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We demonstrate second harmonic generation (SHG) in an $x$-cut congruent lithium niobate (LN) whispering gallery mode resonator. We first show theoretically that independent control of the coupling of the pump and signal modes is optimal for…

We study surface second-harmonic generation (SHG) from a singular plasmonic structure consisting of touching metallic wires. We use the technique of transformation optics and relate the structure to a rather simpler geometry, a slab…

Second-harmonic generation is of paramount importance in several fields of science and technology, including frequency conversion, self-referencing of frequency combs, nonlinear spectroscopy and pulse characterization. Advanced…

Second-order nonlinear optical interactions such as sum- and difference-frequency generation are widely used for bioimaging and as selective probes of interfacial environments. However, inefficient nonlinear optical conversion often leads…

Optics · Physics 2015-05-07 Aaron J. Goodman , William A. Tisdale

We report the fabrication of artificial unidimensional crystals exhibiting an effective bulk second-order nonlinearity. The crystals are created by cycling atomic layer deposition of three dielectric materials such that the resulting…

Raman spectroscopy and Second Harmonic Generation (SHG) are complementary, non-destructive techniques that provide rich and distinct insights into the structural and electronic properties of materials. Raman spectroscopy offers detailed…

Optics · Physics 2026-04-30 Volodymyr Multian , Luigi Bonacina , Jérémie Teyssier

We suggest double-resonant (binary) metamaterials composed of two types of magnetic resonant elements, and demonstrate that in the nonlinear regime such metamaterials provide unique possibilities for phase-matched parametric interaction and…

Optics · Physics 2007-05-23 Maxim V. Gorkunov , Ilya V. Shadrivov , Yuri S. Kivshar

Optical properties of periodic arrays of nanoholes of a triangular shape with experimentally realizable parameters are examined in both linear and nonlinear regimes. Utilizing fully vectorial three-dimensional approach based on the…

Mesoscale and Nanoscale Physics · Physics 2020-03-18 Elena Drobnyh , Maxim Sukharev

Second and third harmonic generation in the opaque region of a GaAs wafer is experimentally observed both in transmission and reflection. These harmonic components can propagate through an opaque material as long as the pump is tuned to a…

Optics · Physics 2019-05-13 L. Rodriguez , J. Trull , M. Scalora , R. Vilaseca , C. Cojocaru

Owing to the discrete frequency spectrum of whispering gallery resonators (WGRs), the resonance and phase-matching conditions for the interacting waves in the case of second-harmonic generation (SHG) cannot generally be fulfilled…

Optics · Physics 2021-04-23 Jan Szabados , Nicolás Amiune , Boris Sturman , Ingo Breunig

We realize and investigate a nonlinear metasurface taking advantage of intersubband transitions in ultranarrow GaN/AlN multi-quantum well heterostructures. Owing to huge band offsets, the structures offer resonant transitions in the telecom…

Metasurfaces represent a new frontier in materials science paving for unprecedented methods of controlling electromagnetic waves, with a range of applications spanning from sensing to imaging and communications. For pulsed terahertz…

We describe an approach based on topology optimization that enables automatic discovery of wavelength-scale photonic structures for achieving high-efficiency second-harmonic generation (SHG). A key distinction from previous formulation and…

Optical second harmonic generation (SHG) has been measured for the first time in reflection from the nanometer-thick films (6 to 40 nm) of the topological insulator Bi2Se3 using 1.51 eV (820 nm) Ti:Sapphire laser photons and revealed a…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 Yuri D. Glinka , Sercan Babakiray , Trent A. Johnson , Mikel B. Holcomb , David Lederman

We present an effective method to generate second harmonic (SH) waves using nonlinear metamaterial composed of coupled split ring resonators (CSRRs) with varactor (variable capacitance) diodes. The CSRR structure has two resonant modes: a…

Optics · Physics 2012-01-30 Toshihiro Nakanishi , Yasuhiro Tamayama , Masao Kitano

Optical frequency conversion processes in nonlinear materials are limited in wavelength by the accessible phase matching and the required high pump powers. In this letter, we report a novel broadband phase matching (PM) technique in high…

Optics · Physics 2013-03-18 Guoping Lin , Josef U. Fürst , Dmitry V. Strekalov , Nan Yu

A new concept for second-harmonic generation (SHG) in an optical nanocircuit is proposed. We demonstrate both theoretically and experimentally that the symmetry of an optical mode alone is sufficient to allow SHG even in centro-symmetric…

We employ transformation optics to optimize the generic nonlinear wave interaction of second-harmonic generation from a pair of touching metallic wires. We demonstrate a 10 orders of magnitude increase in the second-harmonic scattering…

We demonstrate a nonlinear plasmonic metasurface that exhibits strongly asymmetric second-harmonic generation: nonlinear scattering is efficient upon excitation in one direction and it is substantially suppressed when the excitation…

Freed from phase-matching constraints, plasmonic metasurfaces have contributed significantly to the control of the optical nonlinearity and enhancing the nonlinear generation efficiency by engineering subwavelength meta-atoms. However, the…

Optics · Physics 2020-02-11 Basudeb Sain , Cedrik Meier , Thomas Zentgraf
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