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Employing small angle X-ray scattering (SAXS), we explore the conditions under which the assembly of gold nanoparticles (AuNPs) grafted with the thermo-sensitive polymer Poly(N-isopropylacrylamide) (PNIPAM) emerges. We find that short-range…

Soft Condensed Matter · Physics 2023-12-08 Binay P. Nayak , Hyeong Jin Kim , Srikanth Nayak , Wenjie Wang , Wei Bu , Surya K. Mallapragada , David Vaknin

Structure formation in non-equilibrium steady state conditions is poorly understood. Non-equilibrium steady state can be achieved in a system by maintaining temperature gradient. A class of cross-linked micro-gel particles,…

Soft Condensed Matter · Physics 2023-08-02 Rahul Karmakar , Jaydeb Chakrabarti

The selective solute partitioning within a polymeric network is of key importance to applications in which controlled release or uptake of solutes in a responsive hydrogel is required. In this work we investigate the impact of cross-links…

Soft Condensed Matter · Physics 2019-04-05 Sebastian Milster , Richard Chudoba , Matej Kanduč , Joachim Dzubiella

The encapsulation of fragile biomacromolecules is crucial for many biotechnological applications but remains challenging. Interfacial complexation (IC) in water-in-oil emulsions turned out to be an efficient process for the formation of…

Soft Condensed Matter · Physics 2021-09-30 L. Sixdenier , C. Tribet , E. Marie

Recent experiments have demonstrated that the glass transition temperature of thin polymer films can be shifted as compared to the same polymer in the bulk, the amplitude and the sign of this effect depending on the interaction between the…

Statistical Mechanics · Physics 2007-05-23 D. Long , P. Sotta

The combination of the catechol-containing co-monomer dopamine methacrylamide (DMA) with stimuli-responsive microgels such as poly(N-isopropylacrylamide) (PNIPAM) bears a huge potential in research and for applications due to the versatile…

Soft Condensed Matter · Physics 2023-09-29 Sandra Forg , Xuhong Guo , Regine von Klitzing

Confinement breaks the translational symmetry of materials. Such symmetry breaking can be used to obtain configurations that are not otherwise accessible in the bulk. Here, we explore the effect of substrate-liquid interactions on the…

Statistical Mechanics · Physics 2015-12-03 Amir Haji-Akbari , Pablo G. Debenedetti

The electronic properties of superconducting Sn films ($T_c \approx$ 3.8 K) change significantly when reducing the film thickness down to a few nm, in particular close to the percolation threshold. The low-energy electrodynamics of such Sn…

The present paper report is focused toward the preparation of the flexible and freestanding blend solid polymer electrolyte films based on PEO-PVP complexed with NaPF6 by solution cast technique. The structural/morphological features of the…

Materials Science · Physics 2018-07-12 Anil Arya , A. L. Sharma*

Microgels are soft colloids that, in virtue of their polymeric nature, can react to external stimuli such as temperature or pH by changing their size. The resulting swelling/deswelling transition can be exploited in fundamental research as…

Soft Condensed Matter · Physics 2019-02-15 Lorenzo Rovigatti , Nicoletta Gnan , Emanuela Zaccarelli

Thin films made of deformable micro- and nano-units, such as biological membranes, polymer interfaces, and particle-laden liquid surfaces, exhibit a complex behavior during drying, with consequences for various applications like wound…

We explore the impact of three water-soluble polyelectrolytes (PEs) on the flow of concentrated suspensions of poly(N-isopropylacrylamide) (PNIPAm) microgels with thermoresponsive anionic charge density. By progressively adding the PEs to a…

Soft Condensed Matter · Physics 2023-05-23 Rajam Elancheliyan , Edouard Chauveau , Domenico Truzzolillo

The reconfiguration of soft, deformable particles upon adsorption at the interface between two fluids underpins many aspects of their dynamics and interactions, ultimately controlling the macroscopic properties of particle monolayers of…

Soft Condensed Matter · Physics 2022-04-21 Jacopo Vialetto , Shivaprakash N. Ramakrishna , Lucio Isa

We report on the poroelastic indentation response of hydrogel thin films geometrically confined within contacts with rigid spherical probes of radii in the millimeter range. Poly(PEGMA) (poly(ethylene glycol)) methyl ether methacrylate),…

Soft Condensed Matter · Physics 2017-08-28 Jessica Delavoipière , Emilie Verneuil , Yvette Tran , A. Chateauminois

Polyimide (PI) thin films are widely used in advanced technologies, yet accurate characterization of their thermal properties remains challenging, as evidenced by significant inconsistencies in reported data and an incomplete understanding…

Applied Physics · Physics 2026-04-15 Bingjiang Zhang , Dihui Wang , Tao Chen , Heng Ban , Puqing Jiang

Heat management in devices is a key to their efficiency and longevity. Here, thermal switches (TS) are of great importance because of their ability to transition between different thermal conductivity $\kappa$ states. While traditional TS…

Soft Condensed Matter · Physics 2024-10-23 Mokter M. Chowdhury , Robinson Cortes-Huerto , Debashish Mukherji

Nanoscale polymeric thin films are widely used in diverse applications such as energy devices, flexible electronics and biosensors, where a satisfactory mechanical performance is of vital importance to realize their full functionality. It…

Soft Condensed Matter · Physics 2022-06-29 Zhengyang Zhang , Pei Bai , Yuhan Xiao , Yunlong Guo , Yanming Wang

Diffusion mediated interaction in metal-substrate assembly during high temperature annealing leads to possible formation of new composite materials. Here, sputtered grown Ti films on Si3N4/Si substrate has been reported to produce titanium…

Materials Science · Physics 2020-11-19 Sachin Yadav , Sangeeta Sahoo

We report on the frictional properties of thin ($\approx \mu m$) poly(dimethylacrylamide) hydrogel films within contacts with spherical silica probes. In order to focus on the contribution to friction of interfacial dissipation, a dedicated…

Soft Condensed Matter · Physics 2024-12-10 Lola Ciapa , Ludovic Olanier , Yvette Tran , Christian Frétigny , Antoine Chateauminois , Emilie Verneuil

Thermoresponsive poly(N-isopropylacrylamide) (PNIPAM) particles of a nearly constant swelling ratio and with polydispersity indices (PDIs) varying over a wide range (7.4% - 48.9%) are synthesized to study the effects of polydispersity on…

Soft Condensed Matter · Physics 2017-11-01 Sanjay Kumar Behera , Debasish Saha , Paramesh Gadige , Ranjini Bandyopadhyay