Related papers: Towards controlling the dissociation probability b…
Ab initio modeling of conical intersection dynamics is crucial for various photochemical, photophysical, and biological processes. However, adiabatic electronic states obtained from electronic structure computations involve random phases,…
The coupling of matter to the quantized electromagnetic field of a plasmonic or optical cavity can be harnessed to modify and control chemical and physical properties of molecules. In optical cavities, a term known as the dipole self-energy…
We demonstrate that ultrashort pulses carry the possibility for a new regime of light-matter interaction with nonadiabatic electron processes sensitive to the envelope-derivative of the light pulse. A standard single pulse with its two…
Strongly magnetizing a plasma adds a range of waves that do not exist in unmagnetized plasmas and enlarges the laser-plasma interaction (LPI) landscape. In this paper, we use particle-in-cell (PIC) simulations to investigate strongly…
To exploit the high intensity of laser radiation, we propose to select frequencies at which single-photon absorption is of too low energy and two or more photons are needed to produce states of an atom that can undergo interatomic Coulombic…
The photoionization of a helium atom by short intense laser pulses is studied theoretically in the vicinity of the $2s2p\,^1P$ doubly-excited state with the intention to investigate the impact of the intensity and duration of the exciting…
A new method to coherently control the electron dynamics is proposed using a few-cycle laser pulse in combination with a controlling field. It is shown that this method not only broadens the attosecond pulse bandwidth, but also reduces the…
An ab initio simulation of strong-field photodissociation of diatomic molecules was developed, inspired by recent dissociation experiments of F2-. The transition between electronic states was modeled, including the laser pulse and…
Direct laser acceleration of ions by short frequency-chirped laser pulses is investigated theoretically. We demonstrate that intense beams of ions with a kinetic energy broadening of about 1 % can be generated. The chirping of the laser…
The ionization of a hydrogen-like heavy ion by impact of a charged projectile under simultaneous irradiation by a short laser pulse is investigated within the non-perturbative approach, based on numerical solutions of the time-dependent…
The interaction of chirped femtosecond laser pulses with hybrid materials - materials comprised of plasmon sustaining structures and resonant molecules - is scrutinized using a self-consistent model of coupled Maxwell-Bloch equations. The…
Using numerical simulations of two-photon electronic absorption with femtosecond pulses in Na$_2$ we show that: i) it is possible to avoid the characteristic saturation or dumped Rabi oscillations in the yield of absorption by time-delaying…
Here, upon systematic studies of femtosecond-laser processing of monocrystalline Si in oxidation-preventing methanol, we showed that the electromagnetic processes dominating at initial steps of the progressive morphology evolution define…
Accessing coherences is key to fully understand and control ultrafast dynamics of complex quantum systems like molecules. Most photochemical processes are mediated by conical intersections (CIs), which generate coherences between electronic…
The limit of decreasing laser frequency can not be considered independently from nondipole effects due to increase in the laser-induced continuum electron speed in this limit. Therefore, in this work, tunneling ionization in the adiabatic…
Using a 3D Finite-Difference Time-Domain parallel code, we report on the linear and nonlinear propagation of light pulses in a disordered assembly of scatterers, whose spatial distribution is generated by a Molecular Dynamics code;…
Conical intersections are ubiquitous in chemistry and physics, often governing processes such as light harvesting, vision, photocatalysis, and chemical reactivity. They act as funnels between electronic states of molecules, allowing rapid…
We propose a mechanism to achieve the group velocity control of bifurcation light via an imaginary coupling effect in the non-reciprocal lattice. The physical model is composed of two-layer photonic lattices with non-reciprocal coupling in…
We investigate the shift caused by asymmetry of spectroscopic lineshape in atomic interferometers, which has not previously been discussed in the scientific literature. This asymmetry arises because laser field is frequency-chirped not only…
Electrostatic two-stream instabilities play essential roles in an electrostatic collisionless shock formation. They are a key dissipation mechanism and result in ion heating and acceleration. Since the number and energy of the…