Related papers: Cavity-enhanced ultrafast two-dimensional spectros…
Nonlinear optics underpins quantum photonics by enabling the generation and control of quantum states of light. We present new applications of optical resonators as mode selectors in nonlinear processes. First, we show that cavity-enhanced…
Optical spectroscopy and imaging of microscopic samples have opened up a wide range of applications throughout the physical, chemical, and biological sciences. High chemical specificity may be achieved by directly interrogating the…
Mid-infrared microscopy is an important tool for biological analyses, allowing a direct probe of molecular bonds in their low energy landscape. In addition to the label-free extraction of spectroscopic information, the application of…
Optical frequency combs have emerged as a cornerstone for a wide range of areas, including spectroscopy, ranging, optical clocks, time and frequency transfer, waveform synthesis, and communications. However, quantum mechanical fluctuations…
Ultra-fast and multi-dimensional spectroscopy gives a powerful looking glass into the dynamics of molecular systems. In particular two-dimensional electronic spectroscopy (2DES) provides a probe of coherence and the flow of energy within…
Historically, there has been a trade-off in spectroscopic measurements between high spectral resolution, broadband coverage, and acquisition time. Optical frequency combs, initially envisioned for precision spectroscopy of the hydrogen atom…
This paper presents a novel approach to dual-frequency comb generation utilizing a single fiber Fabry-Perot resonator, advancing the implementation of these sources in fiber-based systems. Dual-comb applications such as spectroscopy,…
Photoacoustic spectroscopy (PAS) based gas sensors with high sensitivity, wide dynamic range, low cost, and small footprint are desirable across a broad range of applications in energy, environment, safety, and public health. However, most…
Two-dimensional mass spectrometry (2D MS) is a method for tandem mass spectrometry that enables the correlation between precursor and fragment ions without the need for ion isolation. On a Fourier transform ion cyclotron resonance mass…
Advances in high-resolution laser spectroscopy have enabled many scientific breakthroughs in physics, chemistry, biology and astronomy. Optical frequency combs have pushed measurement limits with ultrahigh-frequency accuracy and…
Frequency combs can be generated in millimeter-sized optical resonators thanks to their ability to store extremely high light intensities and the nonlinearity of their materials. New frequencies are generated through a cascaded parametric…
The generation of shaped laser beams, or structured light, is of interest in a wide range of fields, from microscopy to fundamental physics. There are several ways to make shaped beams, most commonly using spatial light modulators comprised…
This paper presents an analysis of near-resonant, ro-vibrational two-photon spectroscopy and the use of cavity ring-down spectroscopy for its detection. Expressions are derived for the photon absorption rate of a three-level system, correct…
Dual-comb spectroscopy enables broadband analysis of key molecules with unparalleled frequency resolution and exceptional signal-to-noise ratios across various spectral regions. However, fully harnessing its potential for broadband…
Dual-comb spectroscopy is a powerful technique for real-time, broadband optical sampling of molecular spectra which requires no moving components. Recent developments with microresonator-based platforms have enabled frequency combs at the…
Absorption spectroscopy is a widely used technique that permits the detection and characterization of gas species at low concentrations. We propose a sensing strategy combining the advantages of frequency modulation spectroscopy with the…
Ultraviolet spectroscopy provides unique insights into the structure of matter with applications ranging from fundamental tests to photochemistry in the earth's atmosphere and astronomical observations from space telescopes. At longer…
Molecular optomechanical cavities have recently emerged as a promising platform for frequency upconversion, enabling the quantum coherent conversion of infrared signal into the visible range. In a recent work [F. Zou et al., Phys. Rev.…
The phase information provided by the beat note between frequency combs and two continuous-wave lasers is used to extrapolate the phase evolution of comb modes found in a spectral region obtained via nonlinear broadening. This thereafter…
Dual-comb spectroscopy has been proven a powerful tool in molecular characterization, which remains challenging to implement in the mid-infrared region due to difficulties in the realization of two mutually locked comb sources and efficient…