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We have studied the chemisorption processes of O2 on the (100) surface of uranium using generalized gradient approximation to density functional theory. Dissociative adsorptions of O2 are significantly favored compared to molecular…

Strongly Correlated Electrons · Physics 2015-06-24 M. N. Huda , A. K. Ray

Atomic oxygen adsorption on the Mo(112) surface has been investigated by means of first-principles total energy calculations. Among the variety of possible adsorption sites it was found that the bridge sites between two Mo atoms of the…

Materials Science · Physics 2007-05-23 Adam Kiejna , R. M. Nieminen

Dispersion corrected density functional theory ($\omega$B97X-D DFT) method is used to study the molecular hydrogen adsorption in $Ni_nMg_m$ $(1\geq n\geq 3,1\geq m\geq9)$ clusters. All these clusters can effectively adsorb multiple $H_2$ in…

Materials Science · Physics 2022-02-28 Bishwajit Boruah , Bulumoni Kalita

Oxygen molecule adsorptions on a Pu (100) surface have been studied in detail, using the generalized gradient approximation to density functional theory. Dissociative adsorption with a layer by layer alternate spin arrangement of the…

Materials Science · Physics 2009-11-10 M. N. Huda , A. K. Ray

Oxygen adsorption on delta-Pu (100) and (111) surfaces have been studied at both non-spin-polarized and spin-polarized levels using the generalized gradient approximation of density functional theory (GGA-DFT)with Perdew and Wang…

Strongly Correlated Electrons · Physics 2009-11-10 M. N. Huda , A. K. Ray

We report on the structure and adsorption properties of Pd$_n$ ($n=1-4$) clusters supported on the rutile TiO$_2$ (110) surfaces with the possible presence of a surface oxygen vacancy or a subsurface Ti-interstitial atom. As predicted by…

Materials Science · Physics 2012-04-12 Jin Zhang , Anastassia N. Alexandrova

Density functional theory $(DFT)$ studies show that doping of $3d TM$ atoms into $Mg_4^{0,+} (TMMg_3^{0,+})$ can alter the endothermic nature of molecular hydrogen adsorption on bare $Mg_4^{0,+}$. $H_2$ adsorption on $TMMg_3^{0,+}$ clusters…

Materials Science · Physics 2021-12-21 Bishwajit Boruah , Bulumoni Kalita

Adsorption of carbon, nitrogen, and oxygen on the (111) surface of delta-Plutonium has been studied within the framework of density functional theory using the full-potential linear augmented plane wave plus local basis (FP-LAPW+lo) method.…

Strongly Correlated Electrons · Physics 2007-10-29 Raymond Atta-Fynn , Asok K. Ray

We study the atomic oxygen adsorption on Pb(111) surface by using density-functional theory within the generalized gradient approximation and a supercell approach. The atomic and energetic properties of purely on-surface and subsurface…

Materials Science · Physics 2009-11-13 Bo Sun , Ping Zhang , Zhigang Wang , Suqing Duan , Xian-Geng Zhao , Xuchun Ma , Qi-Kun Xue

Unraveling the adsorption mechanism and thermodynamics of O$_2$ and H$_2$O on uranium dioxide surfaces is critical for the nuclear fuel storage and uranium corrosion. Based on the first-principles DFT+U-D3 calculations, we carefully test…

Materials Science · Physics 2025-02-13 Yang Huang , Le Zhang , Hefei Ji , Zhipeng Zhang , Qili Zhang , Bo Sun , Haifeng Liu , Haifeng Song

An ab initio density functional study was performed investigating the adsorption of CO$_2$ on the neutral boron B$_{n}$ ($n = 10-13$) clusters, characterized by planar and quasiplanar ground-state atomic structures. For all four clusters,…

The adsorption and dissociation of H$_2$, O$_2$, and H$_2$O on Ni-Fe alloys with variable Fe:Ni ratio are studied by means of Density Functional Theory calculations. The alloy composition deeply influences the thermochemistry of the…

Materials Science · Physics 2024-10-28 Changyuan Li , Sergio Tosoni

Oxygen adsorption onto Ru (10 bar 1 0) results in the formation of two ordered overlayers, i.e. a c(2 times 4)-2O and a (2 times 1)pg-2O phase, which were analyzed by low-energy electron diffraction (LEED) and density functional theory…

Ab initio self-consistent total energy calculations using second order Moller-Plesset perturbation theory and Hay-Wadt effective core potentials for gallium and arsenic have been used to investigate the chemisorption of atomic oxygen on the…

Condensed Matter · Physics 2007-05-23 Michael L. Mayo , Asok K. Ray

We have performed systematic large-scale all-electron correlated calculations on boron Bn, aluminum Aln and magnesium Mgn clusters (n=2--5), to study their linear optical absorption spectra. Several possible isomers of each cluster were…

Atomic and Molecular Clusters · Physics 2016-07-26 Ravindra Shinde

The urgent need to mitigate rising atmospheric CO2 levels motivates the search for stable, efficient, and tunable adsorbent materials. In this study, we employ first-principles density functional theory to investigate the adsorption of CO2…

Materials Science · Physics 2026-02-16 Jakkapat Seeyangnok , Rungkiat Nganglumpoon , Joongjai Panpranot , Udomsilp Pinsook

The precise understanding of adsorption energetics and molecular geometry at catalytic sites is fundamental for advancing catalysis, particularly under the constraints of resource efficiency and environmental sustainability. This study…

Materials Science · Physics 2025-12-16 Jeonghwan Ahn , Iuegyun Hong , Gwangyoung Lee , Hyeondeok Shin , Anouar Benali , Yongkyung Kwon

The adsorption of MgO molecules on a Fe(001) surface was studied using density functional theory (DFT) and projector augmented wave methods. The energetically most favored configurations for different adsorption sites considered were…

Materials Science · Physics 2015-12-10 D. Wiśnios , A. Kiejna , J. Korecki

The adsorption of carbon monoxide on neutral iridium clusters in the size range of n = 3 to 21 atoms is investigated with infrared multiple photon dissociation spectroscopy. For each cluster size only a single v(CO) band is present with…

Chemical Physics · Physics 2011-10-05 Christian Kerpal , Daniel J. Harding , Gerard Meijer , André Fielicke

The adsorption of $CO_2$ on the $Fe_3$$O_4$(001)-($\sqrt{2}$ $\times$ $\sqrt{2}$)R45{\deg} surface was studied experimentally using temperature programmed desorption (TPD), electron spectroscopies (UPS and XPS), and scanning tunneling…

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