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We extensively study the phase diagram of a diblock copolymer melt confined in a cylindrical nanopore using real-space self-consistent mean-field theory. We discover a rich variety of new two-dimensional equilibrium structures that have no…

Soft Condensed Matter · Physics 2009-11-11 Weihua Li , Robert A. Wickham

The formation of (bio)molecular condensates via liquid-liquid phase separation in cells has received increasing attention, as these coacervates play important functional and regulatory roles within biological systems. However, the majority…

Soft Condensed Matter · Physics 2022-11-24 Arash Nikoubashman , Miho Yanagisawa

A mean field rate theory description of the homo- and co-polymerization of $f$-functional molecules is developed, which contains the formation of short cyclic structures inside the network. The predictions of this model are compared with…

Soft Condensed Matter · Physics 2021-03-31 Michael Lang , Konrad Schwenke , Jens-Uwe Sommer

In this paper we consider a two-dimensional model of a copolymer consisting of a random concatenation of hydrophilic and hydrophobic monomers, immersed in a micro-emulsion of random droplets of oil and water. The copolymer interacts with…

Probability · Mathematics 2012-04-06 Frank den Hollander , Nicolas Pétrélis

One dimensional non-equilibrium systems with short-range interaction can undergo phase transitions from homogeneous states to phase separated states as interaction ($\epsilon$) among particles is increased. One of the model systems where…

Statistical Mechanics · Physics 2011-05-31 Anasuya Kundu , P. K. Mohanty

Colloidal droplets are used in a variety of practical applications. Some of these applications require particles of different sizes. These include medical diagnostic methods, the creation of photonic crystals, the formation of…

Soft Condensed Matter · Physics 2024-04-04 P. A. Zolotarev , K. S. Kolegov

Cell dynamics simulation is used to investigate the phase behavior of block copolymer/homopolymer mixture subjected to a steady shear flow. Phase transitions occur from transverse to parallel and then to perpendicular lamellar structure…

Soft Condensed Matter · Physics 2015-06-29 Y. Guo , J. Zhang , B. Wang , H. Wu , M. Sun , J. Pan

Colloidal suspensions with free polymer coils which are larger than the colloidal particles are considered. The polymer-colloid interaction is modeled by an extension of the Asakura-Oosawa model. Phase separation occurs into dilute and…

Soft Condensed Matter · Physics 2009-10-31 Richard P. Sear

A coarse-graining strategy for dilute and semi-dilute solutions of interacting polymers, and of colloid polymer mixtures is briefly described. Monomer degrees of freedom are traced out to derive an effective, state dependent pair potential…

Soft Condensed Matter · Physics 2009-11-11 J. -P. Hansen , C. I. Addison , A. A. Louis

We study a blend of two kinds of homopolymers with tendency for segragation. Cross-links between the chains of different kinds do not allow macrophase separation. Instead microphase structure appears. Starting from a microscopic model we…

Condensed Matter · Physics 2007-05-23 C. D. Sfatos , A. M. Gutin , E. I. Shakhnovich

A soft particle model for diblock (AB) copolymer melts is proposed. Each molecule is mapped onto two soft spheres built by Gaussian A- and B-monomer distributions. An approximate analytical expression for the joint distribution function for…

Materials Science · Physics 2009-11-13 F. Eurich , A. Karatchentsev , J. Baschnagel , W. Dieterich , P. Maass

In recent experiments, small, thick-walled vesicles with a narrow size distribution were formed from copolymers where the degree of polymerisation of the hydrophobic block, N_B, was significantly greater than that of the hydrophilic block,…

Soft Condensed Matter · Physics 2017-09-12 M. J. Greenall

We perform a thermodynamic analysis of the polymerization-induced phase separation in nanoparticle-monomer-polymer blends using a simple model recently proposed by V. V. Ginzburg (Macromolecules 2005, 38, 2362.). The model was adapted for…

Materials Science · Physics 2013-11-22 Ezequiel R. Soule , Julio Borrajo , Roberto J. J. Williams

We investigate the mechanism of chain exchange in diblock copolymer micelles using two distinct yet complementary simulation techniques. First, enhanced sampling method is combined with coarse-grained molecular dynamics to compute a…

Soft Condensed Matter · Physics 2025-09-09 Samuel Varner , Marcus Müller , Alejandro Gallegos , Timothy P. Lodge , Kevin D. Dorfman , Zhen-Gang Wang

The phase behaviour of binary blends composed of A$_1$B$_1$ and A$_2$B$_2$ diblock copolymers is systematically studied using the polymeric self-consistent field theory, focusing on the formation and relative stability of various spherical…

Soft Condensed Matter · Physics 2021-09-01 Jiayu Xie , Yu Li , An-Chang Shi

We analyze diffusion of small particles in a solid polymeric medium taking into account a short range particle-polymer interaction. The system is modeled by a particle diffusion on a ternary lattice where the sites occupied by polymer…

Statistical Mechanics · Physics 2015-06-11 Federico Camboni , Andreas Koher , Igor M. Sokolov

Based on a microscopic model, we study the interplay between superconductivity and antiferromagnetism in a multi-layered system, where two superconductors are separated by an antiferromagnetic region. Within a self-consistent mean-field…

Superconductivity · Physics 2015-05-19 H. T. Quan , Jian-Xin Zhu

Phase separation, crucial for spatially segregating biomolecules in cells, is well-understood in the simple case of a few components with pairwise interactions. Yet, biological cells challenge the simple picture in at least two ways: First,…

Soft Condensed Matter · Physics 2024-03-12 Chengjie Luo , Yicheng Qiang , David Zwicker

The phase structure of a homopolymer chain is investigated in terms of a universal theoretical model, designed to describe the infrared limit of slow spatial variations. The effects of chirality are studied and compared with the influence…

Soft Condensed Matter · Physics 2015-12-25 A. Sinelnikova , A. J. Niemi , M. Ulybyshev

We investigate spreading of phase separated copolymer films, where domain walls and thickness steps influence polymer flow. We show that at early stages of spreading its rate is determined by slow activated flow at terrace steps (i.e.…

Soft Condensed Matter · Physics 2009-11-10 Vladimir A. Belyi , Thomas A. Witten
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