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A model for a Heisenberg antiferromagnet on a pyrochlore lattice with exchange and dipole-dipole interactions is studied via mean-field theory. In treating the dipoles by use of the Ewald method, a soft (critical) mode with a unique…

Statistical Mechanics · Physics 2007-05-23 Matthew Enjalran , Michel J. P. Gingras

We study the finite temperature and magnetic field phase diagram of electrons on the pyrochlore lattice subject to a local repulsion as a model for the pyrochlore iridates. We provide the most general symmetry-allowed Hamiltonian, including…

Strongly Correlated Electrons · Physics 2013-04-02 William Witczak-Krempa , Ara Go , Yong Baek Kim

Effects of spin-orbit interactions in condensed matter are an important and rapidly evolving topic. Strong competition between spin-orbit, on-site Coulomb and crystalline electric field interactions in iridates drives exotic quantum states…

Strongly Correlated Electrons · Physics 2018-02-27 Gang Cao , Pedro Schlottmann

We present the study of magnetization, thermal expansion, specific heat, resistivity, and a.c. susceptibility of (Pr$_{1-y}$Eu$_y$)$_{0.7}$Ca$_{0.3}$CoO$_3$ cobaltites. The measurements were performed on ceramic samples with $y = 0.12 -…

The magnetic order of the localized Eu$^{2+}$ spins in optimally-doped Eu(Fe$_{1-x}$Ir$_{x}$)$_{2}$As$_{2}$ ($\mathit{x}$ = 0.12) with superconducting transition temperature $\mathit{T_{SC}}$ = 22 K was investigated by single-crystal…

Superconductivity · Physics 2015-02-20 W. T. Jin , Wei Li , Y. Su , S. Nandi , Y. Xiao , W. H. Jiao , M. Meven , A. P. Sazonov , E. Feng , Yan Chen , C. S. Ting , G. H. Cao , Th. Brückel

We perform a general study of spin ordering on the pyrochlore lattice with a 3:1 proportionality of two spin polarizations. Equivalently, this describes valence bond solid conformations of a quantum dimer model on the diamond lattice. We…

Strongly Correlated Electrons · Physics 2007-05-23 Doron L. Bergman , Gregory A. Fiete , Leon Balents

We consider the electronic structure of, and magnetic exchange (spin) interactions between, nominally nonmagnetic Eu^3+ ions (4f^6, S=3, L=3, J=0) within the context of the rocksalt structure compounds EuN and EuP. Both compounds are ionic…

Materials Science · Physics 2009-11-11 M. D. Johannes , W. E. Pickett

We match analytic results to numerical calculations to provide a detailed picture of the metal-insulator and topological transitions found in density functional plus cluster dynamical mean-field calculations of pyrochlore iridates. We…

Strongly Correlated Electrons · Physics 2017-11-30 Runzhi Wang , Ara Go , Andrew Millis

Spin-orbit effects in heavy 5$d$ transition metal oxides, in particular, iridates, have received enormous current interest due to the prediction as well as the realization of a plethora of exotic and unconventional magnetic properties.…

Strongly Correlated Electrons · Physics 2021-09-22 Sayantika Bhowal , Indra Dasgupta

We present AC and DC magnetometry, heat capacity, muon spin relaxation ($\mu$SR) and resonant inelastic X-ray scattering (RIXS) studies of the pyrochlore osmate Y$_2$Os$_2$O$_7$. We observe a non-zero effective moment governed by…

Neutron inelastic scattering has been used to probe the spin dynamics of the quantum (S=1/2) ferromagnet on the pyrochlore lattice Lu2V2O7. Well-defined spin waves are observed at all energies and wavevectors, allowing us to determine the…

Strongly Correlated Electrons · Physics 2015-06-19 M. Mena , R. S. Perry , T. G. Perring , M. D. Le , S. Guerrero , M. Storni , D. T. Adroja , Ch. Ruegg , D. F. McMorrow

We report density functional calculations addressing the electronic structure and magnetic properties of delafossite PdCrO2. We find substantial magnetic interactions in the c-axis direction as well as beyond first nearest neighbors…

Strongly Correlated Electrons · Physics 2015-03-19 K. P. Ong , D. J. Singh

Pyrochlore iridates have attracted growing attention because of a theoretical prediction of a possible topological semimetal phase originating from all-in-all-out spin ordering. Related to the topological band structure, recent findings of…

Materials Science · Physics 2016-01-14 T. C. Fujita , M. Uchida , Y. Kozuka , S. Ogawa , A. Tsukazaki , T. Arima , M. Kawasaki

We present a low-energy muon-spin-rotation study of the magnetic and superconducting properties of YBa2Cu3O7/PrBa2Cu3O7 trilayer and bilayer heterostructures. By determining the magnetic-field profiles throughout these structures we show…

Magnetic and magnetoelastic properties of terbium titanate pyrochlore in paramagnetic phase are simulated. The magnetic field and temperature dependences of magnetization and forced magnetostriction in Tb2Ti2O7 single crystals and…

Strongly Correlated Electrons · Physics 2011-10-27 V. V. Klekovkina , A. R. Zakirov , B. Z. Malkin , L. A. Kasatkina

Motivated by the potential chiral spin liquid in the metallic spin ice Pr2Ir2O7, we consider how such a chiral state might be selected from the spin ice manifold. We propose that chiral fluctuations of the conducting Ir moments promote…

Strongly Correlated Electrons · Physics 2013-04-03 Rebecca Flint , T. Senthil

Magnetic systems with spins sitting on a lattice of corner sharing regular tetrahedra have been particularly prolific for the discovery of new magnetic states for the last two decades. The pyrochlore compounds have offered the playground…

Strongly Correlated Electrons · Physics 2017-10-05 P. Dalmas de Reotier , C. Marin , A. Yaouanc , C. Ritter , A. Maisuradze , B. Roessli , A. Bertin , P. J. Baker , A. Amato

We document the coexistence of ferro- and anti-ferromagnetism in pyrochlore $\rm Yb_2Ti_2O_7$ using three neutron scattering techniques on stoichiometric crystals: elastic neutron scattering shows a canted ferromagnetic ground state,…

Strongly Correlated Electrons · Physics 2020-10-27 A. Scheie , J. Kindervater , S. Zhang , H. J. Changlani , G. Sala , G. Ehlers , A. Heinemann , G. S. Tucker , S. M. Koohpayeh , C. Broholm

Magnetometry, electrical transport, and neutron scattering measurements were performed on single crystals of the Fe^{4+}-containing perovskite-related phase Sr_3Fe_2O_7-x as a function of oxygen content. Although both the crystal structure…

Strongly Correlated Electrons · Physics 2013-06-12 D. C. Peets , J. -H. Kim , P. Dosanjh , M. Reehuis , A. Maljuk , N. Aliouane , C. Ulrich , B. Keimer

We report inelastic neutron scattering measurements from our newly synthesized single crystals of the structurally metastable antiferromagnetic pyrochlore Yb$_{2}$Ge$_{2}$O$_{7}$. We determine the four symmetry-allowed nearest-neighbor…

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