Related papers: Multiple Rabi Splittings under Ultra-Strong Vibrat…
One of the most popular subjects now being researched in molecular science is strong light-matter coupling. The introduction of vibrational strong coupling and the formation vibro-polaritonic states tend to modify chemical reactivity,…
We consider multiphoton dynamics of a quantum system composed of a three-state atom (a qutrit) and a single-mode photonic field in the ultrastrong and deep strong coupling regimes, when the coupling strength is comparable to or larger than…
We demonstrate room-temperature strong-coupling between a mid-infrared ($\lambda$=9.9 $\mu$m) intersubband transition and the fundamental cavity mode of a metal-insulator-metal resonator. Patterning of the resonator surface enables…
As pioneering experiments have shown, strong vibrational coupling between molecular vibrations and light modes in an optical cavity can significantly alter molecular properties and even affect chemical reactivity. However, the current…
Vibrational strong coupling is emerging as a promising tool to modify molecular properties, by making use of hybrid light-matter states known as polaritons. Fabry-Perot cavities filled with organic molecules are typically used, and the…
We demonstrate theoretically the parametric oscillator behavior of a two-level quantum system with broken inversion symmetry exposed to a strong electromagnetic field. A multitude of resonance frequencies and additional harmonics in the…
We demonstrate Resonant Tunneling Diodes, embedded in double metal cavities, strongly coupled to the cavity field, while maintaining their electronic properties. We measure the polariton dispersion and find a relative vacuum Rabi splitting…
We derive the transition rates, dephasing rates, and Lamb shifts for a system consisting of many molecules collectively coupled to a resonant cavity mode. Using a variational polaron master equation, we show that strong vibrational…
Nonadiabatic phenomena are investigated in the rovibrational motion of molecules confined in an infrared cavity. Conical intersections (CIs) between vibrational polaritons, similar to CIs between electronic polaritonic surfaces, are found.…
The study of strong light-matter interaction in van der Waals materials is at the forefront of current research in physics and chemistry, and it can be enhanced dramatically by employing resonances. Here we present the first observation of…
We report on the strong coupling between the Bloch surface wave supported by an inorganic multilayer structure and $J$-aggregate excitons in an organic semiconductor. The dispersion curves of the resulting polariton modes are investigated…
We study the vacuum Rabi splitting of a qubit ultrastrongly coupled to a high-$Q$ cavity mode and a radiation reservoir. Three methods are employed: a numerically exact variational approach with a multiple Davydov ansatz, the rotating-wave…
Strong light-matter coupling manifested by vacuum Rabi splitting has attracted tremendous attention due to its fundamental importance in cavity quantum-electrodynamics research and great potentials in quantum information applications. A…
Multi-normal-mode splitting peaks are experimentally observed in a system with Doppler-broadened two-level atoms inside a relatively long optical cavity. In this system, the atoms-cavity interaction can reach the ``superstrong coupling"…
Two-dimensional (2D) semiconducting microcavity, where exciton-polaritons can be formed, constitues a promising setup for exploring and manipulating various regimes of light-matter interaction. Here, the coupling between 2D excitons and…
Cavity electro-(opto-)mechanics allows us to access not only single isolated but also multiple mechanical modes in a massive object. Here we develop a multi-mode electromechanical system in which a several membrane vibrational modes are…
Recently, we predicted theoretically that in cavities that support several longitudinal modes, strong coupling can occur in very different manners, depending on the system parameters. Distinct longitudinal cavity modes are either entangled…
Strong coupling of molecular vibrations to an infrared cavity mode affects their nature by creating dressed polariton states. We show how the single and double vibrational polariton manifolds may be controlled by varying the cavity coupling…
The coupling of a two-level system with an electromagnetic field, whose fully quantized version is the quantum Rabi model, is among the central topics of quantum physics. When the coupling strength becomes large enough that the field mode…
The central theme of cavity quantum electrodynamics is the coupling of a single optical mode with a single matter excitation, leading to a doublet of cavity polaritons which govern the optical properties of the coupled structure. Especially…