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We study single-photon ionization of aligned H$_2^+$ in low-intensity near-circular laser fields with lower photon energy numerically and analytically. The photoelectron momentum distribution (PMD) within the laser polarization plane,…

Atomic Physics · Physics 2025-05-13 Z. Y. Chen , S. Q. Shen , M. Q. Liu , J. Y. Che , Y. J. Chen

Single-molecule fluorescence spectroscopy is a powerful method that avoids ensemble averaging, but its temporal resolution is limited by the fluorescence lifetime to nanoseconds at most. At the ensemble level, two-dimensional spectroscopy…

Optics · Physics 2024-10-11 Sanchayeeta Jana , Simon Durst , Markus Lippitz

Laser-driven rescattering of electrons is the basis of many strong-field phenomena in atoms and molecules. Here, we will show how this mechanism operates in extended atomic systems, giving rise to effective energy absorption. Rescattering…

Atomic and Molecular Clusters · Physics 2008-04-07 Ulf Saalmann , Jan M. Rost

We propose a photon-recycling dielectric laser accelerator (DLA) system based on silicon photonic device. Our DLA system employs guided electromagnetic waves as a primary energy source, modulated to inject into the electron-light…

Optics · Physics 2025-01-10 Changying Li , Li Zhang , Dingguo Zheng , Xiaoping Liu , Yiming Pan

Photoionization by attosecond (as) extreme ultraviolet (xuv) pulses into the laser-dressed continuum of the ionized atom is commonly described in strong-field approximation (SFA), neglecting the Coulomb interaction between the emitted…

Atomic and Molecular Clusters · Physics 2015-05-20 C. -H. Zhang , U. Thumm

Spectroscopic properties of molecules holds great importance for the description of the molecular response under the effect of an UV/Vis electromagnetic radiation. Computationally expensive ab initio (e.g. MultiConfigurational SCF, Coupled…

An alternative method to the density matrix formalism for the derivation of general expressions of the interaction of polarized atoms with polarized photons and electrons is presented. The expression for the cross-section describing the…

Quantum Physics · Physics 2015-06-26 A. Kupliauskiene

We demonstrate that spin-dependent electron diffraction is possible for a smooth range of transverse electron momenta in a two-photon Bragg scattering scenario of the Kapitza-Dirac effect. Our analysis is rendered possible by introducing a…

Quantum Physics · Physics 2024-01-19 Yang Wang , Sven Ahrens

Diatomic molecules (e.g., O$_2$) in intense laser field exhibit a peculiar suppressed ionization behavior compared to their companion atoms. Several physical models have been proposed to account for this suppression while no consensus has…

Atomic Physics · Physics 2011-11-15 Z. Lin , X. Y. Jia , C. Wang , Z. Hu , H. Kang , W. Quan , X. Y. Lai , X. Liu , J. Chen , B. Zeng , W. Chu , J. P. Yao , Y. Cheng , Z. Z. Xu

The spectra (rotational, rotation-vibrational or electronic) of diatomic molecules due to transitions involving only closed-shell ($^1\Sigma$) electronic states follow very regular, simple patterns and their theoretical analysis is usually…

Chemical Physics · Physics 2016-05-10 Jonathan Tennyson , Lorenzo Lodi , Laura K. McKemmish , Sergei N Yurchenko

Plane-wave electrons undergo momentum transfer as they scatter off a target in overlapping spherical waves. The transferred momentum leads to target structural information to be encoded in angle and energy differential scattering. For…

Atomic and Molecular Clusters · Physics 2024-02-14 Aiswarya R. , Rasheed Shaik , Jobin Jose , Hari R. Varma , Himadri S. Chakraborty

The response of a model micro-electrochemical system to a time-dependent applied voltage is analyzed. The article begins with a fresh historical review including electrochemistry, colloidal science, and microfluidics. The model problem…

Soft Condensed Matter · Physics 2009-11-10 Martin Z. Bazant , Katsuyo Thornton , Armand Ajdari

We study theoretically the dipole radiation of a hydrogen atom driven by an intense sub-cycle pulse. The time-dependent Schr\"odinger equation for the system is solved by ab initio calculation to obtain the dipole response. Remarkably, a…

Atomic Physics · Physics 2016-02-05 Wei-Chun Chu , John C. Travers , Philip St. J. Russell

We investigated the complex index of refraction in the x-ray regime of atoms in laser light. The laser (intensity up to 10^13 W/cm^2, wavelength 800nm) modifies the atomic states but, by assumption, does not excite or ionize the atoms in…

Atomic Physics · Physics 2008-11-18 Christian Buth , Robin Santra

We demonstrate a silicon-based electron accelerator that uses laser optical near fields to both accelerate and confine electrons over extended distances. Two dielectric laser accelerator (DLA) designs were tested, each consisting of two…

During multi-photon ionization of an atom it is well understood how the involved photons transfer their energy to the ion and the photoelectron. However, the transfer of the photon linear momentum is still not fully understood. Here, we…

Atomic Physics · Physics 2020-02-19 Benjamin Willenberg , Jochen Maurer , Benedikt W. Mayer , Ursula Keller

We present a theoretical description of femtosecond laser induced dynamics of the hydrogen molecule and of singly ionised sodium dimers, based on a real-space, real-time, implementation of time-dependent density functional theory (TDDFT).…

Condensed Matter · Physics 2007-05-23 Alberto Castro , M. A. L. Marques , Julio A. Alonso , George F. Bertsch , Angel Rubio

Solving the time-dependent Schr\"odinger equation (TDSE) is pivotal for modeling non-adiabatic electron dynamics, a key process in ultrafast spectroscopy and laser-matter interactions. However, exact solutions to the TDSE remain…

Chemical Physics · Physics 2025-12-29 Bizi Huang , Weizhong Fu , Ji Chen

Upon absorbing a photon, the ionized electron sails through the target force field in attoseconds to reach free space. This navigation probes details of the potential landscape that get imprinted into the phase of the ionization amplitude.…

Atomic Physics · Physics 2024-12-12 Sajad Azizi , Mohamed El-Amine Madjet , Zheng Li , Jan M. Rost , Himadri S. Chakraborty

The screened electron-electron interaction in a multi-band electron system is calculated within the random phase approximation and in the tight-binding representation. The obtained dielectric matrix contains, beside the usual site-site…

Condensed Matter · Physics 2009-10-28 P. Zupanovic , A. Bjelis , S. Barisic