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Chemically induced dynamic nuclear polarization is a signature of spin order appearing in many photosynthetic reaction centers. Such polarization, significantly enhanced above thermal equilibrium, is known to result from the nuclear spin…

Quantum Physics · Physics 2015-06-12 I. K. Kominis

Dynamic nuclear polarization (DNP) is capable of boosting signals in nuclear magnetic resonance by orders of magnitude by creating out-of-equilibrium nuclear spin polarization. The diffusion of nuclear spin polarization in the vicinity of…

Other Condensed Matter · Physics 2023-07-12 Alessandro Chessari , Samuel F. Cousin , Sami Jannin , Quentin Stern

We demonstrate optical control of the polarization eigenstates of a neutral quantum dot exciton without any external fields. By varying the excitation power of a circularly polarized laser in micro-photoluminescence experiments on…

Several recently proposed implementations of scalable quantum computation rely on the ability to manipulate the spin polarization of individual electrons in semiconductors. The most rapid single-spin-manipulation technique to date relies on…

Quantum Physics · Physics 2016-09-08 C. E. Pryor , M. E. Flatté

We have studied the electron spin coherence in an ensemble of positively charged InAs/GaAs quantum dots. In a transverse magnetic field, we show that two main contributions must be taken into account to explain the damping of the circular…

Materials Science · Physics 2009-11-13 L. Lombez , P. -F. Braun , X. Marie , P. Renucci , B. Urbaszek , T. Amand , O. Krebs , P. Voisin

The coherent electron spin dynamics of an ensemble of singly charged (In,Ga)As/GaAs quantum dots in a transverse magnetic field is driven by periodic optical excitation at 1 GHz repetition frequency. Despite the strong inhomogeneity of the…

Mesoscale and Nanoscale Physics · Physics 2021-04-20 E. Evers , N. E. Kopteva , I. A. Yugova , D. R. Yakovlev , D. Reuter , A. D. Wieck , M. Bayer , A. Greilich

The spin dynamics in a broad range of systems can be studied using circularly polarized optical excitation with alternating helicity. The dependence of spin polarization on the frequency of helicity alternation, known as the spin inertia…

Mesoscale and Nanoscale Physics · Physics 2018-09-19 E. A. Zhukov , E. Kirstein , D. S. Smirnov , D. R. Yakovlev , M. M. Glazov , D. Reuter , A. D. Wieck , M. Bayer , A. Greilich

Asymmetrical horizontal interdot coupling was demonstrated to exist in a system of a single plane of self-assembled CdTe/ZnTe quantum dots. Photoluminescence excitation (PLE), second order photon correlation and optical orientation were…

Other Condensed Matter · Physics 2009-06-12 T. Kazimierczuk , J. Suffczynski , P. Wojnar , A. Golnik , J. A. Gaj , P. Kossacki

Coherent two-level systems, or qubits, based on electron spins in GaAs quantum dots are strongly coupled to the nuclear spins of the host lattice via the hyperfine interaction. Realizing nuclear spin control would likely improve electron…

Mesoscale and Nanoscale Physics · Physics 2010-06-15 D. J. Reilly , J. M. Taylor , J. R. Petta , C. M. Marcus , M. P. Hanson , A. C. Gossard

We present a comprehensive investigation of the electron-nuclear system of negatively charged InGaAs/GaAs self-assembled quantum dots under the influence of weak external magnetic fields (up to 2 mT). We demonstrate that, in contrast to…

Other Condensed Matter · Physics 2015-05-13 T. Auer , R. Oulton , A. Bauschulte , D. R. Yakovlev , M. Bayer , S. Yu. Verbin , R. V. Cherbunin , D. Reuter , A. D. Wieck

A dynamical nuclear polarization scheme is studied in gated double dots. We demonstrate that a small polarization ($\sim 0.5%$) is sufficient to enhance the singlet decay time by two orders of magnitude. This enhancement is attributed to an…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 Guy Ramon , Xuedong Hu

We employ optical pump-probe spectroscopy to investigate the voltage dependence of spontaneous electron and nuclear spin polarizations in hybrid MnAs/n-GaAs and Fe/n-GaAs Schottky diodes. Through the hyperfine interaction, nuclear spin…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 R. J. Epstein , J. Stephens , M. Hanson , Y. Chye , A. C. Gossard , P. M. Petroff , D. D. Awschalom

The effect of electron-nuclear spin interactions on qubit operations is investigated for a qubit represented by the spin of an electron localized in a self-assembled quantum dot. The localized electron wave function is evaluated within the…

Quantum Physics · Physics 2009-11-10 Seungwon Lee , Paul von Allmen , Fabiano Oyafuso , Gerhard Klimeck , K. Birgitta Whaley

The spin-memory effect in the GaAs / InGaAs heterostructures with $\delta$<Mn> layer in GaAs barrier have been investigated. The effect consists in spin polarization of Mn atoms due to interaction with photogenerated spin-polarized holes.…

Carrier-dopant exchange interactions in Mn-doped PbS colloidal quantum dots were studied by circularly polarized magneto-photoluminescence. Mn substitutional doping leads to paramagnetic behavior down to 5 K. While undoped quantum dots show…

Mesoscale and Nanoscale Physics · Physics 2016-10-18 Gen Long , Biplob Barman , Savas Delikanli , Yu Tsung Tsai , Peihong Zhang , Athos Petrou , Hao Zeng

We show that detuned optical pulse trains with a modest spectral width can polarize nuclear spins in InAs quantum dots. The pulse bandwidth is large enough to excite a coherent superposition of both electron spin eigenstates in these…

Quantum Physics · Physics 2015-05-27 S. G. Carter , Sophia E. Economou , A. Shabaev , A. S. Bracker

We report on the coherent dynamics of the spin of an individual magnetic atom coupled to carriers in a semiconductor quantum dot which has been investigated by resonant photoluminescence of the positively charged exciton (X+). We…

Mesoscale and Nanoscale Physics · Physics 2015-09-02 A. Lafuente-Sampietro , H. Boukari , L. Besombes

Dynamic nuclear polarization (DNP) of molecules in a solution at room temperature has potential to revolutionize nuclear magnetic resonance spectroscopy and imaging. The prevalent methods for achieving DNP in solutions are typically most…

Chemical Physics · Physics 2016-03-02 Qiong Chen , Ilai Schwarz , Fedor Jelezko , Alex Retzker , Martin B Plenio

The periodic optical orientation of electron spins in (In,Ga)As/GaAs quantum dots leads to the formation of electron spin precession modes about an external magnetic field which are resonant with the pumping periodicity. As the electron…

Mesoscale and Nanoscale Physics · Physics 2019-08-15 E. Evers , V. V. Belykh , N. E. Kopteva , I. A. Yugova , A. Greilich , D. R. Yakovlev , D. Reuter , A. D. Wieck , M. Bayer

We show that optical pumping of electron spins in individual InGaAs quantum dots leads to strong nuclear polarisation that we measure via the Overhauser shift (OHS) in magneto-photoluminescence experiments between 0 and 4T. We find a…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 P. -F. Braun , B. Urbaszek , T. Amand , X. Marie , O. Krebs , B. Eble , A. Lemaitre , P. Voisin
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