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Characterizing a monolayer of biological molecules has been a major challenge. We demonstrate nanophotonic wave-guide enhanced Raman spectroscopy (NWERS) of monolayers in the near-infrared region, enabling real-time measurements of the…
We present a simple method and its experimental implementation to completely determine the characteristics of the pump-and-probe pulse and the Stokes pulse in a coherent anti-Stokes Raman scattering microscope at sample level without…
Stimulated Raman scattering (SRS) microscopy offers great potential to surpass fluorescent-based approaches, owing to the sharp linewidth of Raman vibrations amenable to super-multiplex cell imaging, but currently lacks one crucial…
The integration of stimulated Raman scattering (SRS) and second order nonlinearity in non-centrosymmetric photonic microresonators presents a highly promising solution for developing on-chip coherent light sources with exceptional bandwidth…
We present a tunable, continuous-wave (CW) laser system emitting at 213 nm, based on the frequency quadrupling of a single Ti:sapph laser. The setup features two sequential, cavity-enhanced second-harmonic generation (SHG) stages. The first…
Quantifying formidable multiple coupling effects involved in Surface-enhanced Raman scattering (SERS) is a prerequisite for accurate design of SERS probes with superior detection limit and uniformity which are the targets for trace…
We report that rhomb-shaped metal nanoantenna arrays support multiple plasmonic resonances, making them favorable bio-sensing substrates. Besides the two localized plasmonic dipole modes associated with the two principle axes of the rhombi,…
Miniaturized photonic cavities generating nonlinear optical states of light are central to telecommunications and metrology applications. The emergence of such states is primarily underpinned by the ubiquitous Kerr nonlinearity that is…
Since its first demonstration in the sixties, coherent anti-Stokes Raman scattering (CARS) has become a powerful spectroscopic sensing tool with broad applications in biology and chemistry. However, it is a complex nonlinear optical process…
We report on the development of a compact (volume $\approx$ 100\:cm$^3$), multimode diffraction-limited Raman spectrograph and probe designed to be compact as possible. The spectrograph uses `off the shelf' optics, a custom 3D-printed…
Frequency modulation coherent anti-Stokes Raman scattering (FM CARS) is presented, using a compact as well as fast and widely tunable fiber-based light source. With this light source Raman resonances between 700 cm$^{-1}$ and 3200 cm$^{-1}$…
Many fields such as bio-spectroscopy and photochemistry often require sources of vacuum ultraviolet (VUV) pulses featuring a narrow linewidth and tunable over a wide frequency range. However, the majority of available VUV light sources do…
We study stimulated Raman scattering (SRS) in laser-fusion conditions with the Eulerian Vlasov code ELVIS. Back SRS from homogeneous plasmas occurs in sub-picosecond bursts and far exceeds linear theory. Forward SRS and re-scatter of back…
Interaction of a high intensity short laser pulse with near-critical plasmas allows to achieve extremely high coupling efficiency and transfer laser energy to energetic ions. One dimensional Particle-In-Cell (PIC) simulations are considered…
The "Impulsive Stimulated Raman Scattering" (ISRS), is generally performed using ultrashort laser pulses. It shifts the frequency of the laser beam without any change of the wave surfaces and any appearance of extra lines. ISRS works with…
This study analyzed the optical techniques for high resolution, low-noise spectroscopy of a hyperfine structure (HFS) made of ytterbium-isotope 171 ions ($^{171}\mathrm{Yb}^{3+}$:$\mathrm{Y}_2\mathrm{SiO}_5$). Large energy spacings in…
We demonstrate a hybrid distributed fiber sensing system for multi-parameter detection. The integration of phase-sensitive optical time domain reflectometry ({\Phi}-OTDR) and Brillouin optical time domain reflectometry (B-OTDR) enables…
Laser wakefield accelerators have great potential as the basis for next generation compact radiation sources because their accelerating gradients are three orders of magnitude larger than traditional accelerators. However, X-ray radiation…
Coherent Raman scattering provides highly sensitive vibrational analysis through nonlinear light-matter interactions. However, its application to metal interfaces has remained challenging because the intrinsically large non-resonant…
Nonlinear optical microscopy allows rapid high-resolution microscopy with image contrast generated from intrinsic properties of the sample. Established modalities such as multiphoton excited fluorescence and second/third-harmonic generation…