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While being invented for precision measurement of single atomic transitions, frequency combs have also become a versatile tool for broadband spectroscopy in the last years. In this paper we present a novel and simple approach for broadband…

Two frequency combs can be used to measure the full complex response of a sample in a configuration which can be alternatively viewed as the equivalent of a dispersive Fourier transform spectrometer, infrared time domain spectrometer, or a…

Optics · Physics 2015-05-18 I. Coddington , W. C. Swann , N. R. Newbury

Two-dimensional (2D) heterostructures integrated into nanophotonic cavities have emerged as a promising approach towards novel photonic and opto-electronic devices. However, the thickness of the 2D heterostructure has a strong influence on…

Mesoscale and Nanoscale Physics · Physics 2023-08-29 Peirui Ji , Chenjiang Qian , Jonathan J. Finley , Shuming Yang

Optical frequency combs provide equidistant frequency markers in the infrared, visible and ultra-violet and can link an unknown optical frequency to a radio or microwave frequency reference. Since their inception frequency combs have…

Direct optical frequency Comb Spectroscopy (DCS) is proving to be a fundamental tool in many areas of science and technology thanks to its unique performance in terms of ultra-broadband, high-speed detection and frequency accuracy, allowing…

We experimentally demonstrate and theoretically explain the onset of optical frequency combs in a simple cavity-enhanced second-harmonic-generation system, exploiting second-order nonlinear interactions. Two combs are simultaneously…

We show that two-photon transport can be modulated by a two-level emitter coupled to a cavity in a one-dimensional waveguide. In the ordinary case, the transmitted light has a wider frequency spectrum than the situation without the cavity…

Quantum Physics · Physics 2015-05-28 Zhongling Ji , Shaoyan Gao

A laser frequency combs is a broad spectrum composed of equidistant narrow lines. Initially invented for frequency metrology, such combs enable new approaches to spectroscopy over broad spectral bandwidths, of particular relevance to…

Optics · Physics 2019-03-01 Nathalie Picqué , Theodor W. Hänsch

Optical frequency combs have had a remarkable impact on precision spectroscopy. Enabling this technology in the x-ray domain is expected to result in wide-ranging applications, such as stringent tests of astrophysical models and quantum…

We present an experimental study on the cavity-atom ensemble system, and realize the doubly-resonant cavity enhanced electromagnetically induced transparency, where both the probe and control lasers are resonant with a Fabry-Perot cavity.…

We propose a method for efficiently harnessing the quadratic optical response of two-dimensional graphene-like materials by theoretically investigating second harmonic generation from a current biased sheet placed within a planar active…

Optics · Physics 2014-09-24 Alessandro Ciattoni , Carlo Rizza

Dual-comb spectroscopy is emerging as one of the most appealing applications of mid-infrared frequency combs for high-resolution molecular spectroscopy, as it leverages on the unique coherence properties of frequency combs combined with the…

Two-photon excitation spectroscopy with broad spectral span is demonstrated at Doppler-limited resolution. We describe first Fourier transform two-photon spectroscopy of an atomic sample with two mode-locked laser oscillators in a dual-comb…

Infrared spectroscopy in the spectral fingerprint region from 6-12 um accesses the largest molecular absorption cross-sections, permitting sensitive, quantitative and species-specific measurements. Here, we show how dual-comb…

Optics · Physics 2023-06-26 O. Kara , L. Maidment , T. Gardiner , P. G. Schunemann , D. T. Reid

We demonstrate the generation of multi-photon quantum states of light by cavity-enhanced parametric down-conversion in the high-repetition-rate pulsed regime. An external enhancement cavity resonant with the spectral comb of modes of a…

Quantum Physics · Physics 2009-11-13 Alessandro Zavatta , Valentina Parigi , Marco Bellini

Optical frequency combs are utilized in a wide range of optical applications, including atomic clocks, interferometers, and various sensing technologies. They are often generated via four-wave mixing in chip-integrated microring resonators,…

Quantum Physics · Physics 2026-05-04 Patrick Tritschler , Torsten Ohms , André Zimmermann , Peter Degenfeld-Schonburg

Direct comb spectroscopy is a useful tool for obtaining highly accurate spectroscopic information. However, as the number of comb modes is very large and the optical energy is dispersed over them, the optical energy per each comb mode is…

We investigate the prospects of using two-mode intensity squeezed twin-beams, generated in Rb vapor, to improve the sensitivity of spectroscopic measurements by engaging two-photon Raman transitions. As a proof of principle demonstration,…

Atomic Physics · Physics 2021-04-21 Nikunjkumar Prajapati , Ziqi Niu , Irina Novikova

The femtosecond laser frequency comb has enabled the 21st century revolution in optical synthesis and metrology. A particularly compelling technique that relies on the broadband coherence of two laser frequency combs is dual-comb…

Optics · Physics 2023-07-19 Vicente Duran , Santiago Tainta , Victor Torres-Company

Dual-comb spectroscopy has demonstrated remarkable capabilities for rapid and sensitive measurements; however, significant challenges still exist in generating high-power, mutually coherent mid-infrared combs. Here we demonstrate that a…