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In this article we address the general approach for calculating dynamical dipole polarizabilities of small quantum systems, based on a sum-over-states formula involving in principle the entire energy spectrum of the system. We complement…

Quantum Physics · Physics 2017-07-10 R. Vexiau , D. Borsalino , M. Lepers , A. Orbán , M. Aymar , O. Dulieu , N. Bouloufa-Maafa

Electron quantum path interferences in strongly laser-driven aligned molecules and their dependence on the molecular alignment is an essential open problem in strong-field molecular physics. Here, we demonstrate an approach which provides…

Based on the work done by an electromagnetic field on an atomic or molecular electronic system, a general gauge invariant formulation of transient absorption spectroscopy is presented within the semi-classical approximation. Avoiding…

The local interaction of charges and light in organic solids is the basis of distinct and fundamental effects. We here observe, at the single molecule scale, how a focused laser beam can locally shift by hundreds-time their natural…

The electron nondipole dynamics in tunneling ionization in an elliptically polarized laser field is investigated theoretically using a relativistic Coulomb-corrected strong-field approximation (SFA) based on the eikonal approximation of the…

Atomic Physics · Physics 2022-07-07 Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

Electron energy-loss spectroscopy (EELS) and cathodoluminescence (CL) are widely used experimental techniques for characterization of nanoparticles. The discrete dipole approximation (DDA) is a numerically exact method for simulating…

Optics · Physics 2023-03-03 Alexander A. Kichigin , Maxim A. Yurkin

We present an experimental and computational study of the nonlinear optical response of conduction electrons to intense terahertz (THz) electric field. Our observations (saturable absorption and an amplitude-dependent group refractive…

Mesoscale and Nanoscale Physics · Physics 2017-03-14 Shukai Yu , Kate H. Heffernan , Diyar Talbayev

We investigate laser-induced nonsequential double ionization from aligned diatomic molecules, using the strong-field approximation in its length and velocity gauge formulations. Throughout, we consider that the first electron dislodges the…

Atomic Physics · Physics 2008-12-10 C. Figueira de Morisson Faria

We analyzed the two-dimensional (2D) electron momentum distributions of high-energy photoelectrons of atoms in an intense laser field using the second-order strong field approximation (SFA2). The SFA2 accounts for the rescattering of the…

Atomic Physics · Physics 2009-11-13 Zhangjin Chen , Toru Morishita , Anh-Thu Le , C. D. Lin

We examine the attosecond electron recollision dissociation of D2+ recently demonstrated experimentally [H. Niikura et al., Nature (London) 421, 826 (2003)] from a coherent control perspective. In this process, a strong laser field incident…

Quantum Physics · Physics 2009-11-13 Michael Spanner , Paul Brumer

Ionization, excitation, and de-excitation to the ground state is studied theoretically for the first excited singlet state B $^1\Sigma_u^+$ of H$_2$ exposed to intense laser fields with photon energies in between about 3 eV and 13 eV. A…

Atomic Physics · Physics 2015-05-18 Manohar Awasthi , Alejandro Saenz

In the presence of a (time-dependent) macroscopic electric field the electron dynamics of dielectrics cannot be described by the time-dependent density only. We present a real-time formalism that has the density and the macroscopic…

Materials Science · Physics 2016-07-27 M. Grüning , D. Sangalli , C. Attaccalite

Short-time filtering of the photoionization amplitude extracted straight from the numerical solution of the time-dependent Schr\"{o}dinger equation (TDSE) is used to identify dominant pathways that form photoelectron spectra in strong…

Atomic Physics · Physics 2020-10-21 V. A. Tulsky , D. Bauer

We study the generation of terahertz radiation from atoms and molecules driven by an ultrashort fundamental laser and its second harmonic field by solving time-dependent Schr\"odinger equation (TDSE). The comparisons between one-, two-, and…

Electrometry near a dielectric surface is performed using Rydberg electromagnetically induced transparency (EIT). The large polarizability of high n-state Rydberg atoms gives this method extreme sensitivity. We show that adsorbates on the…

Atomic Physics · Physics 2015-05-28 R. P. Abel , C. Carr , U. Krohn , C. S. Adams

We present a simple diode laser-based photoionization scheme for generating electrons and ions with well-defined spatial and energetic (<2 eV) structures. This scheme can easily be implemented into ion or electron imaging spectrometers for…

Instrumentation and Detectors · Physics 2017-07-24 A. Wituschek , J. von Vangerow , J. Grzesiak , F. Stienkemeier , M. Mudrich

We present a simple exact analytical solution, using the Weyl-Titchmarsh-Kodaira spectral theorem, for the spectral function of the one-dimensional diatomic molecule model consisting of two attractive delta function wells in the presence of…

Atomic Physics · Physics 2007-05-23 Gerald V. Dunne , Christopher S. Gauthier

The ionization of an atom by a high-frequency intense laser pulse, where the energy of a single-photon is sufficient to ionize the system, is investigated from first principles. It is shown that as a consequence of an AC Stark effect in the…

Atomic Physics · Physics 2012-06-26 Philipp V Demekhin , Lorenz S Cederbaum

Analytical solution for optical trapping force on a spherical dielectric particle for an arbitrary positioned focused beam is presented in a generalized Lorenz-Mie and vectorial diffraction theory. In this case the exact electromagnetic…

Present photoionization experiments cannot measure molecular frame photoelectron angular distributions (MFPAD) from the outermost valence electrons of molecules. We show that details of the MFPAD can be retrieved with high-order harmonics…

Atomic Physics · Physics 2009-05-24 Anh-Thu Le , R. R. Lucchese , M. T. Lee , C. D. Lin
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