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Nuclear spin polarization dynamics are measured in optically pumped individual GaAs/AlGaAs interface quantum dots by detecting the time-dependence of the Overhauser shift in photoluminescence (PL) spectra. Long nuclear polarization decay…

Doping a self-assembled InGaAs/GaAs quantum dot (QD) with a single Mn atom, a magnetic acceptor impurity, provides a quantum system with discrete energy levels and original spin-dependent optical selection rules, which thus has large…

Mesoscale and Nanoscale Physics · Physics 2024-10-28 Jovana Filipovic , Ankit Kundu , Neelesh Kumar Vij , Simon Fécherolle , Aristide Lemaître , Shilpi Gupta , Olivier Krebs

Two electrons in a quantum dot (QD) can form triplet states. We analyze the exchange coupling of the triplet states of the negatively charged exciton in a QD (X$^-$, two electrons and one hole) with the spin of a magnetic atom (Mn). Two…

Mesoscale and Nanoscale Physics · Physics 2023-07-12 L. Besombes , S. Ando , S. Kuroda , H. Boukari

Nuclear spin coherence and relaxation dynamics of all constituent isotopes of an n-doped CdTe/(Cd,Mg)Te quantum well structure are studied employing optically detected nuclear magnetic resonance. Using time-resolved pump-probe Faraday…

Mesoscale and Nanoscale Physics · Physics 2019-04-04 E. Evers , T. Kazimierczuk , F. Mertens , D. R. Yakovlev , G. Karczewski , T. Wojtowicz , J. Kossut , M. Bayer , A. Greilich

The dynamic polarization of nuclear spins by photoexcited electrons is studied in a high quality GaAs/AlGaAs quantum well. We find a surprisingly high efficiency of the spin transfer from the electrons to the nuclei as reflected by a…

Mesoscale and Nanoscale Physics · Physics 2017-11-15 R. W. Mocek , V. L. Korenev , M. Bayer , M. Kotur , R. I. Dzhioev , D. O. Tolmachev , G. Cascio , K. V. Kavokin , D. Suter

We observe dynamic nuclear polarization in a GaAs double dot system using two electrons that are never exchanged with the reservoir. By periodically bringing the system to the mixing point where the singlet and the triplet T+ states are…

Mesoscale and Nanoscale Physics · Physics 2008-01-24 S. Foletti , J. Martin , M. Dolev , D. Mahalu , V. Umansky , A. Yacoby

Circularly polarized optical excitation is used to demonstrate the efficient injection of spin-polarized excitons to individual self-assembled CdSe quantum dots in ZnSe barrier. The exciton spin-transfer is studied by means of…

Mesoscale and Nanoscale Physics · Physics 2014-08-14 T. Smoleński , W. Pacuski , M. Goryca , M. Nawrocki , A. Golnik , P. Kossacki

Highly polarized nuclear spins within a semiconductor quantum dot (QD) induce effective magnetic (Overhauser) fields of up to several Tesla acting on the electron spin or up to a few hundred mT for the hole spin. Recently this has been…

Mesoscale and Nanoscale Physics · Physics 2011-11-04 M. N. Makhonin , K. V. Kavokin , P. Senellart , A. Lema^itre , A. J. Ramsay , M. S. Skolnick , A. I. Tartakovskii

Dynamic nuclear polarisation (DNP) refers to a class of techniques used to increase the signal in nuclear magnetic resonance measurements by transferring spin polarisation from ensembles of highly polarised electrons to target nuclear…

Quantum Physics · Physics 2020-12-24 L. T. Hall , D. A. Broadway , A. Stacey , D. A. Simpson , J-P. Tetienne , L. C. L. Hollenberg

Dynamic nuclear spin polarization (DNP) mediated by paramagnetic point defects in semiconductors is a key resource for both initializing nuclear quantum memories and producing nuclear hyperpolarization. DNP is therefore an important process…

The ability to discriminate between simultaneously occurring noise sources in the local environment of semiconductor InGaAs quantum dots, such as electric and magnetic field fluctuations, is key to understanding their respective dynamics…

Mesoscale and Nanoscale Physics · Physics 2014-11-18 Megan J. Stanley , Clemens Matthiesen , Jack Hansom , Claire Le Gall , Carsten H. H. Schulte , Edmund Clarke , Mete Atatüre

We propose a novel scheme to efficiently polarize and manipulate the electron spin in a quantum dot. This scheme is based on the spin-orbit interaction and it possesses following advantages: (1) The direction and the strength of the spin…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Qing-feng Sun , X. C. Xie

Polarization transfers are crucial building blocks in magnetic resonance experiments, i.e., they can be used to polarize insensitive nuclei and correlate nuclear spins in multidimensional NMR spectroscopy. The polarization can be…

Chemical Physics · Physics 2022-08-24 Zhenfeng Pang , Sheetal Jain , Chen Yang , Xueqian Kong , Kong Ooi Tan

Electron spin coherence has been generated optically in n-type modulation doped (In,Ga)As/GaAs quantum dots (QDs) which contain on average a single electron per dot. The coherence arises from resonant excitation of the QDs by…

The optically induced spin dynamics of a single Mn atom embedded into a single semiconductor quantum dot can be strongly influenced by using the optical Stark effect. The exchange interaction gives rise to simultaneous spin flips between…

Mesoscale and Nanoscale Physics · Physics 2013-05-24 D. E. Reiter , V. M. Axt , T. Kuhn

Dynamic nuclear polarization (DNP) involves a polarization transfer from unpaired electrons to hyperfine coupled nuclei and can increase the sensitivity of nuclear magnetic resonance (NMR) signals by several orders of magnitude. The…

Chemical Physics · Physics 2024-07-16 Gevin von Witte , Sebastian Kozerke , Matthias Ernst

We propose a new mechanism for polarizing nuclear spins in quantum dots, based on periodic modulation of the hyperfine coupling by electric driving at the electron spin resonance frequency. Dynamical nuclear polarization results from…

Mesoscale and Nanoscale Physics · Physics 2008-04-14 M. S. Rudner , L. S. Levitov

The paper reports optical orientation experiments performed in the narrow GaAs/AlGaAs quantum wells doped with Mn. We experimentally demonstrate a control over the spin polarization by means of the optical orientation via the…

Mesoscale and Nanoscale Physics · Physics 2016-09-02 P. V. Petrov , I. A. Kokurin , Yu. L. Ivanov , N. S. Averkiev , R. P. Campion , B. L. Gallagher , P. M. Koenraad , A. Yu. Silov

We theoretically investigate dynamic nuclear spin polarization in a self-assembled quantum dot pumped optically by two laser beams. With the assumption that a noncollinear interaction between the hole spin and nuclear spins leads to nuclear…

Mesoscale and Nanoscale Physics · Physics 2013-06-07 Xiao-Feng Shi

We show here the existence of the indirect coupling of electron and magnetic or nuclear ion spins in self-assembled quantum dots mediated by electron-electron interactions. With a single localized spin placed in the center of the dot, only…

Mesoscale and Nanoscale Physics · Physics 2016-11-25 Udson C. Mendes , Marek Korkusinski , Pawel Hawrylak
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