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We have studied Ir spin and orbital magnetic moments in the double perovskites La$_{2-x}$Sr$_x$CoIrO$_6$ by x-ray magnetic circular dichroism. In La$_2$CoIrO$_6$, Ir$^{4+}$ couples antiferromagnetically to the weak ferromagnetic moment of…

Strongly Correlated Electrons · Physics 2012-06-22 A. Kolchinskaya , P. Komissinskiy , M. Baghaie Yazdi , M. Vafaee , D. Mikhailova , N. Narayanan , H. Ehrenberg , F. Wilhelm , A. Rogalev , L. Alff

A three-orbital-model approach for studying spin wave excitations in the strongly spin-orbit coupled layered perovskite iridates is presented which provides a unified description of magnetic excitations as well as the electronic band…

Strongly Correlated Electrons · Physics 2017-04-05 Shubhajyoti Mohapatra , Jeroen van den Brink , Avinash Singh

We report Resonant Inelastic X-ray Scattering (RIXS) study of the magnetic excitation spectrum in a highly insulating Eu$_{2}$Ir$_{2}$O$_{7}$ single crystal that exhibits a metal-insulator transition at $T_{MI}$ = 111(7) K. A propagating…

Strongly Correlated Electrons · Physics 2018-06-13 Sae Hwan Chun , Bo Yuan , Diego Casa , Jungho Kim , Chang-Yong Kim , Zhaoming Tian , Yang Qiu , Satoru Nakatsuji , Young-June Kim

Being motivated by recent experimental studies, we investigate magnetic structures of the Mo pyrochlores $A_2$Mo$_2$O$_7$ ($A$= Y, Nd, and Gd) and their impact on the electronic properties. The latter are closely related with the behavior…

Strongly Correlated Electrons · Physics 2009-11-07 I. V. Solovyev

The quantum pyrochlore antiferromagnet is studied by perturbative expansions and exact diagonalization of small clusters. We find that the ground state is a spin-liquid state: The spin-spin correlation functions decay exponentially with…

Strongly Correlated Electrons · Physics 2009-10-31 Benjamin Canals , Claudine Lacroix

We construct and analyze a microscopic model for insulating rock salt ordered double perovskites, with the chemical formula A$_2$BB'O$_6$, where the magnetic ion B' has a 4d$^2$ or 5d$^2$ electronic configuration and forms a face centered…

Strongly Correlated Electrons · Physics 2013-01-15 Gang Chen , Leon Balents

We investigated the electronic and magnetic properties of the pyrochlore oxide Cd$_2$Os$_2$O$_7$ using the density-functional theory plus on-site repulsion ($U$) method, and depict the ground-state phase diagram with respect to $U$. We…

Strongly Correlated Electrons · Physics 2012-06-15 Hiroshi Shinaoka , Takashi Miyake , Shoji Ishibashi

Owing to comparably strong spin-orbit coupling and Hubbard interaction, iridium based 227 pyrochlore oxides harbor a rich confluence of competing magnetic orders and emergent multipolar Weyl quasiparticles. Here we show that this family of…

Strongly Correlated Electrons · Physics 2021-06-30 Konstantinos Ladovrechis , Tobias Meng , Bitan Roy

The structural, electronic and magnetic properties of Fe7S8 material have been studied within the framework of the ab-initio calculations, the mean field approximation (MFA) and Monte Carlo simulation (MCS). Our study shows that two forms…

Materials Science · Physics 2020-12-09 S. Benyoussef , Y. EL Amraoui , H. Ez-Zahraouy , D. Mezzane , Z. Kutnjak , I. A. Luk'yanchuk , M. EL Marssi

Magnetic pyrochlore oxides, including the spin ice materials, have proved to be a rich field for the study of geometrical frustration in 3 dimensions. Recently, a new family of magnetic oxides has been synthesised in which the half of the…

Strongly Correlated Electrons · Physics 2015-12-08 Owen Benton , Nic Shannon

The possible existence of topological insulators in cubic pyrochlore iridates A$_{2}$Ir$_{2}$O$_{7}$ (A = Y or rare-earth elements) is investigated by taking into account the strong spin-orbit coupling and trigonal crystal field effect. It…

Strongly Correlated Electrons · Physics 2015-03-14 Bohm-Jung Yang , Yong Baek Kim

A new class of materials termed topological insulators have been intensively investigated due to their unique Dirac surface state carrying dissipationless edge spin currents. Recently, it has been theoretically proposed that the three…

Materials Science · Physics 2015-08-07 T. C. Fujita , Y. Kozuka , M. Uchida , A. Tsukazaki , T. Arima , M. Kawasaki

The consequences of nonmagnetic-ion dilution for the pyrochlore family Y$_{2}$($M_{1-x}N_{x}$)$_{2}$O$_{7}$ ($M$ = magnetic ion, $N$ = nonmagnetic ion) have been investigated. As a first step, we experimentally examine the magnetic…

Strongly Correlated Electrons · Physics 2017-10-04 L. Shen , C. Greaves , R. Riyat , T. C. Hansen , E. Blackburn

Non-Fermi liquid behavior in some fermionic systems have attracted significant interest in last few decades. Certain pyrochlore iridates with stronger spin-orbit coupling strength have recently been added to the list. Here, we provide…

Strongly Correlated Electrons · Physics 2022-01-03 Md Salman Khan , Ilaria Carlomagno , Carlo Meneghini , P. K. Biswas , Fabrice Bert , Subham Majumdar , Sugata Ray

Pyrochlore magnets are candidates for spin-ice behavior. We present theoretical simulations of relevance for the pyrochlore family R2Ti2O7 (R= rare earth) supported by magnetothermal measurements on selected systems. By considering long…

Statistical Mechanics · Physics 2009-10-31 R. Siddharthan , B. S. Shastry , A. P. Ramirez , A. Hayashi , R. J. Cava , S. Rosenkranz

We report the low temperature magnetic properties of the pyrochlore Pr$_2$Hf$_2$O$_7$. Polycrystalline and single-crystal samples are investigated using time-of-flight neutron spectroscopy and macroscopic measurements, respectively. The…

We report neutron diffraction measurements of the magnetic structures in two pyrochlore iridates, Yb2Ir2O7 and Lu2Ir2O7. Both samples exhibit the all-in-all-out magnetic structure on the Ir4+ sites below TN~ 150,K, with a low temperature…

We report detailed measurements of the low temperature magnetic phase diagram of Er$_2$Ti$_2$O$_7$. Heat capacity and time-of-flight neutron scattering studies of single crystals, subject to magnetic fields applied along the…

Strongly Correlated Electrons · Physics 2012-07-16 J. P. C. Ruff , J. P. Clancy , A. Bourque , M. A. White , M. Ramazanoglu , J. S. Gardner , Y. Qiu , J. R. D. Copley , H. A. Dabkowska , B. D. Gaulin

The pyrochlore antiferromagnet Tb2Ti2O7 has proven to be an enigma to experimentalists and theorists working on frustrated magnetic systems. The experimentally determined energy level structure suggests a local <111> Ising antiferromagnet…

Statistical Mechanics · Physics 2009-11-10 M. Enjalran , M. J. P. Gingras , Y. -J. Kao , A. Del Maestro , H. R. Molavian

The local electronic structure of YBa2Cu3O7 has been calculated using first-principles cluster methods. Several clusters embedded in an appropriate background potential have been investigated. The electric field gradients at the copper and…

Superconductivity · Physics 2009-11-07 S. Renold , S. Plibersek , E. P. Stoll , T. A. Claxton , P. F. Meier
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