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We investigate second harmonic (SH) generation in a doubly resonant metamaterial. We show that SH generation can be enhanced when the resonant condition is satisfied for the SH frequency as well as for the fundamental frequency. A unit cell…

High-speed modulation and deterministic control of optical nonlinear processes in nanomaterials are essential for realizing future nanoscale optoelectronic devices. Applying strain is a ubiquitous and versatile approach to deform atomically…

Second harmonic generation (SHG) extensively employs periodically poled nonlinear crystals through forward quasi-phase-matching to achieve efficient frequency conversion. As poling periods approach sub-micrometers, backward…

Optics · Physics 2024-07-15 Fengyan Yang , Juanjuan Lu , Mohan Shen , Guangcanlan Yang , Hong X. Tang

Nonlinear light-matter interactions and their applications are constrained by properties of available materials. The use of metamaterials opens the way to achieve precise control over electromagnetic properties at a microscopic level,…

Other Condensed Matter · Physics 2016-09-19 Dmitry Filonov , Yotam Kramer , Vitali Kozlov , Boris A. Malomed , Pavel Ginzburg

The ability to engineer metamaterials with tunable nonlinear optical properties is crucial for nonlinear optics. Traditionally, metals have been employed to enhance nonlinear optical interactions through field localization. Here, inspired…

We report second-harmonic generation (SHG) from thick hexagonal boron nitride (hBN) flakes with approximately 109-111 layers. The resulting effective second-order susceptibility is similar to previously reported few-layer experiments. This…

The second-order nonlinear optical susceptibility $\Pi^{(2)}$ for second harmonic generation is calculated for gapped graphene. The linear and second-order nonlinear plasmon excitations are investigated in context of second harmonic…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Godfrey Gumbs , Yonatan Abranyos , Upali Aparajita , Oleksiy Roslyak

Highly-tunable coherent light generation is crucial for many important photonic applications. Second-harmonic generation (SHG) is a dominant approach for this purpose, which, however, exhibits a trade-off between the conversion efficiency…

Optics · Physics 2018-04-11 Rui Luo , Yang He , Hanxiao Liang , Mingxiao Li , Qiang Lin

The study of the non-linear response of matter to high electric fields has recently encompassed harmonic generation in solids at near-infrared (NIR) driving wavelengths. Interest has been driven by the prospect of ultrafast signal…

Two dimensional transition metal dichalcogenides exhibit strong excitonic responses, direct bandgaps, and remarkable nonlinear optical properties, making them highly attractive for integrated photonic, optoelectronic, and quantum…

Second Harmonic Generation (SHG) from BiFeO3 nanocrystals is investigated for the first time to determine their potential as biomarkers for multiphoton imaging. Nanocrystals are produced by an auto-combustion method with TRIS as a fuel.…

Spectroscopy of magnetization-induced second-harmonic generation (MSHG) is studied in magnetic Co$_{x}$Ag$_{1-x}$ granular films containing Co nanoparticles. A strong resonance of the magnetic contrast of the second-harmonic generation…

Adaptation and Self-Organizing Systems · Physics 2007-05-23 E. M. Kim , T. V. Murzina , A. F. Kravets , M. Inoue , G. Marowsky , O. A. Aktsipetrov

Supraparticles are coordinated assemblies of discrete nanoscale building blocks into complex and hierarchical colloidal superstructures. Holistic optical responses in such assemblies are not observed in an individual building block or in…

Van der Waals stacking presents new opportunities for nonlinear optics with its remarkable tunability and scalability. However, the fundamental role of interlayer interactions in modifying the overall nonlinear optical susceptibilities…

Materials Science · Physics 2026-03-11 Kanchan Shaikh , Taejun Yoo , Zeyuan Zhu , Qiuyang Li , Amalya C. Johnson , Hui Deng , Fang Liu , Yuki Kobayashi

High quality factor optical microcavities have been employed in a variety of material systems to enhance nonlinear optical interactions. While single-crystalline aluminum nitride microresonators have recently emerged as a low loss platform…

Trigonal selenium and tellurium crystalize in helical chain-like structures and thus possess interesting properties such as current-induced spin polarization, gyrotropic effects and nonlinear optical responses. By performing systematic ab…

Computational Physics · Physics 2019-07-17 Meijuan Cheng , Shunqing Wu , Zi-Zhong Zhu , Guang-Yu Guo

In this paper we present a theoretical examination of second-harmonic generation (SHG) in a graphene monolayer integrated within an attenuated total internal reflection (ATR) configuration. By embedding graphene in this optical setup, we…

High quality factor optical nanostructures provide great opportunity to enhance nonlinear optical processes such as third harmonic generation. However, the field enhancement in these high quality factor structures is typically accompanied…

Optics · Physics 2023-11-22 Claudio U. Hail , Lior Michaeli , Harry A. Atwater

Two-dimensional (2D) materials serve as exceptional platforms for controlled second harmonic generation (SHG), an important nonlinear optical phenomenon with diverse applications. Current approaches to SHG control often depend on…

Mesoscale and Nanoscale Physics · Physics 2024-07-03 Soonyoung Cha , Tianyi Ouyang , Takashi Taniguchi , Kenji Watanabe , Nathaniel M. Gabor , Chun Hung Lui

We report on nonlinear frequency conversion from the telecom range via second harmonic generation (SHG) and third harmonic generation (THG) in suspended gallium nitride slab photonic crystal (PhC) cavities on silicon, under continuous-wave…