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Recent experiments suggest that the Ising pyrochlore magnets ${\rm Ho_{2}Ti_{2}O_{7}}$ and ${\rm Dy_{2}Ti_{2}O_{7}}$ display qualitative properties of the spin ice model proposed by Harris {\it et al.} \prl {\bf 79}, 2554 (1997). We discuss…

Disordered Systems and Neural Networks · Physics 2009-10-31 Byron C. den Hertog , Michel J. P. Gingras

From a microscopic model for the pyrochlore antiferromagnet Tb2Sn2O7, including the crystal field Hamiltonian and interactions between the angular momenta, we compute an effective pseudospin-1/2 Hamiltonian Heff$ that incorporates…

Statistical Mechanics · Physics 2010-11-30 Paul A. McClarty , Pawel Stasiak , Michel J. P. Gingras

We report on a study of the inelastic scattering properties of (001) and (111) Ho$_2$Ti$_2$O$_7$ single crystals at room temperature. Structural and compositional analysis along with absorption measurement confirms single crystalline phase…

Strongly Correlated Electrons · Physics 2018-05-16 Naween Anand , L. J. van de Burgt , Q. Huang , Jade Holleman , Haidong Zhou , Stephen A McGill , Christianne Beekman

Low-temperature powder neutron diffraction measurements are performed in the ordered magnetic state of the pyrochlore antiferromagnet Gd2Sn2O7. Symmetry analysis of the diffraction data indicates that this compound has the ground state…

We present a detailed theoretical overview of the thermodynamic properties of the dipolar spin ice model, which has been shown to be an excellent quantitative descriptor of the Ising pyrochlore materials Dy_2Ti_2O_7 and Ho_2Ti_2O_7. We show…

Disordered Systems and Neural Networks · Physics 2015-06-24 Roger G. Melko , Matthew Enjalran , Byron C. den Hertog , Michel. J. P. Gingras

We report the physical properties of Tb2Hf2O7 based on ac magnetic susceptibility \chi_ac(T), dc magnetic susceptibility \chi(T), isothermal magnetization M(H), and heat capacity C_p(T) measurements combined with muon spin relaxation…

Strongly Correlated Electrons · Physics 2018-03-06 V. K. Anand , L. Opherden , J. Xu , D. T. Adroja , A. D. Hillier , P. K. Biswas , T. Herrmannsdörfer , M. Uhlarz , J. Hornung , J. Wosnitza , E. Canevet , B. Lake

We report the synthesis of powder and single-crystal samples of the cerium pyrohafnate and their characterization using neutron diffraction, thermogravimetry and X-ray absorption spectroscopy. We evaluate the amount of non-magnetic…

Pyrochlore magnets of the form $R_2B_2$O$_7$, in which rare-earth ions on the $R$-site form a three-dimensional network of corner-sharing tetrahedra, provide a canonical setting for geometrical frustration. Ho-based pyrochlores host a…

Strongly Correlated Electrons · Physics 2026-04-17 A. A. Aczel , B. R. Ortiz , Y. Luo , G. Pokharel , P. M. Sarte , C. dela Cruz , J. Liu , G. Sala , S. D. Wilson , B. A. Frandsen , J. A. M. Paddison

Pyrochlore $\rm Pr^{3+}_{2+x}Zr^{4+}_{2-x}O_{7-x/2}$ samples in the form of both powders $(-0.02 \le x \le 0.02)$ and bulk single crystals have been studied to elucidate the dependence of their magnetic, compositional and structural…

Materials Science · Physics 2014-07-08 S. M. Koohpayeh , J. -J. Wen , B. A. Trump , C. L. Broholm , T. M. McQueen

The recent discovery of Spin-ice is a spectacular example of non-coplanar spin arrangements that can arise in the pyrochlore A2B2O7 structure. We present magnetic and thermodynamic studies on the metallic-ferromagnet pyrochlore Sm2Mo2O7.…

Strongly Correlated Electrons · Physics 2009-11-13 Surjeet Singh , R. Suryanarayanan , R. Tackett , G. Lawes , A. K. Sood , P. Berthet , A. Revcolevschi

Pyrochlores offer an ideal playground to investigate the magnetic ground state of frustrated magnetic systems. In this class of materials, competition between various magnetic interactions remains frustrated and prevents an ordered magnetic…

Strongly Correlated Electrons · Physics 2022-10-06 Karan Singh , Dheeraj Ranaut , G. Sharma , K. Mukherjee

The antiferromagnetic pyrochlore material NaCaCo$_2$F$_7$ is a thermal spin liquid over a broad temperature range (~ 140 K down to $T_F = 2.4 $K), in which magnetic correlations between Co$^{2+}$ dipole moments explore a continuous manifold…

Strongly Correlated Electrons · Physics 2017-04-26 K. A. Ross , J. M. Brown , R. J. Cava , J. W. Krizan , S. E. Nagler , J. A. Rodriguez-Rivera , M. B. Stone

Low temperature measurements of the ac magnetic susceptibility along the [110] direction of a single crystal of the dipolar spin ice material Ho2Ti2O7, in zero static field, are presented. While behavior that is qualitatively consistent…

Materials Science · Physics 2015-05-27 J. A. Quilliam , L. R. Yaraskavitch , H. A. Dabkowska , B. D. Gaulin , J. B. Kycia

We report new heat capacity measurements on single crystal Ce$_2$Zr$_2$O$_7$ down to $\sim$ 0.1 K in a magnetic field along the $[1,\bar{1}, 0]$ direction. These new measurements show that the broad hump in the zero-field heat capacity…

The superconducting pyrochlore oxide Cd2Re2O7 (Tc = 1 K), which is now considered as a candidate of the spin-orbit-coupled metal, shows an inversion-symmetry-breaking structural transition at Ts1 = 200 K. Ts1 decreases with increasing…

Strongly Correlated Electrons · Physics 2018-04-30 Yasuhito Matsubayashi , Takumi Hasegawa , Norio Ogita , Jun-ichi Yamaura , Zenji Hiroi

Neutron scattering measurements on the spin-ice candidate material Ho$_2$Ru$_2$O$_7$ have revealed two magnetic transitions at T $\sim$ 95 K and T $\sim$ 1.4 K to long-range ordered states involving the Ru and Ho sublattices, respectively.…

Statistical Mechanics · Physics 2009-11-10 C. R. Wiebe , J. S. Gardner , S. -J. Kim , G. M. Luke , A. S. Wills , B. D. Gaulin , J. E. Greedan , I. Swainson , Y. Qiu , C. Jones

Experimental investigation of the resistivity $\rho$, susceptibility $\chi$, specific heat C$_p$, and Hall coefficient R$_H$ of the pyrochlore Cd$_2$Re$_2$O$_7$ reveals the presence of a continuous phase transition of uncertain origin with…

Strongly Correlated Electrons · Physics 2016-08-31 R. Jin , J. He , J. R. Thompson , M. F. Chisholm , B. C. Sales , D. Mandrus

Spin liquids are highly correlated yet disordered states formed by the entanglement of magnetic dipoles$^1$. Theories typically define such states using gauge fields and deconfined quasiparticle excitations that emerge from a simple rule…

We report a detailed study of structural and magnetic properties of the pyrochlore-type (Bi2-xPrx)Ru2O7 series. Eleven compositions with 0 <= x <= 2 were prepared by solid state reaction at 1050 degrees C and found to form a solid solution…

Materials Science · Physics 2008-12-16 Siwar Zouari , Rafik Ballou , Abdelwaheb Cheikh-Rouhou , Pierre Strobel

In the ground state of Ho2Ti2O7 spin ice, the disorder of the magnetic moments follows the same rules as the proton disorder in water ice. Excitations take the form of magnetic monopoles that interact via a magnetic Coulomb interaction.…

Strongly Correlated Electrons · Physics 2013-05-24 L. J. Chang , M. R. Lees , G. Balakrishnan , Y. -J. Kao , A. D. Hillier