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Electrolyte gating is a powerful technique for accumulating large carrier densities in surface two-dimensional electron systems (2DES). Yet this approach suffers from significant sources of disorder: electrochemical reactions can damage or…

By using an electrochemical gating technique with a new combination of polymer and electrolyte, we were able to inject surface charge densities n_2D as high as 3.5 \times 10^15 e/cm^2 in gold films and to observe large relative variations…

Mesoscale and Nanoscale Physics · Physics 2013-01-17 D. Daghero , F. Paolucci , A. Sola , M. Tortello , G. A. Ummarino , R. S. Gonnelli , Jijeesh R. Nair , C. Gerbaldi

Electrostatic modification of functional materials by electrolytic gating has demonstrated a remarkably wide range of density modulation, a condition crucial for developing novel electronic phases in systems ranging from complex oxides to…

Mesoscale and Nanoscale Physics · Physics 2023-07-19 Yuan Ren , Hongtao Yuan , Xiaoyu Wu , Zhuoyu Chen , Yoshihiro Iwasa , Yi Cui , Harold Y. Hwang , Keji Lai

Ionic gating is a very popular tool to investigate and control the electric charge transport and electronic ground state in a wide variety of different materials. This is due to its capability to induce large modulations of the surface…

Superconductivity · Physics 2021-05-27 Erik Piatti

Tungsten oxide and its associated bronzes (compounds of tungsten oxide and an alkali metal) are well known for their interesting optical and electrical characteristics. We have modified the transport properties of thin WO$_3$ films by…

Superconductivity · Physics 2017-07-19 X. Leng , J. Pereiro , J. Strle , G. Dubuis , A. T. Bollinger , A. Gozar , J. Wu , N. Litombe , C. Panagopoulos , D. Pavuna , I. Božović

Manipulating the electrostatic double layer and tuning the conductance in nanofluidic systems at salt concentrations of 100 mM or higher has been a persistent challenge. The primary reasons are (i) the short electrostatic proximity length,…

Using a solid electrolyte to tune the carrier density in thin-film materials is an emerging technique that has potential applications in both basic and applied research. Until now, only materials containing small ions, such as protons and…

Materials Science · Physics 2017-06-16 Jialin Zhao , Meng Wang , Xuefu Zhang , Yue Lv , Tianru Wu , Shan Qiao , Shufeng Song , Bo Gao

We have developed a technique to tune the carrier density in graphene using a lithium-ion-based solid electrolyte. We demonstrate that the solid electrolyte can be used as both a substrate to support graphene and a back gate.It can induce a…

Materials Science · Physics 2016-10-25 Jialin Zhao , Meng Wang , Hui Li , Xuefu Zhang , Lixing You , Shan Qiao , Bo Gao , Xiaoming Xie , Mianheng Jiang

We perform electric double-layer gating experiments on thin films of niobium nitride. Thanks to a cross-linked polymer electrolyte system of improved efficiency, we induce surface charge densities as high as $\approx 2.8 \times…

A Bi2Se3 topological insulator field effect transistor is investigated by using ionic liquid as an electric double layer gating material, leading to a conductance modulation of 365% at room temperature. We discuss the role of charged…

The effect of an electric field on the conductance of ultrathin films of metals deposited on substrates coated with a thin layer of amorphous Ge was investigated. A contribution to the conductance modulation symmetric with respect to the…

Superconductivity · Physics 2009-11-07 N. Markovic , C. Christiansen , G. Martinez-Arizala , A. M. Goldman

This work reports a systematic study of the evolution of charge transport mechanism in granular ultra-thin films of palladium of thickness varying between 6nm and 2nm. While the films with thickness > 4nm exhibit metallic behaviour, that at…

An interface between an oxide and an electrolyte gives rise to various processes as exemplified by electrostatic charge accumulation/depletion and electrochemical reactions such as intercalation/decalation under electric field. Here we…

Materials Science · Physics 2016-08-12 Shinichi Nishihaya , Masaki Uchida , Yusuke Kozuka , Yoshihiro Iwasa , Masashi Kawasaki

When the electron density of highly crystalline thin films is tuned by chemical doping or ionic liq- uid gating, interesting effects appear including unconventional superconductivity, sizeable spin-orbit coupling, competition with…

Mesoscale and Nanoscale Physics · Physics 2018-12-19 G. Dezi , N. Scopigno , S. Caprara , M. Grilli

Ionic liquid gating can markedly modulate the materials' carrier density so as to induce metallization, superconductivity, and quantum phase transitions. One of the main issues is whether the mechanism of ionic liquid gating is an…

The field-effect technique, popular thanks to its application in common field-effect transistors, is here applied to metallic thin films by using as a dielectric a novel polymer electrolyte solution. The maximum injected surface charge,…

Mesoscale and Nanoscale Physics · Physics 2013-12-10 M. Tortello , A. Sola , Kanudha Sharda , F. Paolucci , J. R. Nair , C. Gerbaldi , D. Daghero , R. S. Gonnelli

The correlated electron system SmNiO3 exhibits a metal-insulator phase transition at 130 {\deg}C. Using an ionic liquid as an electric double layer (EDL) gate on three-terminal ultrathin SmNiO3 devices, we investigate gate control of the…

Materials Science · Physics 2013-05-10 Sieu D. Ha , Ulrich Vetter , Jian Shi , Shriram Ramanathan

Electrolyte gating is widely used to induce large carrier density modulation on solid surfaces to explore various properties. Most of past works have attributed the charge modulation to electrostatic field effect. However, some recent…

Promising applications in photonics are driven by the ability to fabricate crystal-quality metal thin films of controlled thickness down to a few nanometers. In particular, these materials exhibit a highly nonlinear response to optical…

Mesoscale and Nanoscale Physics · Physics 2023-08-21 A. Rodríguez Echarri , F. Iyikanat , S. Boroviks , N. Asger Mortensen , Joel D. Cox , F. Javier García de Abajo

Controlling the charge density in low-dimensional materials with an electrostatic potential is a powerful tool to explore and influence their electronic and optical properties. Conventional solid gates impose strict geometrical constraints…

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