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We study laser-assisted photoionization by attosecond pulses using a time-independent formalism based on diagrammatic many-body perturbation theory. Our aim is to provide an ab inito route to the "delays" for this above-threshold ionization…

Atomic Physics · Physics 2015-06-12 J. M. Dahlström , T. Carette , E. Lindroth

Popp and Yan [F. A. Popp, Y. Yan, Phys. Lett. A 293 (2002) 93] proposed a model for delayed luminescence based on a single time-dependent coherent state. We show that the general solution of their model corresponds to a luminescence that is…

Quantitative Methods · Quantitative Biology 2011-06-22 Vahid Salari , Christian Brouder

Relative phases of atomic above-threshold ionization wavepackets have been investigated in a recent experiment [L. J. Zipp, A. Natan, and P. H. Bucksbaum, Optica \textbf{1}, 361-364 (2014)] exploiting interferences between different…

Atomic Physics · Physics 2021-11-10 S. D. López , S. Donsa , S. Nagele , D. G. Arbó , J. Burgdörfer

We present experimental data on the strong-field ionization of the argon dimer in a co-rotating two-color (CoRTC) laser field. We observe a sub-cycle interference pattern in the photoelectron momentum distribution and infer the Wigner time…

Time delays of electrons emitted from an isotropic initial state and leaving behind an isotropic ion are assumed to be angle-independent. Using an interferometric method involving XUV attosecond pulse trains and an IR probe field in…

Attosecond photoemission or photoionization delays are a unique probe of the structure and the electronic dynamics of matter. However, spectral congestion and spatial delocalization of valence electron wave functions set fundamental limits…

We consider a fully quantized model of spontaneous emission, scattering, and absorption, and study propagation of a single photon from an emitting atom to a detector atom both with and without an intervening scatterer. We find an exact…

Quantum Physics · Physics 2009-11-07 Thomas Purdy , Daniel R. Taylor , Martin Ligare

We present the first numerical simulation of the time delay in the photoionization of the simplest diatomic molecule H$_2^+$ as observed by attosecond streaking. We show that the strong variation of the Eisenbud-Wigner-Smith time delay as a…

The effects of confinement resonances on photoelectron group delay (Wigner time delay) following ionization of an atom encapsulated inside a C$_{60}$ cage have been studied theoretically using both relativistic and non-relativistic random…

Atomic Physics · Physics 2014-06-11 P. C. Deshmukh , A. Mandal , S. Saha , A. S. Kheifets , V. K. Dolmatov , S T Manson

We investigate attosecond time delays in the emission of photoelectrons using a hierarchy of models of the $CO_2$ molecule including the strong field approximation, Coulomb-scattering, short-range parts of the molecular potential, Hartree…

Atomic Physics · Physics 2021-03-30 Hakon Volkmann , Vinay P. Majety , Armin Scrinzi

We consider the general expressions for the time delay of photons of different energies in the framework of multi-dimensional cosmological models. In models with compactified extra-dimensions (Kaluza-Klein type models), the main source of…

Astrophysics · Physics 2009-11-10 T. Harko , K. S. Cheng

Attosecond ionization time-delays at photoelectron energies above typically 10 eV are usually interpreted using the so called asymptotic approximation as a sum of the atomic or molecular delays with a universal laser-induced contribution.…

We study ionization of aligned H$_2^+$ in strong elliptically-polarized laser fields numerically and analytically. The calculated offset angle in photoelectron momentum distribution is several degrees larger for the molecule than a model…

Atomic Physics · Physics 2023-01-03 J. Y. Che , Y. G. Peng , F. B. Zhang , X. J. Xie , G. G. Xin , Y. J. Chen

In a recent Letter [Phys. Rev. Lett. {\bf 100}, 120501 (2008)], Avron {\em et al.} discuss a time reordering scheme to achieve efficient "across-generation" of entangled photon pairs in a semiconductor quantum dot with a suppressed…

Mesoscale and Nanoscale Physics · Physics 2009-07-28 P. K. Pathak , S. Hughes

In a recent paper [Phys. Rev. Lett. 125, 043201 (2020)] (Ref.1) Liao et al. propose a theory of the interferometric photoemission delay based on the concepts of the photoelectron phase and photoelectron effective mass. The present comment…

Materials Science · Physics 2021-04-26 E. E. Krasovskii , R. O. Kuzian

We use the non-relativistic random phase approximation with exchange to perform calculations of valence shell photoionization of Ne, Ar, Kr and Xe from their respective thresholds to photon energy of 200 eV. The energy derivative of the…

Atomic Physics · Physics 2026-03-03 A. S. Kheifets

We study ionization of atoms in strong elliptically-polarized laser fields. We focus on the physical origin of the offset angle in the photoelectron momentum distribution and its possible relation to a specific time. By developing a model…

Atomic Physics · Physics 2022-12-12 Y. G. Peng , J. Y. Che , C. Chen , G. G. Xin , Y. J. Chen

Measured photoionization time delays may exhibit large variations as a function of the emission angles, even for spherically symmetric targets, as shown in recent RABBITT (reconstruction of attosecond beating by interference of two-photon…

Atomic Physics · Physics 2022-12-29 D. I. R. Boll , L. Martini , A. Palacios , O. A. Fojón

The mediated photon-photon interaction due to the resonant Kerr nonlinearity in an inhomogeneously broadened atomic vapor is considered. The time-scale for photon-photon scattering is computed and found to be determined by the inhomogeneous…

Optics · Physics 2009-11-06 M. W. Mitchell , R. Y. Chiao

Single and multi-photon ionization of aligned molecular ensembles is examined, with a particular focus on the link between the molecular axis distribution and observable in various angle-integrated and angle-resolved measurements. To…

Chemical Physics · Physics 2015-03-04 Paul Hockett