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Novel nonlinear optical phenomena - photonic flame effect (PFE) and stimulated globular scattering (SGS) are discussed.PFE consisted in the appearance of the few seconds duration emission in blue-green spectral range under 20 ns ruby laser…

Optics · Physics 2009-11-13 A. Esakov , V. Gorelik , A. Kudryavtseva , N. Tcherniega

A laser-Compton backscattering beam, which we call a `Laser-Electron Photon' beam, was upgraded at the LEPS beamline of SPring-8. We accomplished the gains in backscattered photon beam intensities by factors of 1.5--1.8 with the injection…

Lattices of odd-layered two-dimensional (2D) transition metal dichalcogenides (TMDs) such as WSe2 are non-centrosymmetric, and thus could possess linear piezoelectricity that is attractive for applications such as nanoelectromechanical…

Materials Science · Physics 2018-08-10 Ehsan Nasr Esfahani , Terrance Li , Bevin Huang , Xiaodong Xu , Jiangyu Li

Improving the efficiency of photothermal (PT) therapies and photoacoustic (PA) imaging at the microscopic scale hinges on developing multiphoton-absorbing photothermal molecules or contrast agents that operate in the near-infrared (NIR)…

We demonstrate effective background-free continuous wave nonlinear optical excitation of molecules that are sandwiched between asymmetrically constructed plasmonic gold nanoparticle clusters. We observe that near infrared photons are…

Random scattering is usually viewed as a serious nuisance in optical imaging, and needs to be prevented in the conventional imaging scheme based on single-photon interference. Here we proposed a two-photon imaging scheme with the widely…

Optics · Physics 2018-09-25 Peilong Hong

Nonlinear interferometry with entangled photons allows for characterizing a sample without detecting the photons interacting with it. This method enables highly sensitive optical sensing in the wavelength regions where efficient detectors…

Optics · Physics 2025-08-11 Kazuki Hashimoto , Dmitri B. Horoshko , Maria V. Chekhova

We report the first observation of multi-photon photoluminescence excitation (PLE) below the resonant energies of nitrogen vacancy (NV) centers in diamond. The quadratic and cubic dependence of the integrated fluorescence intensity as a…

Materials Science · Physics 2018-04-25 Peng Ji , Ryan B. Balili , Jonathan Beaumariage , Shouvik Mukherjee , David W. Snoke , Gurudev Dutt

We recently demonstrated orders of magnitude enhancement of two-photon absorption (2PA) in direct gap semiconductors due to intermediate state resonance enhancement for photons of very different energies. It can be expected that further…

The dynamics of polarized fluorescence in NADH at 460 nm under two-photon excitation at 720 nm by femtosecond laser pulses in water-methanol solutions has been studied experimentally and theoretically as a function of methanol…

Imaging in thick biological tissues is often degraded by sample-induced aberrations, which reduce image quality and resolution, particularly in super-resolution techniques. While hardware-based adaptive optics, which correct aberrations…

We report the application of fifth order nonlinear optical processes for multiphoton microscopy, including fifth harmonic and 5-photon excitation fluorescence. This novel imaging modality has been characterized with spectral and power…

Optical imaging deep inside scattering media remains a fundamental problem in bio-imaging. While wavefront shaping has been shown to allow focusing of coherent light at depth, achieving it non-invasively remains a challenge. Various…

Optics · Physics 2019-12-24 Antoine Boniface , Baptiste Blochet , Jonathan Dong , Sylvain Gigan

ZnTe/CdSe/(Zn,Mg)Te core/double-shell nanowires are grown by molecular beam epitaxy by employing the vapor-liquid-solid growth mechanism assisted with gold catalysts. A photoluminescence study of these structures reveals the presence of an…

Two-dimensional (2D) fluorescence-excitation (2D-FLEX) spectroscopy is a recently proposed nonlinear femtosecond technique for the detection of photoinduced dynamics. The method records a time-resolved fluorescence signal in its excitation-…

Chemical Physics · Physics 2024-06-24 Sebastian V. Pios , Maxim F. Gelin , Luis Vasquez , Jürgen Hauer , Lipeng Chen

High-numerical-aperture (NA) oblique plane microscopy enables noninvasive fluorescence imaging of subcellular dynamics without requiring radical sample modification. However, performance degrades at depth in multicellular specimens as…

Nonlinear processes can offer pathways to next-generation sensors and frequency mixing devices to overcome modern imaging, detection, and communication challenges. In this article, we report on strong second and third-order nonlinear…

Two-dimensional ferroelectrics have recently emerged as a promising avenue for next-generation optoelectronic and photovoltaic devices. Due to the intrinsic absence of inversion symmetry, 2D ferroelectrics exhibit bulk photovoltaic effect…

Materials Science · Physics 2025-12-08 Francesco Delodovici , Brahim Dkhil , Charles Paillard

We closely replicated and extended a recent experiment ("Spatial properties of entangled two-photon absorption," Phys. Rev. Lett. 129, 183601, 2022) that reportedly observed enhancement of two-photon absorption rates in molecular samples by…

Quantum Physics · Physics 2024-04-26 Tiemo Landes , Brian J. Smith , Michael G. Raymer

We study the isomer-specific photoionization and photofragmentation of 1,2- dibromoethene (DBE) under strong-field fs-laser irradiation in the gas phase complementing previous studies utilising ns- and ps-laser excitation. Our findings are…

Chemical Physics · Physics 2025-04-30 A. Mishra , J. Kim , S. K. Kim , S. Willitsch
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