Related papers: Broadband excitation by method of double sweep
The paper describes the design of band selective excitation and rotation pulses in high resolution NMR by method of double sweep. We first show the design of a pulse sequence that produces band selective excitation to the equator of Bloch…
The paper describes the design of broadband chirp excitation pulses in NMR. We first develop a three stage model for understanding chirp excitation in NMR. We then show how a chirp $\pi$ pulse can be used to refocus the phase of the chirp…
We have a new paradigm to design NMR pulses. Pulses, we call feedback pulses. We want broadband inversion and excitation. We have many offsets, start evolving them all starting from the north pole. Monitor them on the Bloch sphere, see…
Pulsed excitation of broad spectra requires very high field strengths if monochromatic pulses are used. If the corresponding high power is not available or not desirable, the pulses can be replaced by suitable low-power pulses that…
Dynamic nuclear polarization (DNP) is an NMR hyperpolarization technique that mediates polarization transfer from highly polarized unpaired electrons to NMR-active nuclei via microwave (mw) irradiation. The ability to generate arbitrarily…
We studied the underlying mechanism of broadband dispersive-wave emission within a resonance band of gas-filled anti-resonant hollow-core fiber. Both theoretical and experimental results unveiled that the high-order soliton, launched into…
Swept-frequency pulses have found applications in a wide range of areas including spectroscopic techniques where efficient control of spins is required. For many of these applications, a good understanding of the evolution of spin systems…
We show that the duration of broadband universal control pulses can be halved by choosing control targets with a quadratic function of phase dispersion. This class of control pulses perform a broadband universal rotation around an axis, in…
We describe a setup that is used for high-frequency electrical sample excitation in a cathode lens electron microscope with the sample stage at high voltage as used in many synchrotron light sources. Electrical signals are transmitted by…
This paper proposes a new method for joint design of radiofrequency (RF) and gradient waveforms in Magnetic Resonance Imaging (MRI), and applies it to the design of 3D spatially tailored saturation and inversion pulses. The joint design of…
We calculate the {\em exact} time-resolved ARPES spectrum of a two-band model semiconductor driven out of equilibrium by resonant and nonresonant laser pulses, highlighting the effects of phonon-induced decoherence and relaxation. {\em…
We present a broadband microwave setup for electrically detected magnetic resonance (EDMR) based on microwave antennae with the ability to apply arbitrarily shaped pulses for the excitation of electron spin resonance (ESR) and nuclear…
Intense few-to-sub-femtosecond soft x-ray pulses can produce neutral, two-site excited double-core-hole states by promoting two core electrons to the same unoccupied molecular orbital. We theoretically investigate double nitrogen K-edge…
We present an approach for initiating and tracing ultra-fast electron dynamics in core-excited atoms, molecules and solids. The approach is based on stimulated resonant inelastic x-ray scattering induced by a single, chirped, broadband…
We study the effect of the spreading widths on the excitation probabilities of the double giant dipole resonance. We solve the coupled-channels equations for the excitation of the giant dipole resonance and the double giant dipole…
We calculate the frequency-dispersed nonlinear transmission signal of a phase-shaped visible pulse to fourth order in the field. Two phase profiles, a phase-step and phase-pulse, are considered. Two dimensional signals obtained by varying…
Broadband inversion pulses that rotate all magnetization components 180 degrees about a given fixed axis are necessary for refocusing and mixing in high-resolution NMR spectroscopy. The relative merits of various methodologies for…
Improving resolution and sensitivity will widen possible medical applications of magnetic particle imaging. Pulsed excitation promises such benefits, at the cost of more complex hardware solutions and restrictions on drive field amplitude…
Using one-dimensional semiconductor Bloch equations, we investigate the multiband dynamics of electrons in a cutoff extension scheme employing an infrared pulse with additional UV injection. An extended three-step model is firstly validated…
This work investigates the utility of femtosecond pulse shaping in increasing the efficiency of Raman excitation of molecules in the strong-field interaction regime. We study experimentally and theoretically the effect of pulse shaping on…