Related papers: Optical frequency comb spectroscopy at 3-5.4 {\mu}…
Improving spectral acquisition rate of broadband mid-infrared spectroscopy promises further advancements of molecular science and technology. Unlike the pump-probe spectroscopy that requires repeated measurements with different pump-probe…
Ultraviolet spectroscopy provides unique insights into the structure of matter with applications ranging from fundamental tests to photochemistry in the earth's atmosphere and astronomical observations from space telescopes. At longer…
We present an experimental study of optical frequency comb generation based on cascaded quadratic nonlinearities inside a continuous-wave-pumped optical parametric oscillator. We demonstrate comb states which produce narrow-linewidth…
Powerful and efficient optical frequency combs in the mid-infrared (MIR) spectral region are highly desirable for a broad range of applications. Despite extensive efforts utilizing various techniques, MIR frequency comb sources are still…
We present a simple method for fully-stabilized mid-infrared optical frequency comb generation based on single-pass femtosecond optical parametric generation that is seeded by a continuous-wave laser. We have implemented the method in a…
Over the last two decades, frequency combs have brought breakthroughs in length metrology with traceability to length standards. In particular, frequency-comb-based spectral interferometry is regarded as a promising technology for…
Two-photon excitation spectroscopy with broad spectral span is demonstrated at Doppler-limited resolution. We describe first Fourier transform two-photon spectroscopy of an atomic sample with two mode-locked laser oscillators in a dual-comb…
Accurate parameters of molecular hot-band transitions, i.e., those starting from vibrationally excited levels, are needed to accurately model high-temperature spectra in astrophysics and combustion, yet laboratory spectra measured at high…
We developed a novel technique for frequency measurement and synthesis, based on the operation of a femtosecond comb generator as transfer oscillator. The technique can be used to measure frequency ratios of any optical signals throughout…
Reducing the pulse repetition rate of an optical frequency comb increases the pulse energy for a given average power. This enhances the efficiency of nonlinear frequency conversion and it facilitates extending the accessible wavelength…
We present the design of a continuous-wave, highly sensitive optical spectrometer for millimeter-wave frequencies between 50 and 1000 GHz. The spectrometer uses photomixing of near-infrared light to generate radiation in a wide frequency…
A new method, FM-FTS, combining Frequency Modulation heterodyne laser spectroscopy and Fourier Transform Spectroscopy is presented. It provides simultaneous sensitive measurement of absorption and dispersion profiles with broadband spectral…
We present a novel approach to cavity ring-down spectroscopy utilizing an optical frequency comb as the direct probe of the Fabry-Perot cavity, coupled with a time-resolved Fourier transform spectrometer for parallel retrieval of ring-down…
We discuss a simple, linear, zero-delay implementation of spectral shearing interferometry for amplitude and phase characterization of optical frequency comb sources and arbitrary waveforms. We demonstrate this technique by characterizing…
The highly energetic photons of ultraviolet light drive electronic and rovibronic transitions in all molecular species. This radiation is thus a prime tool for strongly selective spectroscopic fingerprinting and real-time environmental…
Mid-infrared (mid-IR) spectroscopy is a crucial workhorse for a plethora of analytical applications and is suitable for diverse materials, including gases, polymers or biological tissue. However, this technologically significant wavelength…
Nonlinear interferometers allow for mid-infrared spectroscopy with near-infrared detection using correlated photons. Previous implementations have demonstrated a spectral resolution limited by spectrally selective detection. In our work, we…
We present a method for absolute calibration of received radio-frequency in the ultra low frequency (ULF), and very low frequency (VLF) range. This is achieved with the use of a radio frequency optically pumped magnetometer (RF-OPM). We…
Chi-3 micro resonators have enabled compact and portable frequency comb generation, but require sophisticated dispersion control. Here we demonstrate an alternative approach using a chi-2 sheet cavity, where the dispersion requirement is…
We investigate the generation of optical frequency combs through a cascade of four-wave mixing processes in nonlinear fibres with optimised parameters. The initial optical field consists of two continuous-wave lasers with frequency…