Related papers: Comment on "Time delays in molecular photoionizati…
We have studied the angular time delay in slow-electron elastic scattering by spherical targets as well as the average time delay of electrons in this process. It is demonstrated how the angular time delay is connected to the…
For a molecule, the two-center interference and the molecular scattering phase of the electron are important for almost all the processes that may occur in a laser field. In this study, we investigate their effects in the transfer of linear…
We present a step by step introduction to the notion of time-delay in classical and quantum mechanics, with the aim of clarifying its foundation at a conceptual level. In doing so, we motivate the introduction of the concepts of "fuzzy" and…
We present a generalization of the pioneering results obtained for single K-shell photoionization of H-like ions by M. Stobbe [Ann. Phys. 7 (1930) 661] to the case of the helium isoelectronic sequence. The total cross section of the process…
Isotopic substitution in molecular systems can affect fundamental molecular properties including the energy position and spacing of electronic, vibrational and rotational levels, thus modifying the dynamics associated to their coherent…
Inconsistencies are pointed out in a recent proposal [L. Diosi, Phys. Rev. A 80, 064104 (2009); arXiv:0905.3908v1] for a quantum version of the classical linear Boltzmann equation.
Resonant two-photon ionization in a system consisting of two spatially well-separated atoms is studied. Due to two-center electron-electron correlations, the ionization may also proceed through photo-excitation of both atoms with subsequent…
We discuss the emergence of time dilation as a normal feature expected of any system where a central processor may have to wait one or more clock cycles before concluding a local calculation. We show how the process of causal implication in…
We apply Brunetti and Fredenhagen's [Phys. Rev. A 66 (2002) 044101] concept of the time of occurrence of an event in quantum mechanics to the example of scattering off a spherical potential. Thereby, we re-derive the expression of…
We determine and analyze the quantum phases and time delays in photoionization and photorecombination of valence 3p and 3s electrons of argon using the Kohn-Sham local density functional approach. The time-dependent local density…
The Mott corrections to the higher moments of the heavy ion energy-loss distribution are calculated in a wide range of relative particle velocity on the basis of the Mott exact cross section. It is shown that the relative Mott corrections…
We derive a Hamiltonian for the external and internal dynamics of an electromagnetically bound, charged two-particle system in external electromagnetic and gravitational fields, including leading-order relativistic corrections. We apply…
We predict a significant delay of two-electron photoemission from the helium atom after absorption of an attosecond XUV pulse. We establish this delay by solving the time dependent Schr\"odinger equation and by subsequent tracing the…
A fully relativistic calculation of the double photoionization of helium-like atoms is presented. The approach is based on the partial-wave representation of the Dirac continuum states and accounts for the retardation in the…
The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…
In the semiclassical picture of photoionization process in intense laser fields, the ionization rate solely depends on the amplitude of the electric field and the final photoelectron momentum corresponds to the instant of ionization of the…
We develop a novel technique for modeling of atomic and molecular ionization in superposition of XUV and IR fields with characteristics typical for attosecond streaking and RABBITT experiments. The method is based on solving the…
Although many physical arguments account for using a modified definition of time delay in multichannel-type scattering processes, one can hardly find rigorous results on that issue in the literature. We try to fill in this gap by showing,…
The decay of photoexcited quantum systems (examples are photodissociation of molecules and autoionization of atoms) can be viewed as a half-collision process (an incoming photon excites the system which subsequently decays by dissociation…
The Eisenbud-Wigner-Smith (EWS) time delay of photoemission depends on the phase term of the matrix element describing the transition. Because of an interference process between partial channels, the photoelectrons acquire a spin…