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Photoionisation is a process where absorption of one or several photons liberates an electron and creates a hole in a quantum system, such as an atom or a molecule. Is it faster to remove an electron using one or many photons, and how to…

Quantum Physics · Physics 2015-09-25 Jivesh Kaushal , Felipe Morales , Lisa Torlina , Misha Ivanov , Olga Smirnova

Focused laser fields with textured polarization on a sub-wavelength scale allow extracting information on electronic processes which are not directly accessible by homogeneous fields. Here, we consider photoionization in radially and…

Atomic Physics · Physics 2021-06-30 Jonas Wätzel , Jamal Berakdar

The photoelectric effect is not truly instantaneous, but exhibits attosecond delays that can reveal complex molecular dynamics. Sub-femtosecond duration light pulses provide the requisite tools to resolve the dynamics of photoionization.…

The possibilities of unlike particle correlations for a study of particle delays and spatial shifts in relativistic heavy ion collisions are demonstrated. This report represents the unpublished Ref. [4] in the paper by S. Voloshin et al.,…

Nuclear Theory · Physics 2007-05-23 R. Lednicky , S. Panitkin , N. Xu

We describe in detail how attosecond delays in laser-assisted photoionization can be computed using perturbation theory based on two-photon matrix elements. Special emphasis is laid on above-threshold ionization, where the electron…

Atomic Physics · Physics 2015-06-19 J. M. Dahlström , E. Lindroth

A technique for measuring photoionization time delays with attosecond precision is combined with calculations of photoionization matrix elements to demonstrate how multi-electron dynamics affect photoionization time delays in carbon…

Photoionization as a half-scattering process is not instantaneous. Usually, time delays in photoionization are of the order of few tens of attoseconds (1 as = 10$^{-18}$ s). While going from a single atom to a nano-object, one can expect…

We solve the time-dependent Schr\"odinger equation describing a water molecule driven by a superposition of the XUV and IR pulses typical for a RABBITT experiment. This solution is obtained by a combination of the time-dependent coordinate…

Atomic Physics · Physics 2018-01-17 Vladislav V. Serov , A. S. Kheifets

We apply a fundamental definition of time delay, as the difference between the time a particle spends within a finite region of a potential and the time a free particle spends in the same region, to determine results for photoionization of…

Atomic Physics · Physics 2015-06-12 Jing Su , Hongcheng Ni , Andreas Becker , Agnieszka Jaroń-Becker

We employ the recently developed multi-photon R-matrix method for molecular above-threshold photoionization to obtain second-order ionization amplitudes that govern the interference in RABITT experiments. This allows us to extract RABITT…

Atomic Physics · Physics 2022-05-03 Jakub Benda , Zdeněk Mašín , Jimena D. Gorfinkiel

Shape resonances in photoionization of atoms and molecules arise from a particular geometry of the ionic potential which traps the receding photoelectron in a quasi-bound state in a particular partial wave. This mechanism allows us to…

Atomic Physics · Physics 2026-03-03 Anatoli S. Kheifets , Stephen Catsamas

Theoretical arguments in favor of energy dependent photon time delays from a modification of special relativity (SR) have met with recent gamma ray observations that put severe constraints on the scale of such deviations. We review the case…

High Energy Physics - Theory · Physics 2018-01-19 J. M. Carmona , J. L. Cortes , J. J. Relancio

Ionizing radiation is known to delay the cell cycle progression. In particular after particle exposure significant delays have been observed and it has been shown that the extent of delay affects the expression of damage such as chromosome…

Cell Behavior · Quantitative Biology 2009-08-24 Anna Ochab-Marcinek , Ewa Gudowska-Nowak , Elena Nasonova , Sylvia Ritter

Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…

We study laser-assisted photodetachment time delays by attosecond pulse trains from the closed-shell negative ions F- and Cl-. We investigate the separability of the delay into two contributions: (i) the Wigner-like delay associated with…

Atomic Physics · Physics 2017-09-13 Eva Lindroth , Jan Marcus Dahlström

We theoretically study time-resolved photoemission in atoms as probed by attosecond streaking. We review recent advances in the study of the photoelectric effect in the time domain and show that the experimentally accessible time shifts can…

Atomic Physics · Physics 2015-03-06 Stefan Nagele , Renate Pazourek , Michael Wais , Georg Wachter , Joachim Burgdörfer

We revisit the time-resolved photoemission in neon atoms as probed by attosecond streaking. We calculate streaking time shifts for the emission of 2p and 2s electrons and compare the relative delay as measured in a recent experiment by…

This tutorial presents an introduction to the interaction of light and matter on the attosecond timescale. Our aim is to detail the theoretical description of ultra-short time-delays, and to relate these to the phase of extreme ultraviolet…

Atomic Physics · Physics 2012-07-20 J. M. Dahlström , A. L'Huillier , A. Maquet

In this paper we present a mathematical analysis of the photoelectric effect for one-electron atoms in the framework of non-relativistic QED. We treat photo-ionization as a scattering process where in the remote past an atom in its ground…

Mathematical Physics · Physics 2015-05-14 Marcel Griesemer , Heribert Zenk

The problem of time delay in tunneling ionization is revisited. The origin of time delay at the tunnel exit is analysed, underlining the two faces of the concept of the tunnelling time delay: the time delay around the tunnel exit and the…