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We present an experimental study of the two-dimensional S=1/2 square-lattice antiferromagnet Cu(pz)$_2$(ClO$_4$)$_2$ (pz denotes pyrazine - $C_4H_4N_2$) using specific heat measurements, neutron diffraction and cold-neutron spectroscopy.…

Strongly Correlated Electrons · Physics 2010-07-15 N. Tsyrulin , F. Xiao , A. Schneidewind , P. Link , H. M. Rønnow , J. Gavilano , C. P. Landee , M. M. Turnbull , M. Kenzelmann

Correlation functions (CFs) of the classical Heisenberg antiferromagnet on the pyrochlore lattice are studied by solving exactly the infinite-component spin-vector model. % As in many Fully Frustrated Lattices, the constraint due to the…

Strongly Correlated Electrons · Physics 2009-11-07 Benjamin Canals , Dmitry Garanin

We present a muon spin relaxation study on the Ising pyrochlore Nd$_2$Zr$_2$O$_7$ which develops an "all-in-all-out" magnetic order below 0.4~K. At 20~mK far below the ordering transition temperature, the zero-field muon spin relaxation…

Materials Science · Physics 2016-09-07 J. Xu , C. Balz , C. Baines , H. Luetkens , B. Lake

We report detailed measurements of the low temperature magnetic phase diagram of Er$_2$Ti$_2$O$_7$. Heat capacity and time-of-flight neutron scattering studies of single crystals, subject to magnetic fields applied along the…

Strongly Correlated Electrons · Physics 2012-07-16 J. P. C. Ruff , J. P. Clancy , A. Bourque , M. A. White , M. Ramazanoglu , J. S. Gardner , Y. Qiu , J. R. D. Copley , H. A. Dabkowska , B. D. Gaulin

We report low-temperature powder X-ray and neutron diffraction studies on breathing pyrochlore magnets Cu$M$Cr$_{4}$S$_{8}$ ($M$ = Al, Ga), which undergo a magnetic transition at $T_{\rm N} \approx$ 21 and 31 K for {$M$ = Al and Ga,…

Materials Science · Physics 2024-05-09 Masaki Gen , Taro Nakajima , Hiraku Saito , Yusuke Tokunaga , Taka-hisa Arima

We address the concomitant metal-insulator transition (MIT) and antiferromagnetic ordering in the novel pyrochlore iridate Eu2Ir2O7 by combining x-ray absorption spectroscopy, x-ray and neutron diffractions and density functional theory…

The perovskite TbFe$_{0.5}$Cr$_{0.5}$O$_3$ shows two anomalies in the magnetic susceptibility at $T_N$ = 257K and $T_{SR}$ = 190K which are respectively, the antiferromagnetic and spin reorientation transition that occur in the Fe/Cr…

We report measurements of the specific heat and magnetization of single crystal samples of the spin-1/2 kagome compound ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$ (herbertsmithite), a promising quantum spin-liquid candidate, in high magnetic fields and…

We present an experimental study of the pyrochlore coumpound Nd2Zr2O7 by means of neutron scattering and magnetization measurements down to 90 mK. The Nd$^{3+}$ magnetic moments exhibit a strong local $\langle$111$\rangle$ Ising anisotropy…

Strongly Correlated Electrons · Physics 2016-01-05 E. Lhotel , S. Petit , S. Guitteny , O. Florea , M. Ciomaga Hatnean , C. Colin , E. Ressouche , M. R. Lees , G. Balakrishnan

In this Comment we argue that Ho$_2$Ti$_2$O$_7$ does not exhibit a transition to a partially ordered state unlike what is argued in PRL 83, 1854 (1999), that it exhibits spin ice behavior, and that the experimental specific heat data by…

Disordered Systems and Neural Networks · Physics 2016-08-31 B. C. den Hertog , Michel J. P. Gingras , Steven T. Bramwell , Mark J. Harris

We present the low temperature magnetic properties in Ni1.5Fe1.5O4 ferrite as the function of pH at which the material was prepared by chemical route and post annealing temperature. The material is a ferri or ferromagnet, but showed…

Materials Science · Physics 2018-05-09 R. N. Bhowmik , K. S. Aneeshkumar

Inelastic neutron scattering reveals a broad continuum of excitations in Pr$_2$Zr$_2$O$_7$, the temperature and magnetic field dependence of which indicate a continuous distribution of quenched transverse fields ($\Delta$) acting on the…

Ice states, in which frustrated interactions lead to a macroscopic ground-state degeneracy, occur in water ice, in problems of frustrated charge order on the pyrochlore lattice, and in the family of rare-earth magnets collectively known as…

Strongly Correlated Electrons · Physics 2015-03-19 Nic Shannon , Olga Sikora , Frank Pollmann , Karlo Penc , Peter Fulde

We used a local susceptibility approach in extensive polarized neutron diffraction studies of the spin liquid \tbti. For a magnetic field applied along the [110] and [111] directions, we found that, at high temperature, all Tb moments are…

Strongly Correlated Electrons · Physics 2015-05-13 Arsen Gukasov , Huibo Cao , Isabelle Mirebeau , Pierre Bonville

The antiferromagnetic pyrochlore material NaCaCo$_2$F$_7$ is a thermal spin liquid over a broad temperature range (~ 140 K down to $T_F = 2.4 $K), in which magnetic correlations between Co$^{2+}$ dipole moments explore a continuous manifold…

Strongly Correlated Electrons · Physics 2017-04-26 K. A. Ross , J. M. Brown , R. J. Cava , J. W. Krizan , S. E. Nagler , J. A. Rodriguez-Rivera , M. B. Stone

The magnetic order and the spin dynamics in the antiferromagnetic entropy-stabilized oxide (Mg$_{0.2}$Co$_{0.2}$Ni$_{0.2}$Cu$_{0.2}$Zn$_{0.2}$)O (MgO-ESO) have been studied using muon spin relaxation ($\mu$SR) and inelastic neutron…

PbCuTe2O6 is a rare example of a spin liquid candidate featuring a three dimensional magnetic lattice. Strong geometric frustration arises from the dominant antiferromagnetic interaction which generates a hyperkagome network of Cu2+ ions…

Strongly Correlated Electrons · Physics 2016-03-14 P. Khuntia , F. Bert , P. Mendels , B. Koteswararao , A. V. Mahajan , M. Baenitz , F. C. Chou , C. Baines , A. Amato , Y. Furukawa

Spin ices, frustrated magnetic materials analogous to common water ice, are exemplars of high frustration in three dimensions. Recent experimental studies of the low-temperature properties of the paradigmatic Dy$_2$Ti$_2$O$_7$ spin ice…

Statistical Mechanics · Physics 2016-01-19 P. Henelius , T. Lin , M. Enjalran , Z. Hao , J. G. Rau , J. Altosaar , F. Flicker , T. Yavors'kii , M. J. P. Gingras

FeF$_3$, with its half-filled Fe$^{3+}$ $3d$ orbital, hence zero orbital angular momentum and $S=5/2$, is often put forward as a prototypical highly-frustrated classical Heisenberg pyrochlore antiferromagnet. By employing {\it ab initio}…

Strongly Correlated Electrons · Physics 2015-04-29 Azam Sadeghi , Mojtaba Alaei , Farhad Shahbazi , MIchel J. P. Gingras

Neutron scattering, a.c. magnetic susceptibility and specific heat studies have been carried out on polycrystalline Dy2Zr2O7. Unlike the pyrochlore spin ice Dy2Ti2O7, Dy2Zr2O7 crystallizes into the fluorite structure and the magnetic Dy3+…

Disordered Systems and Neural Networks · Physics 2019-07-01 J. G. A. Ramon , C. W. Wang , L. Ishida , P. L. Bernardo , M. M. Leite , F. M. Vichi , J. S. Gardner , R. S. Freitas