English
Related papers

Related papers: Alignment dependent ultrafast electron-nuclear dyn…

200 papers

We extend our recently developed semiclassical strong-field Herman-Kluk propagator (SFHK) method to calculate high-order harmonic generation (HHG) for atoms in intense lasers. We show that our method, based on a combination of the…

Atomic Physics · Physics 2026-01-27 Phi-Hung Tran , Hao Quan Truong , R. Esteban Goetz , Anh-Thu Le

We investigate the high harmonic generation (HHG) from solids by simulating the dynamics of a single active electron in periodic potentials. The corresponding time-dependent Schr\"odinger equations (TDSE) are solved numerically by using…

Atomic Physics · Physics 2016-03-31 Zhong Guan , Xiao-Xin Zhou , Xue-Bin Bian

High harmonic generation (HHG) has unleashed the power of strong laser physics in solids. Here we investigate HHG from a large system, solid C$_{60}$, with 240 valence electrons engaging harmonic generation at each crystal momentum, the…

Materials Science · Physics 2020-12-23 G. P. Zhang , Y. H. Bai

We perform a detailed analysis of high-order harmonic generation (HHG) in atoms within the strong field approximation (SFA) by considering spatially inhomogeneous monochromatic laser fields. We investigate how the individual pairs of…

Atomic Physics · Physics 2015-06-05 T. Shaaran , M. F. Ciappina , M. Lewenstein

Attosecond light sources based on high-order harmonic generation (HHG) constitute to date the only table-top solution for producing coherent broadband radiation covering the spectral range from the extreme ultraviolet to the soft X-rays.…

We analyze the influence of different recombination scenarios, involving one or two centers, on high-order harmonic generation (HHG) in diatomic molecules, for different values of the internuclear separation. We work within the strong-field…

Atomic Physics · Physics 2015-05-13 C. Figueira de Morisson Faria

We study high order harmonics generation (HHG) in crystalline silicon and diamond subjected to near and mid-infrared laser pulses. We employ time-dependent density functional theory and solve the time-dependent Kohn-Sham equation in the…

Materials Science · Physics 2022-08-31 David Freeman , Shunsuke Yamada , Atsushi Yamada , Kazuhiro Yabana , Anatoli Kheifets

The interaction of a helium atom with intense short 800 nm laser pulse is studied theoretically beyond the single-active-electron approximation. For this purpose, the time-dependent Schr\"odinger equation for the two-electron wave packet…

Atomic and Molecular Clusters · Physics 2017-03-08 Anton N. Artemyev , Lorenz S. Cederbaum , Philipp V. Demekhin

State-of-the-art experiments employ strong ultrafast optical fields to study the nonlinear response of electrons in solids on an attosecond time-scale. Notably, a recent experiment retrieved a 3rd order nonlinear susceptibility by comparing…

By employing the exact diagonalization method, we investigate the high-harmonic generation (HHG) of the correlated systems under the strong laser irradiation. For the extended Hubbard model on a periodic chain, HHG close to the quantum…

Strongly Correlated Electrons · Physics 2022-03-07 Can Shao , Hantao Lu , Xiao Zhang , Chao Yu , Takami Tohyama , Ruifeng Lu

The order of high harmonics emitted by an atom in an intense laser field is limited by the so-called cutoff frequency. Solving the time-dependent Schr\"odinger equation, we show that this frequency can be increased considerably by a…

Atomic Physics · Physics 2016-09-08 Carla Figueira de Morisson Faria , Jan-Michael Rost

The alignment dependence of the ionization behavior of H$_2$ exposed to intense ultrashort laser pulses is investigated on the basis of solutions of the full time-dependent Schr\"odinger equation within the fixed-nuclei and dipole…

Quantum Physics · Physics 2013-05-29 Yulian V. Vanne , Alejandro Saenz

Using Time-Dependent Density Functional Theory (TDDFT) nonlinear nonperturbative response of the molecular system is studied for photoisomerization reaction. The 1,3-cyclohexadiene photoisomerization is probed by the high-harmonic…

Chemical Physics · Physics 2024-08-06 Lauren Bauerle , Agnieszka Jaron

A theoretical model is developed describing high-order harmonic generation (HHG) from a gas of multiply-charged ions driven by a laser field of relativistic intensity. Macroscopic propagation of harmonics is investigated in a relativistic…

Atomic Physics · Physics 2012-02-21 Markus C. Kohler , Karen Z. Hatsagortsyan

We present a study of the possibility to significantly enhance the efficiency of high-order harmonic generation (HHG) using few-cycle optical waveforms obtained by superposing two laser pulses of different color delayed optimally relative…

Optics · Physics 2024-12-11 O. V. Meshkov , M. Yu. Emelin , M. Yu. Ryabikin

We experimentally disentangle the contributions of different quantum paths in high-order harmonic generation (HHG) from the spectrally and spatially resolved harmonic spectra. By adjusting the laser intensity and focusing position, we…

Atomic Physics · Physics 2015-10-08 Lixin He , Pengfei Lan , Qingbin Zhang , Chunyang Zhai , Feng Wang , Wenjing Shi , Peixiang Lu

High-order harmonic generation (HHG) in gases leads to short-pulse extreme ultraviolet (XUV) radiation useful in a number of applications, for example, attosecond science and nanoscale imaging. However, this process depends on many…

In the past two decades high-harmonic generation (HHG) has become a key process in ultra-fast science due to the extremely short time-structure of the underlying electron dynamics being imprinted in the emitted harmonic light bursts. After…

Atomic Physics · Physics 2012-01-25 Markus C. Kohler , Thomas Pfeifer , Karen Z. Hatsagortsyan , Christoph H. Keitel

We present theoretical predictions of high-order harmonic generation (HHG) resulting from the interaction of short femtosecond laser pulses with metal nanotips. It has been demonstrated that high energy electrons can be generated using…

High-order harmonic generation (HHG) in the relativistic regime is employed to obtain zeptosecond pulses of $\gamma$-rays. The harmonics are generated from atomic systems in counterpropagating strong attosecond laser pulse trains of linear…

Atomic Physics · Physics 2007-07-20 Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel