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The coupled quantum dynamics of electrons and protons is ubiquitous in many dynamical processes involving light-matter interaction, such as solar energy conversion in chemical systems and photosynthesis. A first-principles description of…

Chemical Physics · Physics 2023-11-07 Jianhang Xu , Ruiyi Zhou , Tao E. Li , Volker Blum , Sharon Hammes-Schiffer , Yosuke Kanai

Positions of protons in DNA hydrogen bonds are fundamental for the fidelity of the replication process. Because the hydrogen bond is partially covalent the electronic structure of DNA plays an important role in the replication process.…

Strongly Correlated Electrons · Physics 2007-05-23 Chun-Min Chang , A. H. Castro Neto , A. R. Bishop

Hydrogen bonds play a pivotal role in chemistry, biology, and condensed-matter physics, where quantum tunnelling can strongly influence structure and dynamics. Isotope substitution (H $\rightarrow$ D) provides a sensitive probe of such…

Chemical Physics · Physics 2025-11-05 Krishna Kingkar Pathak

Collective decays of multiply-excited atoms become subradiant and bound in space when they are strongly coupled to the guided modes in an atom-waveguide interface. In this interface, we analyze their average density-density and modified…

Quantum Physics · Physics 2021-06-29 H. H. Jen

When two or more atoms bind to a solid surface, the substrate can mediate an interaction between them. In this paper, we use density-functional theory to quantify the substrate-mediated pair interaction between two adatoms on a…

Materials Science · Physics 2007-05-23 Kristen A. Fichthorn , Matthias Scheffler

In hydrogen bonded systems, nuclear quantum effects such as zero-point motion and tunneling can significantly affect their material properties through underlying physical and chemical processes. Presently, direct observation of the…

Leading neutron production on protons is known to be subject to strong absorptive corrections, which have been under debate for a long time. On nuclear targets these corrections are significantly enhanced and push the partial cross sections…

Nuclear Theory · Physics 2017-04-05 B. Z. Kopeliovich , I. K. Potashnikova , Ivan Schmidt

Water is a key ingredient for life and plays a central role as solvent in many biochemical reactions. However, the intrinsically quantum nature of the hydrogen nucleus, revealing itself in a large variety of physical manifestations,…

In solid acid solid electrolytes CsH$_2$PO$_4$ and CsHSO$_4$, mechanisms of fast proton conduction have long been debated and attributed to either local proton hopping or polyanion rotation. However, the precise role of polyanion rotation…

The work is devoted to the investigation of physical nature of H-bond. The H-bond potential $\Phi_{H} (r,\Omega)$ is studied as an irreducible part of the interaction energy of water molecules. It is defined as a difference between…

Chemical Physics · Physics 2012-02-27 Paul Makhlaichuk , Mykola Malomuzh , Igor Zhyganiuk

The hitherto neglected phonon-exchange interaction between interstitial protons in metal lattices is found to be large. It is shown that this effect may give rise to a phase of protonic superconductivity, characterized by the formation of…

Superconductivity · Physics 2007-05-23 J. S. Brown

Hydrogen bond is often assumed to be a purely electrostatic interaction between a electron-deficient hydrogen atom and a region of high electron density. Here, for the first time, we directly image hydrogen bond in real space by…

Chemical Physics · Physics 2013-02-28 Xiu Chen , Shuyi Liu , Lacheng Liu , Xiaoqing Liu , Yingxing Cai , Nianhua Liu , Li Wang

Break-up and recombination processes for loosely-bound molecules composed of atoms with a large scattering length $a$ necessarily involve interactions that are nonperturbative in the exact 2-body interaction. If these processes involve…

Other Condensed Matter · Physics 2009-11-11 Eric Braaten , Dongqing Zhang

The frequency dependence of dynamical conductivity of the quasi-one-dimensional structures with hydrogen bonds is studied on the basis of pseudospin-electron model. It takes into account the proton-electron interaction, external…

Statistical Mechanics · Physics 2012-04-27 R. Ya. Stetsiv

The pair- and three-proton interaction potentials for metal-phase hydrogen are calculated. Irreducible three-proton interactions are shown to be essential in the development of the metal hydrogen structure. Possible manifestations of the…

Materials Science · Physics 2007-05-23 E. V. Vasiliu , S. D. Kaim , N. P. Kovalenko

The thermodynamics of a homopolymeric chain with both Van der Waals and highly-directional hydrogen bond interaction is studied. The effect of hydrogen bonds is to reduce dramatically the entropy of low-lying states and to give raise to…

Condensed Matter · Physics 2009-10-31 J. Borg , M. H. Jensen , K. Sneppen , G. Tiana

Photon-photon interactions mediated by an atomic gas can effect efficient polarization exchanges between two beams, leaving the medium exactly in its initial state. In, e.g., hydrogen, the distance required for macroscopic exchange is of…

Quantum Physics · Physics 2015-06-18 R. F. Sawyer

When atoms are coupled to a common electromagnetic environment, the exchange of photons through dipole-dipole interactions leads to the emergence of cooperative effects. As a particular example, superradiance arises from spontaneous…

Quantum Physics · Physics 2024-09-11 Hanzhen Ma , Oriol Rubies-Bigorda , Susanne F. Yelin

We perform simulations of a system containing simple model proteins and a polymer representing chromatin. We study the interplay between protein-protein and protein-chromatin interactions, and the resulting condensates which arise due to…

Soft Condensed Matter · Physics 2022-07-20 Marco Ancona , Chris A. Brackley

We have performed ab initio molecular dynamics simulations to study the nature of the synchronous double proton transfer in formic acid dimer. In order to understand the evolution of the bonding during the double proton transfer, we have…

Materials Science · Physics 2007-05-23 Sharan Shetty , Sourav Pal , Dilip G. Kanhere , Annick Goursot
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