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Studying the primary {\alpha}- and secondary {\beta}-relaxation process has contributed significantly to the understanding of the structure and rheology of metallic glasses. In this letter, we report on a third relaxation mechanism…

Materials Science · Physics 2017-03-28 Stefan Küchemann , Robert Maaß

A new relaxation mechanism is shown to arise from overdamped two-level systems above a critical temperature $T^*\approx 5$ K, thus yielding an explanation for experimental observations in dielectric glasses in the temperature range between…

Condensed Matter · Physics 2009-10-22 Peter Neu , Alois Würger

We report the experimental investigations on a liquid crystal comprised of thiophene-based achiral bent-core banana shaped molecules. The results reveal the presence of a short range nematic phase at high temperatures and a long-range SmA…

Soft Condensed Matter · Physics 2023-07-03 Vishnu Deo Mishra , G. Pratap , Arun Roy

In the present work, a detailed analysis of the glassy behavior and the relaxation dynamics of the liquid crystal dimer {\alpha}-(4-cyanobiphenyl-4'-yloxy)-{\omega}-(1-pyrenimine-benzylidene-4'-oxy) heptane (CBO7O.Py) throughout both…

Soft Condensed Matter · Physics 2018-10-02 David O. López , Josep Salud , María Rosario de la Fuente , Nerea Sebastián , Sergio Diez-Berart

Analysis of temperature dependence of structural relaxation time in supercooled liquids revealed a qualitatively distinct feature - a sharp, cusp-like maxumum in the second derivative of its logarithm. It suggests that the super-Arrhenius…

Soft Condensed Matter · Physics 2016-01-20 V. N. Novikov , A. P. Sokolov

In an earlier preprint (V. V. Ginzburg, O. V. Gendelman, R. Casalini, and A. Zaccone, arxiv:2409.17291), we demonstrated that the dynamic (relaxation time) and volume equations of state for many amorphous polymers are near-universal -- each…

Soft Condensed Matter · Physics 2025-01-03 Valeriy V. Ginzburg , Oleg V. Gendelman , Riccardo Casalini , Alessio Zaccone

Amorphous metallic foams are prospective materials due to unique combination of their mechanical and energy-absorption properties. In the present work, atomistic dynamics simulations are performed under isobaric conditions with the pressure…

Materials Science · Physics 2020-05-22 Bulat N. Galimzyanov , Anatolii V. Mokshin

Dielectric study over a broadband was carried out from 10 to 70 K on ceramic Gd1-xYxMnO3 (x= 0.2, 0.3, and 0.4). For all the compositions, a prominent sharp peak about ~18K was observed in the temperature dependence of both {\epsilon}'(T)…

Materials Science · Physics 2017-06-28 R. M. Sarguna , V. Sridahran , A. M. Awasthi , N. Subramanian

Dielectric measurements on molecular liquids just above the glass transition indicate that alpha relaxation is characterized by a generic high-frequency loss varying as $\omega^{-1/2}$, whereas deviations from this come from one or more…

Soft Condensed Matter · Physics 2009-11-11 Jeppe C. Dyre

This review deals with the kinetic and thermodynamic fragility of bulk metallic glass forming liquids. The experimental methods to determine the kinetic fragility, relaxation behavior and thermodynamic functions of undercooled metallic…

Materials Science · Physics 2014-05-12 Ralf Busch , Zach Evenson , Isabella Gallino , Shuai Wei

The glass transition temperature and relaxation dynamics of the segmental motions of thin films of polystyrene labeled with a dye, 4-[N-ethyl-N-(hydroxyethyl)]amino-4-nitraozobenzene (Disperse Red 1, DR1) are investigated using dielectric…

Soft Condensed Matter · Physics 2009-11-13 Rodney D. Priestley , Linda J. Broadbelt , John M. Torkelson , Koji Fukao

Recent experiments and computer simulations show that supercooled liquids around the glass transition temperature are "dynamically heterogeneous" [1]. Such heterogeneity is expected from the random first order transition theory of the glass…

Disordered Systems and Neural Networks · Physics 2009-10-31 Xiaoyu Xia , Peter G. Wolynes

We presented that the relaxation of n coupling molecules in a molecular string exhibits n individual relaxation modes (RMs), each mode being characterized by a definite relaxation time and amplitude according to the string model. The n RMs…

Disordered Systems and Neural Networks · Physics 2008-02-29 Y. N Huang , J. L. Zhang , L. L. Zhang , L. N. Wang

A wide range of glassy and disordered materials exhibit complex, non-exponential, structural relaxation (aging). We propose a simple nonlinear rate equation d\delta/dt = a [1-exp (b\delta)], where '\delta' is the normalized deviation of a…

Disordered Systems and Neural Networks · Physics 2012-07-31 Itamar Kolvin , Eran Bouchbinder

Glass sound velocity shift was observed to be longarithmically temperature dependent in both relaxation and resonance regimes: $\Delta c/c=\mathcal{C}\ln T$. It does not monotonically increase with temperature from $T=0$K, but to reach a…

Disordered Systems and Neural Networks · Physics 2016-08-12 Di Zhou

As a nontrivial solid state of matter, the glassy-crystal state embraces physical features of both crystalline and amorphous solids, where a long-range ordered periodic structure formed by the mass centers of constituent molecules…

The primary relaxation in glass forming supercooled liquids (SCLs) above the glass transformation temperature T_g is discussed in terms of the first-order (steepness) and the second-order (curvature) temperature derivatives of the observed…

Chemical Physics · Physics 2007-05-23 Valery B. Kokshenev , Pablo D. Borges , Neil S. Sullivan

Non-equilibrium charge dynamics, such as cooling-rate-dependent charge vitrification and physical aging, have been demonstrated for a charge-cluster glass in $\theta$-(BEDT-TTF)$_2$CsZn(SCN)$_4$ using electron transport measurements. The…

Strongly Correlated Electrons · Physics 2014-03-17 T. Sato , F. Kagawa , K. Kobayashi , K. Miyagawa , K. Kanoda , R. Kumai , Y. Murakami , Y. Tokura

We discuss the microscopic mechanisms by which low-temperature amorphous states, such as ultrastable glasses, transform into equilibrium fluids, after a sudden temperature increase. Experiments suggest that this process is similar to the…

Statistical Mechanics · Physics 2016-07-05 Robert L. Jack , Ludovic Berthier

Glasses encode the memory of any thermo-mechanical treatment applied to them. This ability is associated to the existence of a myriad of metastable amorphous states which can be probed through different experimental pathways. It is usually…