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This study theoretically investigates the angular distribution of core-level photoemission time delay within a molecular frame. This phenomenon can be measured with the advancement of attosecond pulsed lasers and metrology. Our focus is on…

Chemical Physics · Physics 2025-02-19 Yoshiaki Tamura , Kaoru Yamazaki , Kiyoshi Ueda , Keisuke Hatada

The narrowing of electron and ion wave packets in the process of photoionization is investigated, with the electron-ion recoil fully taken into account. Packet localization of this type is directly related to entanglement in the joint…

Quantum Physics · Physics 2009-11-10 M. V. Fedorov , M. A. Efremov , A. E. Kazakov , K. W. Chan , C. K. Law , J. H. Eberly

We consider time delay and symmetrised time delay (defined in terms of sojourn times) for quantum scattering pairs $\{H_0=h(P),H\}$, where $h(P)$ a dispersive operator of hypoelliptic-type. For instance $h(P)$ can be one of the usual…

Mathematical Physics · Physics 2015-05-13 Rafael Tiedra de Aldecoa

After photon absorption, electrons from a dispersive band of a solid require a finite time in the photoemission process before being photoemitted as free particles, in line with recent attosecondresolved photoemission experiments. According…

Mesoscale and Nanoscale Physics · Physics 2017-02-15 Mauro Fanciulli , Henrieta Volfová , Stefan Muff , Jürgen Braun , Hubert Ebert , Jan Minár , Ulrich Heinzmann , J. Hugo Dil

We analyze two-center interference effects in the yields of ionization of a dissociating hydrogen molecular ion by an ultrashort VUV laser pulse. To this end, we performed numerical simulations of the time-dependent Schr\"odinger equation…

Quantum Physics · Physics 2015-05-27 A. Picón , A. Bahabad , H. C. Kapteyn , M. M. Murnane , A. Becker

A compact analysis of development and prospects in the study of the tunnelling evolution is given. A new systematization of various approaches to defining tunnelling times in the light of time as a quantum mechanical observable is proposed.…

General Physics · Physics 2008-02-03 V. S. Olkhovsky , A. Agresti

We discuss the relationship between modern time-dependent density functional theory and earlier time-periodic versions, and why the criticisms in a recent paper (Chem. Phys. Lett. {\bf 433} (2006) 204) of our earlier analysis (Chem. Phys.…

Materials Science · Physics 2007-05-23 Neepa T. Maitra , Kieron Burke

We introduce a time-dependent R-matrix theory generalised to describe double ionization processes. The method is used to investigate two-photon double ionization of He by intense XUV laser radiation. We combine a detailed B-spline-based…

Atomic Physics · Physics 2014-05-14 H. W. van der Hart

The behavior of a single molecule driven simultaneously by a laser and by an electric radio frequency field is investigated using a non-Hermitian Hamiltonian approach. Employing the renormalization group method for differential equations we…

Quantum Physics · Physics 2013-05-29 Igor Rozhkov , E. Barkai

In this short review paper, we discuss the concept of time delay for an abstract quantum scattering system. Its definition in terms of sojourn times is explained as well as its identity with the so-called Eisenbud-Wigner time delay.…

Mathematical Physics · Physics 2011-03-22 S. Richard

Photoionization and its inverse, electron-ion recombination, are key processes that influence many astrophysical plasmas (and gasses), and the diagnostics that we use to analyse the plasmas. In this review we provide a brief overview of the…

Solar and Stellar Astrophysics · Physics 2023-03-21 D. John Hillier

The measured distribution of the single-channel delay time of localized microwave radiation and its correlation with intensity differ sharply from the behavior of diffusive waves. The delay time is found to increase with intensity, while…

Disordered Systems and Neural Networks · Physics 2009-11-07 A. A. Chabanov , A. Z. Genack

Crank-Nicolson (C-N) Method combined with $ B $-spline basis set can be used in both time-dependent and time-independent calculations of the photoionization cross sections of atoms and molecules. For time-independent systems, it is found…

Atomic Physics · Physics 2014-09-15 Xue-Bin Bian

We evaluate the joint distributions of electron waiting times in coherent conductors described by scattering theory. Successive electron waiting times in a single-channel conductor are found to be correlated due to the fermionic statistics…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 David Dasenbrook , Patrick P. Hofer , Christian Flindt

Time lags are ubiquitous in biophysiological processes and more generally in real-world complex networks. It has been recently proposed to use information-theoretic tools such as transfer entropy to detect and estimate a possible delay in…

Statistical Mechanics · Physics 2018-10-03 M. L. Rosinberg , G. Tarjus , T. Munakata

Signatures of the Coulomb corrections in the photoelectron momentum distribution during laser-induced ionization of atoms or ions in tunneling and multiphoton regimes are investigated analytically in the case of an one-dimensional problem.…

Measuring the time it takes to remove an electron from an atom or molecule during photoionization using newly developed attosecond spectroscopies has been a focus of many recent experiments. However, the outcome of such measurement depends…

Atomic Physics · Physics 2017-03-08 Lisa Torlina , Olga Smirnova

We investigate the limitations arising from atomic collisions on the storage and delay times of probe pulses in EIT experiments. We find that the atomic collisions can be described by an effective decay rate that limits storage and delay…

Quantum Physics · Physics 2009-11-07 D. C. Roberts , T. Gasenzer , K. Burnett

A theoretical comparison of the electronic excitation and ionisation behaviour of molecular hydrogen oriented either parallel or perpendicular to a linear polarised laser pulse is performed. The investigation is based on a non-perturbative…

Quantum Physics · Physics 2009-11-13 Yulian V. Vanne , Alejandro Saenz

Temporal and angular correlations in atom-mediated photon-photon scattering are measured. Good agreement is found with the theory presented in Part~I.

Optics · Physics 2007-05-23 M. W. Mitchell , Cindy I. Hancox , R. Y. Chiao