI) with the electrochemical property of graphite-based composite electrodes. Using electrochemical strain microscopy (ESM) and X-ray…

This study utilizes molecular dynamics simulations to scrutinize the influence of type and volume fraction of nanoparticle on the density of nanofluids, i.e. silver (as a hydrophilic case) and titanium dioxide (as a hydrophobic case)…

Applied Physics · Physics 2021-05-20 M. M. Heyhat , M. Abbasi , A. Rajabpour

The electrostatic potential profile of a spherical soft particle is derived by solving the Poisson-Boltzmann equations on a spherical system both numerically and analytically. The soft particle is assumed to consist of an ion-permeable…

Soft Condensed Matter · Physics 2015-06-18 Anh D. Phan , Dustin A. Tracy , T. L. Hoai Nguyen , N. A. Viet , The-Long Phan , Thanh H. Nguyen

We consider the correlation functions in a gas of electrons moving within a thin layer on the surface of nanosize sphere. A closed form of expressions for the RKKY indirect exchange, superconducting Cooper loop and `density-density'…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 D. N. Aristov