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The magnetization processes of the spin-3/2 antiferromagnet LiInCr4O8 comprising a "breathing" pyrochlore lattice, which is an alternating array of small and large tetrahedra, are studied under ultrahigh magnetic fields of up to 130 T using…

The magnetization (both dc and ac) of pyrochlore Eu2Ti2O7 have been investigated. Ac susceptibility measurements reveal a new unusual spin freezing below 35K for pure Eu2Ti2O7. Frequency dependence of these ac peak positions indicate slow…

Materials Science · Physics 2018-05-23 Arkadeb Pal , Abhishek Singh , Prajyoti Singh , A. K. Ghosh , Sandip Chatterjee

We study the low-temperature behaviour of the classical Heisenberg antiferromagnet with nearest neighbour interactions on the pyrochlore lattice. Because of geometrical frustration, the ground state of this model has an extensive number of…

Statistical Mechanics · Physics 2009-10-30 R. Moessner , J. T. Chalker

CuAl2O4 is a normal spinel oxide having quantum spin, S=1/2 for Cu2+. It is a rather unique feature that the Cu2+ ions of CuAl2O4 sit at a tetrahedral position, not like the usual octahedral position for many oxides. At low temperatures, it…

Motivated by recent experiments on Ce$_2$Zr$_2$O$_7$ that reveal a dynamic, liquid-like ground state, we study the nearest neighbor XYZ Hamiltonian of dipolar-octupolar pyrochlore magnets with the pseudofermion functional renormalization…

Strongly Correlated Electrons · Physics 2024-05-21 Li Ern Chern , Félix Desrochers , Yong Baek Kim , Claudio Castelnovo

Quantum spin liquid (QSL) is an exotic quantum phase of matter whose ground state is quantum-mechanically entangled without any magnetic ordering. A central issue concerns emergent excitations that characterize QSLs, which are…

Strongly Correlated Electrons · Physics 2018-05-08 Y. Tokiwa , T. Yamashita , D. Terazawa , K. Kimura , Y. Kasahara , T. Onishi , Y. Kato , M. Halim , P. Gegenwart , T. Shibauchi , S. Nakatsuji , E. -G. Moon , Y. Matsuda

We report the low-temperature magnetothermal properties and spin dynamics of a mixed pyrochlore, Dy2GaSbO7 through the coordination of measurements of dc magnetization, ac susceptibility, and heat capacity, and CF computation. In Dy2GaSbO7,…

Materials Science · Physics 2021-04-19 Saikat Nandi , Yatramohan Jana , Jahangir Alam , Pallab Bag , S. S. Islam , Ramesh Nath

The "spin ice" state found in the rare earth pyrochlore magnets Ho2Ti2O7 and Dy2Ti2O7 offers a beautiful realisation of classical magnetostatics, complete with magnetic monopole excitations. It has been suggested that in "quantum spin ice"…

Strongly Correlated Electrons · Physics 2015-06-04 Owen Benton , Olga Sikora , Nic Shannon

We determine the magnetic phase diagram for the YBa$_2$Cu$_3$O$_{6+x}$ and La$_{2-x}$Sr$_x$CuO$_4$ systems from various NMR experiments. We discuss the possible interpretation of NMR and neutron scattering experiments in these systems in…

Condensed Matter · Physics 2009-10-28 V. Barzykin , D. Pines

We present an investigation of magnetic ordering in the two-dimensional S=1/2 quantum magnet Cu(Pz)_2(ClO_4)_2 using specific heat and zero field muon-spin relaxation (\mu^+SR). The magnetic contribution to the specific heat is consistent…

Using inelastic magnetic neutron scattering we have discovered a localized spin resonance at 4.5 meV in the ordered phase of the geometrically frustrated cubic antiferromagnet $\rm ZnCr_2O_4$. The resonance develops abruptly from quantum…

Strongly Correlated Electrons · Physics 2009-10-31 S. -H. Lee , C. Broholm , T. H. Kim , W. Ratcliff , S-W. Cheong

We present a detailed theoretical overview of the thermodynamic properties of the dipolar spin ice model, which has been shown to be an excellent quantitative descriptor of the Ising pyrochlore materials Dy_2Ti_2O_7 and Ho_2Ti_2O_7. We show…

Disordered Systems and Neural Networks · Physics 2015-06-24 Roger G. Melko , Matthew Enjalran , Byron C. den Hertog , Michel. J. P. Gingras

We have characterized spin-squeezed states produced at a temperature of $26^\circ{\mathrm C}$ on a Nuclear Magnetic Resonance (NMR) quadrupolar system. The implementation is carried out in an ensemble of $^{133}$Cs nuclei with spin $I=7/2$…

MgV$_{2}$O$_{4}$ is a spinel based on magnetic V$^{3+}$ ions which host both spin ($S=1$) and orbital ($l_{eff}=1$) moments. Owing to the underlying pyrochlore coordination of the magnetic sites, the spins in MgV$_{2}$O$_{4}$ only…

We show by extensive Monte Carlo simulations that we need a multi-spin interaction in addition to pairwise interactions in order to reproduce the temperature dependence of the experimental magnetization observed in the perovskite compound…

Strongly Correlated Electrons · Physics 2024-02-13 Yethreb Essouda , Hung T. Diep , Mohamed Ellouze

The spin-liquid phase of two highly frustrated pyrochlore magnets Gd2Ti2O7 and Gd2Sn2O7 is probed using electron spin resonance in the temperature range 1.3 - 30 K. The deviation of the absorption line from the paramagnetic position \nu…

Strongly Correlated Electrons · Physics 2013-05-29 S. S. Sosin , L. A. Prozorova , A. I. Smirnov , P. Bonville , G. Jasmin - Le Bras , O. A. Petrenko

We have studied the temperature and magnetic field dependence of the total magnetic moment of large-area permalloy artificial square spin ice arrays. The temperature dependence and hysteresis behavior are consistent with the coherent…

Mesoscale and Nanoscale Physics · Physics 2022-08-17 N. S. Bingham , X. Zhang , J. Ramberger , O. Heinonen , C. Leighton , P. Schiffer

The XY-pyrochlore antiferromagnet \ETO\ is studied by heat capacity measurements and electron spin resonance spectroscopy performed on single crystal samples. The magnetic phase diagrams are established for two directions of applied field,…

Strongly Correlated Electrons · Physics 2015-05-19 S. S. Sosin , L. A. Prozorova , M. R. Lees , G. Balakrishnan , O. A. Petrenko

We report the growth of large high quality crystals of the frustrated magnet, Pr2Zr2O7 by the floating zone technique. Several crystals have been produced starting with varying levels of excess of Pr6O11 to compensate for the loss of Pr2O3…

Materials Science · Physics 2016-11-09 M. Ciomaga Hatnean , C. Decorse , M. R. Lees , O. A. Petrenko , D. S. Keeble , G. Balakrishnan

We have studied the field induced magnetic structures in the spin liquid Tb$_2$Ti$_2$O$_7$, in a wide temperature (0.3$<$$T$$<$270 K) and field (0$<$$H$$<$7 T) range, by single crystal neutron diffraction with $\bf{H}$ // [110] axis. We…

Strongly Correlated Electrons · Physics 2009-11-13 H. Cao , A. Gukasov , I. Mirebeau , P. Bonville , G. Dhalenne
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